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arXiv:1807.00828 · Physical Review Letters

Identification and Control of Electron-Nuclear Spin Defects in Diamond

Alexandre Cooper, Won Kyu Calvin Sun, Jean-Christophe Jaskula, Paola Cappellaro

Published Feb 25, 2020• 26 citations
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Abstract

We experimentally demonstrate an approach to scale up quantum devices by harnessing spin defects in the environment of a quantum probe. We follow this approach to identify, locate, and control two electron-nuclear spin defects in the environment of a single nitrogen-vacancy center in diamond. By performing spectroscopy at various orientations of the magnetic field, we extract the unknown parameters of the hyperfine and dipolar interaction tensors, which we use to locate the two spin defects and design control sequences to initialize, manipulate, and readout their quantum state. Finally, we create quantum coherence among the three electron spins, paving the way for the creation of genuine tripartite entanglement. This approach will be useful in assembling multispin quantum registers for applications in quantum sensing and quantum information processing.

DOI
10.1103/physrevlett.124.083602

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We experimentally demonstrate an approach to scale up quantum devices by harnessing spin defects in the environment of a quantum probe. We follow this approach to identify, locate, and control two electron-nuclear spin defects in the environment of a single nitrogen-vacancy center in diamond. By performing spectroscopy at various orientations of the magnetic field, we extract the unknown parameters of the hyperfine and dipolar interaction tensors, which we use to locate the two spin defects and design control sequences to initialize, manipulate, and readout their quantum state. Finally, we create quantum coherence among the three electron spins, paving the way for the creation of genuine tripartite entanglement. This approach will be useful in assembling multispin quantum registers for applications in quantum sensing and quantum information processing.
Nitrogen-vacancy centers in diamond are sensitive probes of time-varying magnetic fields that can be used to identify unknown spin defects in their nearby environment. Performing spectral quantum measurements on such single quantum probes enables gaining information about the internal structure and dynamics of nearby spin defects that would otherwise be inaccessible through direct or indirect measurements with classical probes. Here, we identify a system composed of two electron-nuclear spin defects in a diamond crystal by performing a series of spectral identification measurements using a single nitrogen-vacancy center in diamond. Besides enabling the identification of new spin defects and studies of their formation mechanisms, these techniques will be useful for scaling up quantum systems by converting environmental spin defects into quantum resources.
A promising approach for multi-qubit quantum registers is to use optically addressable spins to control multiple dark electron-spin defects in the environment. While recent experiments have observed signatures of coherent interactions with such dark spins, it is an open challenge to realize the individual control required for quantum information processing. Here, we demonstrate the heralded initialisation, control and entanglement of individual dark spins associated to multiple P1 centers, which are part of a spin bath surrounding a nitrogen-vacancy center in diamond. We realize projective measurements to prepare the multiple degrees of freedom of P1 centers-their Jahn-Teller axis, nuclear spin and charge state-and exploit these to selectively access multiple P1s in the bath. We develop control and single-shot readout of the nuclear and electron spin, and use this to demonstrate an entangled state of two P1 centers. These results provide a proof-of-principle towards using dark electron-nuclear spin defects as qubits for quantum sensing, computation and networks.
Isolated nuclear spins provide a promising building block for quantum information science, motivating development of techniques to characterize, control, and detect them in suitable systems. Working with the nitrogen-vacancy center in diamond, we demonstrate robust initialization, manipulation, and readout of individual 13C^{13}\text{C}13C, 15N^{15}\text{N}15N, and 14N^{14}\text{N}14N nuclear spins and identify a mechanism to extend our results to arbitrary magnetic field environments. These techniques enable precise characterization of nuclear-spin hyperfine parameters and coherence properties and may pave the way for nuclear-spin-based quantum information architectures in diamond.
Electronic spin defects in the environment of an optically active spin can be used to increase the size and hence the performance of solid-state quantum registers, especially for applications in quantum metrology and quantum communication. Previous works on multiqubit electronic spin registers in the environment of a nitrogen-vacancy (NV) center in diamond have only included spins directly coupled to the NV. As this direct coupling is limited by the central spin coherence time, it significantly restricts the maximum attainable size of the register. To address this problem, we present a scalable approach to increase the size of electronic spin registers. Our approach exploits a weakly coupled probe spin together with double-resonance control sequences to mediate the transfer of spin polarization between the central NV spin and an environmental spin that is not directly coupled to it. We experimentally realize this approach to demonstrate the detection and coherent control of an unknown electronic spin outside the coherence limit of a central NV. Our work paves the way for engineering larger quantum spin registers with the potential to advance nanoscale sensing, enable correlated noise spectroscopy for error correction, and facilitate the realization of spin-chain quantum wires for quantum communication. Published by the American Physical Society 2024
The key challenge in experimental quantum information science is to identify isolated quantum mechanical systems with long coherence times that can be manipulated and coupled together in a scalable fashion. We describe the coherent manipulation of an individual electron spin and nearby individual nuclear spins to create a controllable quantum register. Using optical and microwave radiation to control an electron spin associated with the nitrogen vacancy (NV) color center in diamond, we demonstrated robust initialization of electron and nuclear spin quantum bits (qubits) and transfer of arbitrary quantum states between them at room temperature. Moreover, nuclear spin qubits could be well isolated from the electron spin, even during optical polarization and measurement of the electronic state. Finally, coherent interactions between individual nuclear spin qubits were observed and their excellent coherence properties were demonstrated. These registers can be used as a basis for scalable, optically coupled quantum information systems.
Robust entanglement at room temperature is a necessary requirement for practical applications in quantum technology. We demonstrate the creation of bipartite- and tripartite-entangled quantum states in a small quantum register consisting of individual 13C nuclei in a diamond lattice. Individual nuclear spins are controlled via their hyperfine coupling to a single electron at a nitrogen-vacancy defect center. Quantum correlations are of high quality and persist on a millisecond time scale even at room temperature, which is adequate for sophisticated quantum operations.