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arXiv:1804.09608 · Physical review. B./Physical review. B

Control of competing superconductivity and charge order by nonequilibrium currents

Anne Matthies, Jiajun Li, Martin Eckstein

Published Nov 13, 2018• 13 citations
arXivHTMLPDF

Abstract

We study the competing charge-density-wave and superconducting order in the attractive Hubbard model under a voltage bias, using steady-state nonequilibrium dynamical mean-field theory. We show that the charge-density wave is suppressed in a current-carrying nonequilibrium steady state. This effect is beyond a simple Joule-heating mechanism and a ``supercooled'' metallic state is stabilized at a nonequilibrium temperature lower than the equilibrium superconducting ${T}_{c}$. On the other hand, a current-carrying superconducting state is dissipationless and thus not subject to the same nonthermal suppression, and can therefore nucleate out of the supercooled metal, e.g., in a resistive switching experiment. The fact that an electric current can change the relative stability of different phases compared to thermal equilibrium, even when a system appears locally thermal due to electron-electron scattering, provides a general perspective to control intertwined orders out of equilibrium.

DOI
10.1103/physrevb.98.180502

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We study the competing charge-density-wave and superconducting order in the attractive Hubbard model under a voltage bias, using steady-state nonequilibrium dynamical mean-field theory. We show that the charge-density wave is suppressed in a current-carrying nonequilibrium steady state. This effect is beyond a simple Joule-heating mechanism and a ``supercooled'' metallic state is stabilized at a nonequilibrium temperature lower than the equilibrium superconducting Tc{T}_{c}Tc​. On the other hand, a current-carrying superconducting state is dissipationless and thus not subject to the same nonthermal suppression, and can therefore nucleate out of the supercooled metal, e.g., in a resistive switching experiment. The fact that an electric current can change the relative stability of different phases compared to thermal equilibrium, even when a system appears locally thermal due to electron-electron scattering, provides a general perspective to control intertwined orders out of equilibrium.
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We investigate the nonequilibrium dynamics of competing coexisting superconducting (SC) and charge-density wave (CDW) orders in an attractive Hubbard model. A time-periodic laser field A[over →](t) lifts the SC-CDW degeneracy, since the CDW couples linearly to the field (A[over →]), whereas SC couples in second order (A[over →]^{2}) due to gauge invariance. This leads to a striking resonance: When the photon energy is red detuned compared to the equilibrium single-particle energy gap, CDW is enhanced and SC is suppressed, while this behavior is reversed for blue detuning. Both orders oscillate with an emergent slow frequency, which is controlled by the small amplitude of a third induced order, namely η pairing, given by the commutator of the two primary orders. The induced η pairing is shown to control the enhancement and suppression of the dominant orders. Finally, we demonstrate that light-induced superconductivity is possible starting from a predominantly CDW initial state.
We study how strongly correlated electrons on a dissipative lattice evolve out of equilibrium under a constant electric field, focusing on the extent of the linear regime and hysteretic nonlinear effects at higher fields. We access the nonequilibrium steady states, nonperturbatively in both the field and the electronic interactions, by means of a nonequilibrium dynamical mean-field theory in the Coulomb gauge. The linear response regime, limited by Joule heating, breaks down at fields much smaller than the quasiparticle energy scale. For large electronic interactions, strong but experimentally accessible electric fields can induce a resistive switching by driving the strongly correlated metal into a Mott insulator. We predict a nonmonotonic upper switching field due to an interplay of particle renormalization and the field-driven temperature. Hysteretic I-V curves suggest that the nonequilibrium current is carried through a spatially inhomogeneous metal-insulator mixed state.
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We study the charge-density-wave order and its competition with superconductivity in the one-band Hubbard model for high-Tc{T}_{c}Tc​ superconducting cuprates. We use cluster dynamical mean field theory at T=0T=0T=0. The one-band Hubbard model contains only copper atoms, and a physical charge-density wave with charge excesses located on the oxygen atoms manifests itself as a bond-density wave (BDW) within this context. It arises purely out of local correlation effects and also leads to an ${s}^{\ensuremath{'}}$-wave pair-density wave in the presence of ddd-wave superconductivity. The ddd-wave BDW is suppressed on increasing UUU and is favored on increasing the magnitude of the second-neighbor hopping ${t}^{\ensuremath{'}}$. Further, the ddd-wave BDW order is weakened when in competition with superconductivity, as seen in experiments. Additionally, it behaves quite differently on varying UUU in the superconducting state compared to the normal state.
Pump-probe experiments have turned out as a powerful tool in order to study the dynamics of competing orders in a large variety of materials. The corresponding analysis of the data often relies on standard linear-response theory generalized to nonequilibrium situations. Here we examine the validity of such an approach for the charge and pairing response of systems with charge-density wave and (or) superconducting (SC) order. Our investigations are based on the attractive Hubbard model which we study within the time-dependent Hartree-Fock approximation. In particular, we calculate the quench and pump-probe dynamics for SC and charge order parameters in order to analyze the frequency spectra and the coupling of the probe field to the specific excitations. Our calculations reveal that the ``linear-response assumption'' is justified for small to moderate nonequilibrium situations (i.e., pump pulses) in the case of a purely charge-ordered ground state. However, the pump-probe dynamics on top of a superconducting ground state is determined by phase and amplitude modes which get coupled far from the equilibrium state indicating the failure of the linear-response assumption.