Quasicrystals are long-range ordered and yet nonperiodic. This interplay results in a wealth of intriguing physical phenomena, such as the inheritance of topological properties from higher dimensions, and the presence of nontrivial structure on all scales. Here, we report on the first experimental demonstration of an eightfold rotationally symmetric optical lattice, realizing a two-dimensional quasicrystalline potential for ultracold atoms. Using matter-wave diffraction we observe the self-similarity of this quasicrystalline structure, in close analogy to the very first discovery of quasicrystals using electron diffraction. The diffraction dynamics on short timescales constitutes a continuous-time quantum walk on a homogeneous four-dimensional tight-binding lattice. These measurements pave the way for quantum simulations in fractal structures and higher dimensions.
Quasicrystals are long-range ordered and yet nonperiodic. This interplay results in a wealth of intriguing physical phenomena, such as the inheritance of topological properties from higher dimensions, and the presence of nontrivial structure on all scales. Here, we report on the first experimental demonstration of an eightfold rotationally symmetric optical lattice, realizing a two-dimensional quasicrystalline potential for ultracold atoms. Using matter-wave diffraction we observe the self-similarity of this quasicrystalline structure, in close analogy to the very first discovery of quasicrystals using electron diffraction. The diffraction dynamics on short timescales constitutes a continuous-time quantum walk on a homogeneous four-dimensional tight-binding lattice. These measurements pave the way for quantum simulations in fractal structures and higher dimensions.
Quasicrystals are long-range ordered and yet non-periodic. This interplay results in a wealth of intriguing physical phenomena, such as the inheritance of topological properties from higher dimensions, self-similarity, and the presence of non-trivial structure on all scales. The concept of aperiodic order has been extensively studied in mathematics and geometry, exemplified by the celebrated Penrose tiling. However, the understanding of physical quasicrystals (the vast majority of them are intermetallic compounds) is still incomplete owing to their complexity, regarding both growth processes and stability. Ultracold atoms in optical lattices offer an ideal, yet untested environment for investigating quasicrystals. Optical lattices, i.e. standing waves of light, allow the defect-free formation of a large variety of potential landscapes, including quasiperiodic geometries. In recent years, optical lattices have become one of the most successful tools in the large-scale quantum simulation of condensed-matter problems. This study presents the first experimental realisation of a two-dimensional quasicrystalline potential for ultracold atoms, based on an eightfold symmetric optical lattice. It is aimed at bringing together the fields of ultracold atoms and quasicrystals – and the more general concept of aperiodic order. The first part of this thesis introduces the theoretical aspects of aperiodic order and quasicrystalline structure. The second part comprises a detailed account of the newly designed apparatus that has been used to produce quantum-degenerate gases in quasicrystalline lattices. The third and final part summarises the matter-wave diffraction experiments that have been performed in various lattice geometries. These include one- and two-dimensional simple cubic lattices, one-dimensional quasiperiodic lattices, as well as two-dimensional quasicrystalline lattices. The striking self-similarity of this quasicrystalline structure has been directly observed, in close analogy to Shechtman’s very first discovery of quasicrystals using electron diffraction. In addition, an in-depth study of the diffraction dynamics reveals the fundamental differences between periodic and quasicrystalline lattices, in excellent agreement with ab initio theory. The diffraction dynamics on short timescales constitutes a continuous-time quantum walk on a homogeneous four-dimensional tight-binding lattice. On the one hand, these measurements establish a novel experimental platform for investigating quasicrystals proper. On the other hand, ultracold atoms in quasicrystalline optical lattices are worth studying in their own right: Possible avenues include the observation many-body localisation and Bose glasses, as well as the creation of topologically non-trivial systems in higher dimensions.
Quasicrystals are long-range ordered and yet non-periodic. This interplay results in a wealth of intriguing physical phenomena, such as self-similarity, the inheritance of topological properties from higher dimensions, and the presence of non-trivial structure on all lengthscales. However, quasicrystalline materials are notoriously hard to synthesise, as defects and impurities may greatly alter their final microscopic composition. The field of quantum simulation with ultracold atoms offers a solution to this problem, namely the use of optical lattices – standing waves of light. Optical lattices are free of impurities and therefore ideally suited to study quasicrystals, enabling unprecedented access to observables that are unattainable in condensed matter systems. This study presents the first experimental realisation of a two-dimensional quasicrystalline potential for ultracold atoms, based on an eightfold symmetric optical lattice. Features pertaining to both ordered and disordered phases are observed, from sharp diffraction peaks in the matter-wave interference pattern, to a disorder-induced localised phase emerging at a critical lattice depth V_loc ~ 1.78 E_rec. The localised phase seems to be resilient against moderate interactions, which would make this the first experimental realisation of a 2D Bose glass.
