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arXiv:1807.01015 · Physical Review A

Design considerations for high-purity heralded single-photon sources

Francesco Graffitti, Jérémy Kelly-Massicotte, Alessandro Fedrizzi, Agata M. Brańczyk

Published Nov 7, 2018• 58 citations
arXivHTMLPDF

Abstract

When building a parametric down-conversion photon-pair source with spectrally separable photons, e.g., for making high-purity heralded single photons, two practical issues must be accounted for: the design of the experiment, and its characterization. To address experiment design, we study the impact on spectral separability of realistic (sech-shaped and chirped) pump fields, realistic nonlinear crystals with fabrication imperfections, and undesirable PDC generation far from the central PMF peak coming from nonlinearity shaping methods. To address experiment characterization, we study the effect of discretization and spectral range of the measured biphoton joint spectrum, the difference between inferring separability from the joint spectral amplitude versus the joint spectral intensity, and advantages of interference experiments for purity characterization over methods based on the joint spectral intensity. This study will be of practical interest to researchers building the next generation of nonlinear sources of separable photon pairs.

DOI
10.1103/physreva.98.053811

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When building a parametric down-conversion photon-pair source with spectrally separable photons, e.g., for making high-purity heralded single photons, two practical issues must be accounted for: the design of the experiment, and its characterization. To address experiment design, we study the impact on spectral separability of realistic (sech-shaped and chirped) pump fields, realistic nonlinear crystals with fabrication imperfections, and undesirable PDC generation far from the central PMF peak coming from nonlinearity shaping methods. To address experiment characterization, we study the effect of discretization and spectral range of the measured biphoton joint spectrum, the difference between inferring separability from the joint spectral amplitude versus the joint spectral intensity, and advantages of interference experiments for purity characterization over methods based on the joint spectral intensity. This study will be of practical interest to researchers building the next generation of nonlinear sources of separable photon pairs.
Summary form only given. Parametric downconversion (PDC) allows the generation of highly coherent, spectrally pure single photons for quantum photonics. In a typical heralded PDC source, the signal photon emerges in a spectrally mixed state due to strong (anti)correlation in the joint spectrum of PDC photon pairs.One method for reducing spectral correlations is spectral filtering, but this compromises the heralding efficiency and the brightness of the source. A more sophisticated method for increasing the heralded photon purity is group-velocity matching, which works by erasing part of the timing information between the pump and PDC photons. What group-velocity matching cannot address, however, are the remaining correlations in the joint spectrum that come from the sinc-shaped phase-matching function (PMF) typical to standard PDC crystals. Further source engineering is therefore required to remove these correlations. Several studies have introduced domain-engineering techniques for shaping the phase matching function (PMF) in periodically poled crystals to improve single photon purities [1-4]. We present a new technique for tailoring crystal nonlinearities which combines the advantages of a deterministic method for domain engineering [4] and an annealing method developed for classical applications in higher-harmonic generation [5]. In our method, we first choose each domain orientation such that the generated field amplitude along the crystal matches the target field amplitude obtained by integrating the desired nonlinearity profile. Using a one-block structure instead of a two-blocks structure (as in [4]) results in a higher flexibility of the algorithm in tracking the target function and yields to more accurate results. We then use an annealing algorithm to slightly vary the width of each domain, further improving the effective PMF. Our technique outperforms its predecessors, particularly for short crystals, leading to high single photon purities, as shown in Fig.1. We experimentally characterise our method through a high-precision measurement of multiphoton interference between two heralded photons generated by two independent sources.We also notice that by considering a complex target field amplitude function it is possible to generalise the algorithm in [5] to any constant domain width (not necessarily equal to the coherence length), leading to a better approximation of the desired phase matching function, especially in the very short crystal regime. Moreover, tracking both the real and imaginary components of the target function allows us to approximate more exotic cases such as chirped nonlinearity profiles. Since scalable quantum photonics will require integrated architectures in which nonlinear processes are typically employed for single-photon generation, it will be interesting to explore new techniques similar to in-fibre Bragg grating structures which might yield quasi-periodic four-wave mixing and apply our algorithm to these new platforms.
One method to produce pure heralded single photons (HSP) when using the optical process of spontaneous parametric down-conversion (SPDC) is by modifying the joint spectrum of the photon pairs by means of spectral filters. In this work, we characterize the dependence, with the bandwidth of such filters, of the spectral purity and heralding efficiency of the HSP generated in a bulk SPDC. The values we report for the purity and heralding efficiency are obtained from measurements of the joint spectrum. Our results are in agreement with the theoretical model that predicts a trade-off between the purity and heralding efficiency, and they complement similar measurements that have been done for HSP produced by other types of sources.
The ability to determine the joint spectral properties of photon pairs produced by the processes of spontaneous parametric downconversion (SPDC) and spontaneous four-wave mixing (SFWM) is crucial for guaranteeing the usability of heralded single photons and polarization-entangled pairs for multi-photon protocols. In this paper, we compare six different techniques that yield either a characterization of the joint spectral intensity or of the closely related purity of heralded single photons. These six techniques include: (i) scanning monochromator measurements, (ii) a variant of Fourier transform spectroscopy designed to extract the desired information exploiting a resource-optimized technique, (iii) dispersive fibre spectroscopy, (iv) stimulated-emission-based measurement, (v) measurement of the second-order correlation function g(2) for one of the two photons, and (vi) two-source Hong–Ou–Mandel interferometry. We discuss the relative performance of these techniques for the specific cases of a SPDC source designed to be factorable and SFWM sources of varying purity, and compare the techniques’ relative advantages and disadvantages.
Photon pairs produced by parametric down-conversion or four-wave mixing can interfere with each other in multiport interferometers or carry entanglement between distant nodes for use in entanglement swapping. This requires the photons to be spectrally pure to ensure good interference and have high heralding efficiency to know accurately the number of photons involved and to maintain high rates as the number of photons grows. Spectral filtering is often used to remove noise and define spectral properties. For heralded single photons high purity and heralding efficiency are possible by filtering the heralding arm, but when both photons in typical pair sources are filtered, we show that the heralding efficiency of one or both of the photons is strongly reduced even by ideal spectral filters with 100% transmission in the passband: any improvement in reduced-state spectral purity from filtering comes at the cost of lowered heralding efficiency. We consider the fidelity to a pure, lossless single photon, symmetrize it to include both photons of the pair, and show this quantity is intrinsically limited for sources with spectral correlation. We then provide a framework for this effect for benchmarking common photon-pair sources and present an experiment where we vary the photon filter bandwidths and measure the increase in purity and corresponding reduction in heralding efficiency.
Existing nonlinear-optic implementations of pure, unfiltered heralded single-photon sources do not offer the scalability required for densely integrated quantum networks. Additionally, lithium niobate has hitherto been unsuitable for such use due to its material dispersion. We engineer the dispersion and the quasi-phasematching conditions of a waveguide in the rapidly emerging thin-film lithium niobate platform to generate spectrally separable photon pairs in the telecommunications band. Such photon pairs can be used as spectrally pure heralded single-photon sources in quantum networks. We estimate a heralded-state spectral purity of >94% based on joint spectral intensity measurements. Further, a joint spectral phase-sensitive measurement of the unheralded time-integrated second-order correlation function yields a heralded-state purity of ( 86 ± 5 ) % .