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arXiv:1809.02577 · Physical review. B./Physical review. B

Spectra of heavy polarons and molecules coupled to a Fermi sea

Dimitri Pimenov, Moshe Goldstein

Published Dec 12, 2018• 5 citations
arXivHTMLPDF

Abstract

We study the spectrum of an impurity coupled to a Fermi sea (e.g., minority atom in an ultracold gas, exciton in a solid) by attraction strong enough to form a molecule/trion. We introduce a diagrammatic scheme which allows treating a finite mass impurity while reproducing the Fermi-edge singularity in the immobile limit. For large binding energies the spectrum is characterized by a semicoherent repulsive polaron and an incoherent molecule-hole continuum, which is the lowest-energy feature in the single-particle spectrum. The previously predicted attractive polaron seems not to exist for strong binding.

DOI
10.1103/physrevb.98.220302

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We study the spectrum of an impurity coupled to a Fermi sea (e.g., minority atom in an ultracold gas, exciton in a solid) by attraction strong enough to form a molecule/trion. We introduce a diagrammatic scheme which allows treating a finite mass impurity while reproducing the Fermi-edge singularity in the immobile limit. For large binding energies the spectrum is characterized by a semicoherent repulsive polaron and an incoherent molecule-hole continuum, which is the lowest-energy feature in the single-particle spectrum. The previously predicted attractive polaron seems not to exist for strong binding.
The Fermi polaron, formed by an impurity interacting with a surrounding Fermi sea, exemplifies the canonical quasiparticle concept as a cornerstone in our description of quantum many-body systems across a wide range of energy scales. Experiments on atomic quantum gases have provided profound insights into the universal nature of the Fermi polaron. While most previous studies have focused on the case of zero impurity momentum, finite-momentum properties have remained largely uncharted. Here, we investigate the moving Fermi polaron by combining a novel Raman acceleration scheme with high-precision radio-frequency spectroscopy, exploring the quasiparticle dispersion relation over a wide range of momenta. We compare our measurements of energy shifts and spectral linewidths with a microscopic theory and reach quantitative agreement for all momenta. For low momenta, we find the energy of the moving polaron to be fully consistent with the Fermi liquid picture of a dressed particle with a constant effective mass. At high momenta, the polaron approaches the behavior of a weakly interacting bare particle, featuring small energy shifts and weak broadening. For intermediate momenta, broadening is generally larger and, most strikingly, the behavior differs for attractive and repulsive polarons. While the repulsive polaron exhibits a smooth connection between both regimes along with a monotonic change of the energy shift, the attractive case shows a peculiar non-monotonic behavior. With increasing momentum, the attractive polaron enters a regime where its energy deviates from the constant effective mass expression and broadening suddenly increases. By comparing this observation with theory, we show that this abrupt behavior coincides with the attractive polaron entering a molecule-hole continuum, where it is no longer the ground state. We interpret this as a motion-induced polaron-molecule transition.
We consider the highly spin-imbalanced limit of a two-component Fermi gas, where there is a small density of $\ensuremath{\downarrow}$ impurities attractively interacting with a sea of $\ensuremath{\uparrow}$ fermions. In the single-impurity limit at zero temperature, there exists the so-called polaron-molecule transition, where the impurity sharply changes its character by binding a $\ensuremath{\uparrow}$ fermion at sufficiently strong attraction. Using a recently developed variational approach, we calculate the thermodynamic properties of the impurity, and we show that the transition becomes a smooth crossover at finite temperature due to the thermal occupation of excited states in the impurity spectral function. However, remnants of the single-impurity transition are apparent in the momentum-resolved spectral function, which can in principle be probed with Raman spectroscopy. We furthermore show that the Tan contact exhibits a characteristic nonmonotonic dependence on temperature that provides a signature of the zero-temperature polaron-molecule transition. For a finite impurity density, we argue that descriptions purely based on the behavior of the Fermi polaron are invalid near the polaron-molecule transition, since correlations between impurities cannot be ignored. In particular, we show that the spin-imbalanced system undergoes phase separation at low temperatures due to the strong attraction between $\ensuremath{\uparrow}\ensuremath{\downarrow}$ molecules induced by the Fermi sea. Thus, we find that the impurity spectrum and the induced impurity-impurity interactions are key to understanding the phase diagram of the spin-imbalanced Fermi gas.
An extremely polarized mixture of an ultracold Fermi gas is expected to reduce to a Fermi polaron system, which consists of a single impurity immersed in the Fermi sea of majority atoms. By developing a many-body T -matrix theory, we investigate spectral properties of the polarized mixture in experimentally relevant regimes in which the system of finite impurity concentration at nonzero temperature is concerned. We explicitly demonstrate presence of polaron physics in the polarized limit and discuss effects of many polarons in an intermediate regime in a selfconsistent manner. By analyzing the spectral function at finite impurity concentration, we extract the attractive and repulsive polaron energies. We find that a renormalization of majority atoms via an interaction with minority atoms and a thermal depletion of the impurity chemical potential are of significance to depict the many-polaron regime.
An extremely polarized mixture of an ultracold Fermi gas is expected to reduce to a Fermi polaron system, which consists of a single impurity immersed in the Fermi sea of majority atoms. By developing a many-body T-matrix theory, we investigate spectral properties of the polarized mixture in experimentally relevant regimes in which the system of finite impurity concentration at nonzero temperature is concerned. We explicitly demonstrate presence of polaron physics in the polarized limit and discuss effects of many polarons in an intermediate regime in a selfconsistent manner. By analyzing the spectral function at finite impurity concentration, we extract the attractive and repulsive polaron energies. We find that a renormalization of majority atoms via an interaction with minority atoms is of significance to depict the many-polaron regime.
We report a study of a spin-down impurity strongly coupled to a spin-up Fermi sea (a so-called Fermi polaron) with the diagrammatic Monte Carlo (DiagMC) technique. Conditions of zero temperature and three dimensions are considered for an ultracold atomic gas with resonant interactions in the zero-range limit. A Feynman diagrammatic series is developed for the one-body and two-body propagators providing information about the polaron and molecule channel, respectively. The DiagMC technique allows us to reach diagram orders that are high enough for extrapolation to infinite order. The robustness of the extracted results is examined by checking various resummation techniques and by running the simulations with various choices for the propagators and vertex functions. It turns out that dressing the lines in the diagrams as much as possible is not always the optimal choice. We also identify classes of dominant diagrams for the one-body and two-body self-energy in the region of strong interaction. These dominant diagrams turn out to be the leading processes of the strong-coupling limit. The quasiparticle energies and ZZZ factor are obtained as a function of the interaction strength. We find that the DiagMC results for the molecule and polaron properties are very similar to those obtained with a variational ansatz. Surprisingly, this variational ansatz gives very good predictions for the quasiparticle residue even when this residue is significantly less than 1.
Using exact Bethe ansatz solutions, we show that a spin-down fermion immersed into a fully polarized spin-up Fermi sea with a weak attraction is dressed by the surrounding spin-up fermions to form the one-dimensional analog of a polaron. As the attraction becomes strong, the spin-down fermion binds with one spin-up fermion to form a tightly bound molecule. Throughout the whole interaction regime, a crossover from the polaron to a molecule state is fully demonstrated through exact results of the excitation spectrum, the effective mass, binding energy and kinetic energy. Furthermore, a clear distinction between the polaron and molecule is conceived by the probability distribution, single-particle reduced density matrix, and density-density correlations, which are calculated directly from the Bethe ansatz wave function. Such a polaron-molecule crossover presents a universal nature of an impurity immersed into a fermionic medium with an attraction in one dimension.