This thesis concerns the physics of ultracold bosons in quasicrystalline lattices, studied by means of quantum simulation using ultracold 39K atoms loaded to an eight-fold rotationally symmetric optical quasicrystal. Quasicrystalline and quasiperiodic systems, thanks to their long-range order and lack of periodicity, exhibit a wealth of interesting properties such as a dense and self-similar momentum space, and a localization transition to Anderson insulator or Bose glass states (in non-interacting or interacting cases respectively) reminiscent of that in disordered systems, whilst lacking the rare regions that typically exist in such systems. Here we will cover experiments into this system’s behaviour in both equilibrium and non-equilibrium settings. First, we focus on mapping out its phase diagram in both weakly and strongly interacting regimes. We observe consistency with numerical predictions for the superfluid-Bose glass phase transition using coherence measurements, as well as finding a region of roughly zero compressibility around where the numerics predicts the existence of a Mott insulator ground state. We also study which regimes of the phase diagram can be ramped through adiabatically, finding that entropy is created upon traversing the Bose glass phase irrespective of ramp duration, which we attribute to its localized nature. Next we look into the dynamics of the system after a quench of the lattice depth in the weakly interacting regime. Upon quenching from the superfluid regime to the Bose glass regime, we observe a quantum walk to higher order diffraction peaks in momentum space whose maximum order is unbounded by kinetic energy thanks to the dense, self-similar nature of the quasicrystal’s momentum space. Quenching in the opposite direction we observe instead a walk between sites in real space for short times by looking at the position (as opposed to momentum) space autocorrelation function of the cloud, finding an expansion rate in agreement with an intuitive estimate based on the Lieb-Robinson bounds of a periodic system. We also look into the timescales of these dynamics in the context of what we might expect from the underlying Hamiltonian, before finally investigating the loss of coherence exhibited by the system after a slower quench of the lattice depth from an initially superfluid cloud. We observe that coherence is lost sooner after the quench for deeper final lattices, with the loss becoming almost instantaneous for quenches that cross the localization transition across the whole cloud. After this we explore the system’s transport dynamics by means of a quench to an excited state at the same time as an additional confining potential is switched off. We observe that unlike in the case of a periodic square lattice, where ballistic expansion that scales with the tunnelling strength occurs in the non-interacting case before becoming slower upon the introduction of interactions thanks to diffusion, in the quasicrystal the transport rate no longer scales with tunnelling strength. Instead we observe a drop relative to the tunnelling rate by 2 − 3 orders of magnitude as the lattice depth is increased from 1Er to 5Er with little dependence on the interaction strength. We also note that the finite rate measured for the deeper lattices is potentially an overestimate since the finite loss rate of atoms makes mass transport indistinguishable from density-dependent losses at that point. Finally, we discuss use of a quantum gas magnification scheme with which to magnify the real space density distribution of our atoms such that it can be measured with single-site resolution. Some preliminary results are presented regarding how the density distribution changes with lattice depth in the weakly interacting regime, in which we observe that as lattice depth increases a higher proportion of atoms occupy deeper sites close to the centre of the quasicrystal’s configuration space, as we might expect.
Quasicrystals are long-range ordered but not periodic, representing an interesting middle ground between order and disorder. We experimentally and numerically study the localization transition in the ground state of noninteracting and weakly interacting bosons in an eightfold symmetric quasicrystalline optical lattice. In contrast to typically used real space in situ techniques, we probe the system in momentum space by recording matter wave diffraction patterns. Shallow lattices lead to extended states whereas we observe a localization transition at a critical lattice depth of V_{0}≈1.78(2)E_{rec} for the noninteracting system. Our measurements and Gross-Pitaevskii simulations demonstrate that in interacting systems the transition is shifted to deeper lattices, as expected from superfluid order counteracting localization. Quasiperiodic potentials, lacking conventional rare regions, provide the ideal testing ground to realize many-body localization in 2D.
The discovery of quasicrystals with crystallographically forbidden rotational symmetries has changed the notion of the ordering in materials, yet little is known about the dynamical emergence of such exotic forms of order. Here we theoretically study a nonequilibrium cavity-QED setup realizing a zero-temperature quantum phase transition from a homogeneous Bose-Einstein condensate to a quasicrystalline phase via collective superradiant light scattering. Across the superradiant phase transition, collective light scattering creates a dynamical, quasicrystalline optical potential for the atoms. Remarkably, the quasicrystalline potential is "emergent" as its eightfold rotational symmetry is not present in the Hamiltonian of the system, rather appears solely in the low-energy states. For sufficiently strong two-body contact interactions between atoms, a quasicrystalline order is stabilized in the system, while for weakly interacting atoms the condensate is localized in one or few of the deepest minima of the quasicrystalline potential.
Quasicrystals exhibit exotic properties inherited from the self-similarity of their long-range ordered, yet aperiodic, structure. The recent realization of optical quasicrystal lattices paves the way to the study of correlated Bose fluids in such structures, but the regime of strong interactions remains largely unexplored, both theoretically and experimentally. Here, we determine the quantum phase diagram of two-dimensional correlated bosons in an eightfold quasicrystal potential. Using large-scale quantum Monte Carlo calculations, we demonstrate a superfluid-to-Bose glass transition and determine the critical line. Moreover, we show that strong interactions stabilize Mott insulator phases, some of which have spontaneously broken eightfold symmetry. Our results are directly relevant to current generation experiments and, in particular, drive prospects to the observation of the still elusive Bose glass phase in two dimensions and exotic Mott phases.