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arXiv:1807.07257 · Physical Review A

Coherent manipulation of a three-dimensional maximally entangled state

Shi-Long Liu, Zhi‐Yuan Zhou, Shi-Kai Liu, Yin‐Hai Li, Yan Li, Chen Yang, Zhao-Huai Xu, Zhao‐Di Liu, Guang‐Can Guo, Bao-Sen Shi

Published Dec 12, 2018• 60 citations
arXivHTMLPDF

Abstract

Maximally entangled photon pairs with a spatial degree of freedom is a potential way for realizing high-capacity quantum computing and communication. However, methods to generate such entangled states with high quality, high brightness, and good controllability are needed. Here, a scheme is experimentally demonstrated that generates spatially maximally entangled photon pairs with an orbital angular momentum degree of freedom via spontaneous parametric down-conversion in a nonlinear crystal. Compared with existing methods using postselection, the technique can directly modulate the spatial spectrum of down-converted photon pairs by engineering the input pump beam. In addition, the relative phase between spatially entangled photon pairs can be easily manipulated by preparing the relative phase of input pump states.

DOI
10.1103/physreva.98.062316

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Maximally entangled photon pairs with a spatial degree of freedom is a potential way for realizing high-capacity quantum computing and communication. However, methods to generate such entangled states with high quality, high brightness, and good controllability are needed. Here, a scheme is experimentally demonstrated that generates spatially maximally entangled photon pairs with an orbital angular momentum degree of freedom via spontaneous parametric down-conversion in a nonlinear crystal. Compared with existing methods using postselection, the technique can directly modulate the spatial spectrum of down-converted photon pairs by engineering the input pump beam. In addition, the relative phase between spatially entangled photon pairs can be easily manipulated by preparing the relative phase of input pump states.
Photon pairs generated from spontaneous parametric down-conversion are a well-established method to realize entangled bipartite photonic systems. Laguerre-Gaussian modes, which carry orbital angular momentum (OAM), are commonly exploited to engineer high-dimensional entangled quantum states. For Hilbert spaces with dimension d>2d>2d>2, maximally entangled states (MESs) help to improve the capacity and security of quantum communication protocols, among several other promising features. However, the direct generation of MESs in well-defined high-dimensional subspaces of the infinite OAM basis has remained a challenge. Here, we formalize how the spatial distribution of the pump beam and the nonlinear profile of the crystal can be simultaneously utilized to generate MESs without additional spatial filtering of OAM modes within a subspace. We illustrate our approach with maximally entangled qutrits (d=3)(d=3)(d=3) and ququints (d=5)(d=5)(d=5).
High-dimensional entanglement is a valuable resource for quantum communication, and photon pairs entangled in orbital angular momentum (OAM) are commonly used for encoding high-dimensional quantum states. However, methods for the preparation of maximally entangled states of arbitrary dimensionality are still lacking, and currently used approaches essentially rely on filtering and entanglement concentration. Here, we experimentally realize a method for the generation of high-dimensional maximally entangled OAM states of photon pairs which does not require any of these procedures. Moreover, the prepared state is restricted to the subspace of the specified dimensionality, thus requiring minimal spatial postselection.
Spatial states of single photons and spatially entangled photon pairs are becoming an important resource in quantum communication. This additional degree of freedom provides an almost unlimited information capacity, making the development of high-quality sources of spatial entanglement a well-motivated research direction. We report an experimental method for generation of photon pairs in a maximally entangled spatial state. In contrast to existing techniques, the method does not require postselection of a particular subspace of spatial modes and allows one to use the full photon flux from the nonlinear crystal, providing a tool for creating high-brightness sources of pure spatially entangled photons. Such sources are a prerequisite for emerging applications in free-space quantum communication.
Photon pairs entangled in high-dimensional orbital angular momentum (OAM) degrees of freedom (DOF) have been widely regarded as a possible source for improving the capacity of quantum information processing. The generation of a high-dimensional maximally entangled state in the OAM DOF is therefore much desired. In this work, we demonstrate a simple method to generate a broader and flatter OAM spectrum, i.e., a larger spiral bandwidth (SB), of entangled photon pairs generated through spontaneous parametric down-conversion by modifying the pump beam profile. By investigating both experimentally and theoretically, we find that an exponential pump profile that is roughly the inverse of the mode profiles of the single-mode fibers used for OAM detection will provide a much larger SB compared to a Gaussian-shaped pump.
High-dimensional quantum entanglement is an important resource for fundamental research and quantum technological application. Recently, the orbital angular momentum (OAM) of light has received much attention to realize high-dimensional quantum systems, and generating and manipulating the OAM entanglement has become an important topic. Here, we propose an inverse design technique to manipulate the OAM entanglement of the photon pair generated through spontaneous parametric down-conversion. The proposed technique directly tailors the OAM states of entangled photon pairs by shaping the incident pump beam. In particular, we construct a physics-informed model by leveraging the backpropagation algorithm and adhering to the overlap integral relation. Our model automatically optimizes diffractive masks, allowing the structured pump to quantitatively modulate the OAM distribution. The generation of maximally entangled states in different dimensions is demonstrated numerically and experimentally.
We demonstrate experimental generation of spatially entangled photon pairs by spontaneous parametric down-conversion (SPDC) using a partial spatially coherent pump beam. By varying the spatial coherence of the pump, we show its influence on the down-converted photon's spatial correlations and on its degree of entanglement, in excellent agreement with theory. We then exploit this property to produce pairs of photons with a specific degree of entanglement by tailoring of the pump coherence length. This work thus unravels the fundamental transfer of coherence occurring in SPDC processes, and provides a simple experimental scheme to generate photon pairs with a well-defined degree of spatial entanglement, which may be useful for quantum communication and information processing.