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arXiv:1808.07134 · Nature Communications

Unifying scrambling, thermalization and entanglement through measurement of fidelity out-of-time-order correlators in the Dicke model

Robert J. Lewis-Swan, Arghavan Safavi-Naini, J. J. Bollinger, Ana María Rey

Published Apr 5, 2019• 208 citations
arXivHTMLPDF

Abstract

Scrambling is the process by which information stored in local degrees of freedom spreads over the many-body degrees of freedom of a quantum system, becoming inaccessible to local probes and apparently lost. Scrambling and entanglement can reconcile seemingly unrelated behaviors including thermalization of isolated quantum systems and information loss in black holes. Here, we demonstrate that fidelity out-of-time-order correlators (FOTOCs) can elucidate connections between scrambling, entanglement, ergodicity and quantum chaos (butterfly effect). We compute FOTOCs for the paradigmatic Dicke model, and show they can measure subsystem Rényi entropies and inform about quantum thermalization. Moreover, we illustrate why FOTOCs give access to a simple relation between quantum and classical Lyapunov exponents in a chaotic system without finite-size effects. Our results open a path to experimental use FOTOCs to explore scrambling, bounds on quantum information processing and investigation of black hole analogs in controllable quantum systems.

DOI
10.1038/s41467-019-09436-y

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Scrambling is the process by which information stored in local degrees of freedom spreads over the many-body degrees of freedom of a quantum system, becoming inaccessible to local probes and apparently lost. Scrambling and entanglement can reconcile seemingly unrelated behaviors including thermalization of isolated quantum systems and information loss in black holes. Here, we demonstrate that fidelity out-of-time-order correlators (FOTOCs) can elucidate connections between scrambling, entanglement, ergodicity and quantum chaos (butterfly effect). We compute FOTOCs for the paradigmatic Dicke model, and show they can measure subsystem Rényi entropies and inform about quantum thermalization. Moreover, we illustrate why FOTOCs give access to a simple relation between quantum and classical Lyapunov exponents in a chaotic system without finite-size effects. Our results open a path to experimental use FOTOCs to explore scrambling, bounds on quantum information processing and investigation of black hole analogs in controllable quantum systems.
Abstract Out-of-time-order correlators (OTOCs) have emerged as the preeminent theoretical and experimental probe of quantum information scrambling — the delocalization of quantum information across many-body degrees of freedom. Here we present a comprehensive computational study of OTOCs across three paradigmatic models: the Sachdev-Ye-Kitaev (SYK) model, the non-integrable transverse-field Ising chain, and random unitary circuits. Through exact diagonalization and large-N analytics, we extract Lyapunov exponents, scrambling times, and butterfly velocities, demonstrating that all chaotic systems studied approach, but do not saturate, the Maldacena-Shenker-Stanford (MSS) bound λ_L ≤ 2π/β. Crucially, we introduce the Spectral Out-of-Time-Order Correlator (SOTOC), a novel frequency-domain diagnostic that decomposes information scrambling into its constituent spectral modes. The SOTOC achieves a 32% improvement in Lyapunov exponent extraction precision over conventional log-linear fitting and maintains robust performance at noise levels σ > 0.30, where traditional methods fail. Our phase diagram reveals a sharp transition in scrambling dynamics at h/J ≈ 1.0 in the TFIM, coinciding with the onset of quantum chaos as measured by level-spacing statistics. These results establish SOTOC as a practical and theoretically grounded tool for probing scrambling in near-term quantum devices and holographic systems.
Out-of-time-order correlators (OTOCs) can be used to probe how quickly a quantum system scrambles information when the initial conditions of the dynamics are changed. In sufficiently large quantum systems, one can extract from the OTOC the quantum analog of the Lyapunov coefficient that describes the timescale on which a classical chaotic system becomes scrambled. OTOCs have been applied only to a very limited number of toy models, such as the Sachdev-Ye-Kitaev model connected with black hole information scrambling, but they could find much wider applicability for information scrambling in quantum systems that allow comparison with experiments. The vibrations of polyatomic molecules are known to undergo a transition from regular dynamics at low energy to facile energy flow at sufficiently high energy. Molecules therefore represent ideal quantum systems to study scrambling in many-body systems of moderate size (here 6 to 36 degrees of freedoms). By computing quantum OTOCs and their classical counterparts we quantify how information becomes ``scrambled'' quantum mechanically in molecular systems. Between early ``ballistic'' dynamics, and late ``saturation'' of the OTOC when the full density of states is explored, there is indeed a regime where a quantum Lyapunov coefficient can be defined for all molecules in this study. Comparison with experimental rate data shows that slow scrambling as measured by the OTOC can reach the timescale of molecular reaction dynamics. Even for the smallest molecules we discuss, the Maldacena bound remains satisfied by regularized OTOCs, but not by unregularized OTOCs, highlighting that the former are more useful for discussing information scrambling in this type of moderate-size quantum system.
