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arXiv:1807.09463

$Z_{2}$ spin liquid ground state of the spin-$\frac{1}{2}$ Kagome antiferromagnetic Heisenberg model

Tao Li

Published Jul 25, 2018• 1 citation
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Abstract

We show that the best variational ground state of the spin-$\frac{1}{2}$ Kagome antiferromagnetic Heisenberg model with nearest-neighboring exchange coupling(NN-KAFH) is a $Z_{2}$ spin liquid state, rather than the widely believed $U(1)$ Dirac spin liquid state. The spinon excitation in the $Z_{2}$ spin liquid state has a small gap of about $1/40$ of the spinon band width. We find that while the $Z_{2}$ and the $U(1)$ spin liquid state have a large overlap on finite clusters and are thus very close in energy, they host totally different spinon excitation spectrum. The strength of the RVB theory becomes particularly clear in such a situation, as it provides not only a variational understanding of the ground state structure, but also a comprehensive picture for the excitation spectrum of the system. Our result indicates that the spin-$\frac{1}{2}$ NN-KAFH should be better understood as a nearly critical system, rather than a prototypical gapped $Z_{2}$ spin liquid system.

DOI
10.48550/arxiv.1807.09463

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Z2Z_{2}Z2​ spin liquid ground state of the spin-12\frac{1}{2}21​ Kagome antiferromagnetic Heisenberg model
We show that the best variational ground state of the spin-12\frac{1}{2}21​ Kagome antiferromagnetic Heisenberg model with nearest-neighboring exchange coupling(NN-KAFH) is a Z2Z_{2}Z2​ spin liquid state, rather than the widely believed U(1)U(1)U(1) Dirac spin liquid state. The spinon excitation in the Z2Z_{2}Z2​ spin liquid state has a small gap of about 1/401/401/40 of the spinon band width. We find that while the Z2Z_{2}Z2​ and the U(1)U(1)U(1) spin liquid state have a large overlap on finite clusters and are thus very close in energy, they host totally different spinon excitation spectrum. The strength of the RVB theory becomes particularly clear in such a situation, as it provides not only a variational understanding of the ground state structure, but also a comprehensive picture for the excitation spectrum of the system. Our result indicates that the spin-12\frac{1}{2}21​ NN-KAFH should be better understood as a nearly critical system, rather than a prototypical gapped Z2Z_{2}Z2​ spin liquid system.
Z2_{2}2​ spin liquid phase on the kagome lattice: a new saddle point
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Competing Spin Liquid Phases in the S=12\frac{1}{2}21​ Heisenberg Model on the Kagome Lattice
The properties of ground state of spin- \frac{1}{2} 1 2 kagome antiferromagnetic Heisenberg (KAFH) model have attracted considerable interest in the past few decades, and recent numerical simulations reported a spin liquid phase. The nature of the spin liquid phase remains unclear. For instance, the interplay between symmetries and Z_2 Z 2 topological order leads to different types of Z_2 Z 2 spin liquid phases. In this paper, we develop a numerical simulation method based on symmetric projected entangled-pair states (PEPS), which is generally applicable to strongly correlated model systems in two spatial dimensions. We then apply this method to study the nature of the ground state of the KAFH model. Our results are consistent with that the ground state is a U(1) U ( 1 ) Dirac spin liquid rather than a Z_2 Z 2 spin liquid.
Motivated by recent density-matrix renormalization group (DMRG) calculations [Yan, Huse, and White, Science 332, 1173 (2011)], which claimed that the ground state of the nearest-neighbor spin-1/21/21/2 Heisenberg antiferromagnet on the kagome lattice geometry is a fully gapped spin liquid with numerical signatures of Z2{\mathbb{Z}}_{2}Z2​ gauge structure, and a further theoretical work [Lu, Ran, and Lee, Phys. Rev. B 83, 224413 (2011)], which gave a classification of all Schwinger-fermion mean-field fully symmetric Z2{\mathbb{Z}}_{2}Z2​ spin liquids on the kagome lattice, we have thoroughly studied Gutzwiller-projected fermionic wave functions by using quantum variational Monte Carlo techniques, hence implementing exactly the constraint of one fermion per site. In particular, we investigated the energetics of