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arXiv:1806.08774 · Journal of Physics B Atomic Molecular and Optical Physics

Impact of detuning and dephasing on a laser-corrected subnatural-linewidth single-photon source

J C López Carreño, E Zubizarreta Casalengua, Fabrice P. Laussy, E del Valle

Published Dec 6, 2018• 5 citations
arXivHTMLPDF

Abstract

Abstract The elastic scattering peak of a resonantly driven two-level system has been argued to provide narrow-linewidth antibunched photons. Although independent measurements of spectral width on the one hand and antibunching, on the other hand, do seem to show that this is the case, a joint measurement reveals that only one or the other of these attributes can be realised in the direct emission. We discuss a scheme which interferes the emission with a laser to produce simultaneously single photons of subnatural linewidth. In particular, we consider the effect of dephasing and of the detuning between the driving laser and/or the detector with the emitter. We find that our scheme brings such considerable improvement as compared to the standard schemes as to make it the best single-photon source in terms of all-order multi-photon suppression by several orders of magnitudes. While the scheme is particularly fragile to dephasing, its superiority holds even for subnatural-linewidth emission down to a third of the radiative lifetime.

DOI
10.1088/1361-6455/aaf68d

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Abstract The elastic scattering peak of a resonantly driven two-level system has been argued to provide narrow-linewidth antibunched photons. Although independent measurements of spectral width on the one hand and antibunching, on the other hand, do seem to show that this is the case, a joint measurement reveals that only one or the other of these attributes can be realised in the direct emission. We discuss a scheme which interferes the emission with a laser to produce simultaneously single photons of subnatural linewidth. In particular, we consider the effect of dephasing and of the detuning between the driving laser and/or the detector with the emitter. We find that our scheme brings such considerable improvement as compared to the standard schemes as to make it the best single-photon source in terms of all-order multi-photon suppression by several orders of magnitudes. While the scheme is particularly fragile to dephasing, its superiority holds even for subnatural-linewidth emission down to a third of the radiative lifetime.
Abstract Resonance fluorescence—the light emitted when exciting resonantly a two-level system—is a popular quantum source as it seems to inherit its spectral properties from the driving laser and its statistical properties from the two-level system, thus providing a subnatural-linewidth single-photon source (SPS). However, these two qualities do not actually coexist in resonance fluorescence, since an optical target detecting these antibunched photons will either be spectrally broad itself and not benefit from the spectrally narrow source, or match spectrally with the source but in this case the antibunching will be spoiled. We first explain this failure through a decomposition of the field-emission and how this gets affected by frequency resolution. We then show how to restore the sought joint subnatural linewidth and antibunched properties, by interfering the resonance fluorescence output with a coherent beam. We finally discuss how the signal that is eventually generated in this way features a new type of quantum correlations, with a plateau of antibunching which suppresses much more strongly close photon pairs. This introduces a new concept of perfect SPS.
Resonance fluorescence has played a major role in quantum optics with predictions and later experimental confirmation of nonclassical features of its emitted light such as antibunching or squeezing. In the Rayleigh regime where most of the light originates from the scattering of photons with subnatural linewidth, antibunching would appear to coexist with sharp spectral lines. Here, we demonstrate that this simultaneous observation of subnatural linewidth and antibunching is not possible with simple resonant excitation. Using an epitaxial quantum dot for the two-level system, we independently confirm the single-photon character and subnatural linewidth by demonstrating antibunching in a Hanbury Brown and Twiss type setup and using high-resolution spectroscopy, respectively. However, when filtering the coherently scattered photons with filter bandwidths on the order of the homogeneous linewidth of the excited state of the two-level system, the antibunching dip vanishes in the correlation measurement. Our observation is explained by antibunching originating from photon-interferences between the coherent scattering and a weak incoherent signal in a skewed squeezed state. This prefigures schemes to achieve simultaneous subnatural linewidth and antibunched emission.
The observation of quantum-dot resonance fluorescence enabled a new solid-state approach to generating single photons with a bandwidth approaching the natural linewidth of a quantum-dot transition. Here, we operate in the small Rabi frequency limit of resonance fluorescence--the Heitler regime--to generate subnatural linewidth and high-coherence quantum light from a single quantum dot. The measured single-photon coherence is 30 times longer than the lifetime of the quantum-dot transition, and the single photons exhibit a linewidth which is inherited from the excitation laser. In contrast, intensity-correlation measurements reveal that this photon source maintains a high degree of antibunching behavior on the order of the transition lifetime with vanishing two-photon scattering probability. Generating decoherence-free phase-locked single photons from multiple quantum systems will be feasible with our approach.
The photon blockade is a key quantum-nonlinear effect in which the admission of a second photon to a resonator is inhibited, enabling on-demand single-photon emission. Its practical use is limited by the weak intrinsic nonlinearity of most optical platforms. We address this limitation in a coupled-cavity architecture by engineering two-photon dissipation as a control resource rather than a detrimental loss. Within a quantum-master-equation framework, we model single-photon loss, engineered two-photon decay, and pure dephasing, and analyze their joint impact on the steady-state statistics of the driven cavities. We track the zero-delay correlation, photon populations, and detuning/drive dependences under distinct driving schemes (both cavities driven vs. single-cavity drive with. The results show that adding two-photon dissipation (i) suppresses multiphoton occupation and strengthens antibunching, (ii) broadens the operating window in detuning and drive amplitude, and (iii) improves robustness against moderate dephasing and device imperfections. A mechanism analysis attributes these gains to interference between coherent second-order processes and dissipative selection that stabilizes the odd-photon manifold. The study yields design guidelines for realizing stable, cavity-based single-photon sources using dissipation engineering.
Recent works [PhysRevLett.125.170402 (2020) and PhysRevLett.125.043603 (2020)] verify that the perfect single-photon character is a global property of resonance fluorescence including all the spectral components, and then the absence of some components can spoil the single-photon character, which considerably limits the application of filtering scheme to obtain single-photon source (SPS) with subnatural linewidth. Here, we note that the linewidth of fluorescent photon is not always limited by the intrinsic linewidth of the emitter, and provide a scheme where the linewidth of the fluorescent single photon can be much smaller than the natural linewidth of emitter by manipulating external coherent fields. By simulating the response of the filter or detection setup with a bandwidth approaching and even much smaller than the natural linewidth of emitter, the realization of ultranarrow SPS can be confirmed. Besides, we demonstrate that this scheme of ultranarrow SPS can be implemented based on various real physical platforms.
Single-photon purity is one of the most important key metrics of many quantum states of light. For applications in photonic quantum technologies, e.g. quantum communication and linear optical quantum computing, a minimization of the multi-photon error rate is required because of its error-introducing nature. Ultimately, the purity of state-of-the-art single-photon sources was found to be limited by spontaneous emission and subsequent reexcitation during the interaction with the driving field. Here, we demonstrate that even this fundamental limit to the single-photon purity can be overcome due to the distinct spectro-temporal properties of the individual photons forming multi-photon errors. For driving pulses shorter than the emitter lifetime, we find that photons emitted during the pulse exhibit a significantly broader spectral shape than the emitter's natural linewidth. Thus, we can selectively filter out the majority of this instantaneously emitted photon by employing narrowband spectral filters, which reduces the measured degree of second-order coherence at zero time delay by almost one order of magnitude. This enables a significant suppression of the multi-photon error rate without detrimental effects on the desired single-photon emission.