The periodically modulated Bose-Hubbard dimer model offers an experimentally realizable and highly tunable platform for observing the scrambling of quantum information and the apparent thermalization of isolated, interacting quantum many-body systems. In this work we apply fidelity out-of-time correlators (FOTOCs) to establish connections between the thermalization in the Floquet system, the exponential growth of FOTOCs as quantified by a nonzero quantum Lyapunov exponent, and the underlying classical transition from regular to chaotic dynamics in the dimer. Moreover, we demonstrate that a nonzero quantum Lyapunov exponent can also be inferred from measures quantifying the delocalization of the Floquet modes of the system such as the Shannon entropy, which approaches unity if the system thermalizes to the periodic Gibbs ensemble prediction.
Early studies on the Dicke model linked superradiance to quantum chaos, whereas later anisotropic Dicke and Rabi studies reached apparently conflicting conclusions. We resolve this tension by distinguishing global chaos from local instability. Along the isotropic Dicke path, a sweep at fixed low excitation energy crosses both the superradiant boundary and a nearby chaotic window, explaining the reported correlation. However, the anisotropic Dicke model can be chaotic in the normal phase and regular in the superradiant phase, making superradiance neither necessary nor sufficient for global chaos. A fidelity out-of-time-order correlator (FOTOC), in contrast, probes the local stability of the stationary point selected by the initial wave packet. The superradiant transition destabilizes the origin, whereas a change in anisotropy can restore its stability and create displaced saddles. Wave packets centered at these saddles exhibit exponential FOTOC growth even on a classically regular Dicke energy shell with Poisson statistics. This local sensitivity also enables quantitative spectroscopy: combined with the topology of stationary points and local density of states relations, FOTOC dynamics reconstructs the absolute amplitudes of spectral singularities in both models without fitting the density of states.
A closed quantum system never forgets its initial state, but the encoded information can get scrambled and become inaccessible without measuring a large fraction of all the system degrees of freedom. This scrambling can be diagnosed by studying the spatial spreading of initially local operators under the Heisenberg time evolution, and the decay of the out-of-time-ordered correlators (OTOC). What insights can OTOCs provide to understand the dynamics of quantum many-body systems? What are the characteristic behaviors of OTOCs during the time evolution? How is information scrambling affected by the dissipation in open quantum many-body systems? We first study slow scrambling in many-body localized systems via calculating various correlators, two-point retarded correlators and OTOCs. Comparing with retarded correlators, OTOCs provide more information about the dynamics. We find that disorder slows and partially halts the onset of information scrambling. Instead of ballistic spreading, propagation of information forms a logarithmic light cone. Next, we study the finite-size scaling of OTOCs at late times in generic thermalizing quantum many-body systems. When energy is conserved, the late-time saturation value of the OTOC of generic traceless local operators scales as an inverse polynomial in the system size. This is in contrast to the inverse exponential scaling expected for chaotic dynamics without energy conservation. We also study information scrambling in open quantum many-body systems. We define a dissipative version of OTOC and study its behaviors in a prototypical chaotic quantum chain with dissipation. We find that dissipation leads to not only the overall decay of the scrambled information due to leaking, but also structural changes so that the information light cone can only reach a finite distance even when the effect of overall decay is removed. Finally, we construct a family of local Hamiltonians for understanding the asymmetric information scrambling. Our models live on a one-dimensional lattice and exhibit asymmetric butterfly light cone between the left and right spatial directions.
Quantum scrambling describes the spreading of information into many degrees of freedom in quantum systems, such that the information is no longer accessible locally but becomes distributed throughout the system. This idea can explain how quantum systems become classical and acquire a finite temperature, or how in black holes the information about the matter falling in is seemingly erased. We probe the exponential scrambling of a multiparticle system near a bistable point in phase space and utilize it for entanglement-enhanced metrology. A time-reversal protocol is used to observe a simultaneous exponential growth of both the metrological gain and the out-of-time-order correlator, thereby experimentally verifying the relation between quantum metrology and quantum information scrambling. Our results show that rapid scrambling dynamics capable of exponentially fast entanglement generation are useful for practical metrology, resulting in a 6.8(4)-decibel gain beyond the standard quantum limit.