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arXiv:1807.04149 · Physical Review A

Quantum hydrodynamics for supersolid crystals and quasicrystals

Vili Heinonen, Keaton J. Burns, Jörn Dunkel

Published Jun 24, 2019• 27 citations
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Abstract

Supersolids are theoretically predicted quantum states that break the continuous rotational and translational symmetries of liquids while preserving superfluid transport properties. Over the last decade, much progress has been made in understanding and characterizing supersolid phases through numerical simulations for specific interaction potentials. The formulation of an analytically tractable framework for generic interactions still poses theoretical challenges. By going beyond the usually considered quadratic truncations, we derive a systematic higher-order generalization of the Gross-Pitaevskii mean-field model in conceptual similarity with the Swift-Hohenberg theory of pattern formation. We demonstrate the tractability of this broadly applicable approach by determining the ground-state phase diagram and the dispersion relations for the supersolid lattice vibrations in terms of the potential parameters. Our analytical predictions agree well with numerical results from direct hydrodynamic simulations and earlier quantum Monte Carlo studies. The underlying framework is universal and can be extended to anisotropic pair potentials with a complex Fourier-space structure.

DOI
10.1103/physreva.99.063621

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Supersolids are theoretically predicted quantum states that break the continuous rotational and translational symmetries of liquids while preserving superfluid transport properties. Over the last decade, much progress has been made in understanding and characterizing supersolid phases through numerical simulations for specific interaction potentials. The formulation of an analytically tractable framework for generic interactions still poses theoretical challenges. By going beyond the usually considered quadratic truncations, we derive a systematic higher-order generalization of the Gross-Pitaevskii mean-field model in conceptual similarity with the Swift-Hohenberg theory of pattern formation. We demonstrate the tractability of this broadly applicable approach by determining the ground-state phase diagram and the dispersion relations for the supersolid lattice vibrations in terms of the potential parameters. Our analytical predictions agree well with numerical results from direct hydrodynamic simulations and earlier quantum Monte Carlo studies. The underlying framework is universal and can be extended to anisotropic pair potentials with a complex Fourier-space structure.
Supersolids are theoretically predicted quantum states that break the continuous rotational and translational symmetries of liquids while preserving superfluid transport properties. Over the last decade, much progress has been made in understanding and characterizing supersolid phases through numerical simulations for specific interaction potentials. The formulation of an analytically tractable framework for generic interactions still poses theoretical challenges. By going beyond the usually considered quadratic truncations, we derive a systematic higher-order generalization of the Gross-Pitaevskii mean-field model in conceptual similarity with the Swift-Hohenberg theory of pattern formation. We demonstrate the tractability of this broadly applicable approach by determining the ground state phase diagram and the dispersion relations for the supersolid lattice vibrations in terms of the potential parameters. Our analytical predictions agree well with numerical results from direct hydrodynamic simulations and earlier quantum Monte-Carlo studies. The underlying framework is universal and can be extended to anisotropic pair potentials with complex Fourier-space structure.
Abstract Within the mean field Gross–Pitaevskii framework, ultracold atomic condensates with long-range interaction are predicted to have a supersolid-like ground state beyond a critical interaction strength. Such a mean field supersolid-like ground state has periodically modulated superfluid density which implies the coexistence of superfluid and crystalline order. An ultracold atomic system in such a mean field ground state can be subjected to an artificial gauge field created either through rotation or by introducing space dependent coupling among hyperfine states of the atoms using Raman lasers. Starting from this Gross–Pitaevskii energy functional that describes such systems at zero temperature, we construct a hydrodynamic theory to describe the low-energy long-wavelength excitations of a rotating supersolid of weakly interacting ultracold atoms in two spatial dimensions for a generic type of long-range interaction. We treat the supersolidity in such a system within the framework of the well known two-fluid approximation. Considering such a system in the fast rotation limit where a vortex lattice in superfluid coexists with the supersolid lattice, we analytically obtain the dispersion relations of collective excitations around this equilibrium state. The dispersion relation gives the modes of the rotating supersolid which can be experimentally measured within the current technology. We point out that this can clearly identify an ultracold atomic supersolid phase in an unambiguous way.