all Z2{\mathbb{Z}}_{2}Z2​ candidates (gapped and gapless) that lie in the neighborhood of the energetically competitive U(1) gapless spin liquids. By using a state-of-the-art optimization method, we were able to conclusively show that the U(1) Dirac state is remarkably stable with respect to all Z2{\mathbb{Z}}_{2}Z2​ spin liquids in its neighborhood, and in particular for opening a gap toward the so-called ${\mathbb{Z}}_{2}[0,\ensuremath{\pi}]\ensuremath{\beta}$ state, which was conjectured to describe the ground state obtained by the DMRG method. Finally, we also considered the addition of a small second nearest-neighbor exchange coupling of both antiferromagnetic and ferromagnetic type, and obtained similar results, namely, a U(1) Dirac spin-liquid ground state.
We find that the best resonating valence bond (RVB) state of the spin-12\frac{1}{2}21​ kagome antiferromagnetic Heisenberg model (spin-12\frac{1}{2}21​ KAFH) is described by a Z2{Z}_{2}Z2​ mean field ansatz belonging to the ${Z}_{2}[0,\ensuremath{\pi}]\ensuremath{\beta}$ class, which hosts a mean field spinon dispersion very different from that of the widely studied U(1)U(1)U(1) Dirac spin liquid state. However, we find that the physical spin fluctuation spectrum calculated from the Gutzwiller projected random phase approximation (RPA) (GRPA) theory above such an RVB state is actually gapless and is almost identical to that above the U(1)U(1)U(1) Dirac spin liquid state. We find that such a peculiar behavior can be attributed to the unique flat band physics on the kagome lattice, which makes the mapping between the mean field ansatz and the RVB state noninjective. We find that the spin fluctuation spectrum of the spin-12\frac{1}{2}21​ KAFH is not at all featureless, but is characterized by a prominent spectral peak at about 0.25J0.25J0.25J around the M\mathbf{M}M point, which is immersed in a broad continuum extending to 2.7J2.7J2.7J. Based on these results, we argue that the spectral peak below 2 meV in the inelastic neutron scattering spectrum of hebertsmithite ZnCu3(OH)6Cl2{\mathrm{ZnCu}}_{3}{(\mathrm{OH})}_{6}{\mathrm{Cl}}_{2}ZnCu3​(OH)6​Cl2​, which has been attributed to the contribution of Cu2+{\mathrm{Cu}}^{2+}Cu2+ impurity spins occupying the Zn2+{\mathrm{Zn}}^{2+}Zn2+ site, should rather be understood as the intrinsic contribution from the kagome layer. We propose to verify such a picture by measuring the Knight shift on the Cu site, rather than the O site, which is almost blind to the spin fluctuation at the M\mathbf{M}M point as a result of the strong antiferromagnetic correlation between nearest neighboring spins on the kagome lattice.
We study the energy and the static spin structure factor of the ground state of the spin-1/21/21/2 quantum Heisenberg antiferromagnetic model on the kagome lattice. By the iterative application of a few Lanczos steps on accurate projected fermionic wave functions and the Green's function Monte Carlo technique, we find that a gapless (algebraic) U(1)U(1)U(1) Dirac spin liquid is competitive with previously proposed gapped (topological) Z2{\mathbb{Z}}_{2}Z2​ spin liquids. By performing a finite-size extrapolation of the ground-state energy, we obtain an energy per site $E/J=\ensuremath{-}0.4365(2)$, which is equal, within three error bars, to the estimates given by the density-matrix renormalization group (DMRG). Our estimate is obtained for a translationally invariant system, and, therefore, does not suffer from boundary effects, like in DMRG. Moreover, on finite toric clusters at the pure variational level, our energies are lower compared to those from DMRG calculations.
We provide strong numerical evidence, using improved variational wave functions, for a ground state with vanishing spin gap in the spin-1/21/21/2 quantum Heisenberg model on the kagome lattice. Starting from the algebraic U(1)U(1)U(1) Dirac spin liquid state proposed by Ran et al. [Phys. Rev. Lett. 98, 117205 (2007)] and iteratively applying a few Lanczos steps, we compute the lowest S=2S=2S=2 excitation constructed by exciting spinons close to the Dirac nodes. Our results are compatible with a vanishing spin gap in the thermodynamic limit and in consonance with a power-law decay of long distance spin-spin correlations in real space. The competition with a gapped (topological) spin liquid is discussed.