In two-dimensional bosonic systems ultrasoft interactions develop an interesting phenomenology that ultimately leads to the appearance of supersolid phases in free space conditions. While suggested in early theoretical works and despite many further analytical efforts, the appearance of these exotic phases as well as the detailed shape of the ground-state phase diagrams have not been established yet. Here we develop a variational mean-field calculation for a generic quantum system with cluster-forming interactions. We show that by including the restriction of a fixed integer number of particles per cluster the ground-state phase diagram can be obtained in great detail. The great detail includes the determination of coexistence regimes of crystals of different occupancy as well as crystals with superfluid phases. To illustrate the application of the method we consider the softened van der Waals potential, for which the phase diagram is known via quantum Monte Carlo simulations. For densities other than that corresponding to the single-particle crystal, our results show very good quantitative agreement with the simulations regarding the location of the superfluid transitions. Additionally, the phase diagrams suggest that the solid-superfluid coexistence could be a reliable marker to locate supersolidity.
Quasicrystal is a class of ordered structures defying conventional classification of solid crystals and may carry classically forbidden (e.g., 5-fold) rotational symmetries. In view of long-sought supersolids, a nature question is whether the quasicrystal order can also coexist with superfluidity, forming super-quasicrystals, which spontaneously break U(1)U(1)U(1) symmetry due to superfluidity and forms quasicrystalline order that is not possessed by the underlying Hamiltonian. Here we show that a super-quasicrystal stripe state with the minimum 5-fold rotational symmetry can be realized as the ground state of a Bose-Einstein condensate in an optical superlattice with Raman-assisted tunneling. There exists a rich phase diagram consisting of various super-quasicrystal, supersolid, plane-wave phases, and their phase transitions. Our scheme can be generalized for generating other higher-order (e.g., 7-fold) quasicrystal states, and provides a platform for investigating such new exotic quantum matter.
A quasicrystal is a class of ordered structures defying conventional classification of solid crystals and may carry classically forbidden (e.g., fivefold) rotational symmetries. In view of long-sought supersolids, a natural question is whether a superfluid can spontaneously form quasicrystalline order that is not possessed by the underlying Hamiltonian, forming "superfluid-quasicrystals." Here we show that a superfluid-quasicrystal stripe state with the minimal fivefold rotational symmetry can be realized as the ground state of a Bose-Einstein condensate within a practical experimental scheme. There exists a rich phase diagram consisting of various superfluid-quasicrystal, supersolid, and plane-wave phases. Our scheme can be generalized for generating other higher-order (e.g., sevenfold) quasicrystal states, and provides a platform for investigating such new exotic quantum matter.
We study the emergence of quasicrystal configurations in the ground-state phase diagram of bosonic systems interacting through pair potentials of Lifshitz's type. By using a variational mean-field approach, we determine the relevant features of the corresponding potential interaction kind stabilizing such quasicrystalline states in two dimensions. Unlike their classical counterpart, in which the interplay between only two wave vectors determines the resulting symmetries of the solutions, the quantum picture relates in a more complex way to the instabilities of the excitation spectrum. Moreover, the quantum quasicrystal patterns are found to emerge as the ground state with no need of moderate thermal fluctuations. The study extends to the exploration of the excitation properties and the possible existence of superquasicrystals, i.e., supersolidlike quasicrystalline states in which the long-range nonperiodic density profile coexists with a nonzero superfluid fraction. Our calculations suggest that, in an intermediate region between the homogeneous superfluid and the normal quasicrystal phases, these exotic states indeed exist at zero temperature. Comparison with full numerical simulations provides a solid verification of the variational approach adopted in this paper.