In the ultrastrong coupling regime, light and matter can no longer be distinguished: their coupling strengths are as large as their own energy scales. Even for simple two-level systems, this represents a new regime to explore within the quantum Rabi model. There has been considerable theoretical and experimental progress on the physics of these systems in recent years, as presented in this review. Key experimental results are discussed in a set of current platforms arising in quantum information research, including superconducting and semiconducting devices, and other hybrid quantum systems.
In the ultrastrong coupling regime, light and matter can no longer be distinguished: their coupling strengths are as large as their own energy scales. Even for simple two-level systems, this represents a new regime to explore within the quantum Rabi model. There has been considerable theoretical and experimental progress on the physics of these systems in recent years, as presented in this review. Key experimental results are discussed in a set of current platforms arising in quantum information research, including superconducting and semiconducting devices, and other hybrid quantum systems.
In the last decades, the experimental and theoretical study of light-matter interactions in confined quantum systems has allowed to considerably widen and deepen our understanding of the quantum world.The simplest fully-quantized light-matter interaction is the quantum Rabi model (QRM), where a two-level system is coupled to a single bosonic mode.The implementation of quantum-optical systems in which the interaction strength overcomes losses brought a revolution to this research area.Under this condition, dubbed strong coupling (SC) regime, quantum processes can be observed at the single-photon level, and even exploited to perform Quantum Information tasks.Recent developments in solid-state Quantum Technologies have made possible to push the line further, achieving the ultrastrong coupling (USC) regime of the QRM, in which the interaction strength is comparable with the bare frequencies of the interacting systems.In the USC regime of the QRM, light and matter degrees of freedom merge into collective bound states called polaritons, the system ground state is not the vacuum and excitations are not conserved.The growing interest in USC-related phenomena is mainly motivated by the fundamental counterintuitive modifications to light-matter interactions entailed by this regime.At the same time, the USC regime is also expected to provide computational benefits in terms of operational speed, coherence time, and noise protection.In this Thesis, we theoretically analyze novel quantum phenomena emerging in the USC regime, which can be observed using nowadays technology and can motivate foreseeable improvements.The results here presented have been derived using two conceptually different approaches.On one side, we have analyzed interesting models that can be implemented in superconducting circuits, a quantum platform where the USC regime can be naturally achieved.In particular, we focused on excitation transfer across USC impurities, entanglement generation via modulation of electrical boundary conditions and quantum state engineering in ultrastrongly-coupled systems.On the other hand, we have developed methods to reproduce the physics of light-matter interactions in the USC regime, by tailoring the Hamiltonian of atomic systems, like trapped ions and cold atoms.These proposals take profit of the specific features of such quantum platforms, in order to implement regimes and measurements that are not directly accessible.We believe that this Thesis will contribute to develop a thorough understanding of quantum phenomena related to the USC regime of light-matter interaction, and that it will foster the dialog between experimental and theoretical research in this area.I would like to thank first my PhD supervisor Prof. Enrique Solano, for his constant support and invaluable guidance.Countless thought-provoking discussions held with him during my PhD studies have contributed to develop my critical skills, and his advice has covered all facets of nowadays top-level research.
Ultrastrong coupling between light and matter has, in the past decade, transitioned from a theoretical idea to an experimental reality. It is a new regime of quantum light–matter interaction, which goes beyond weak and strong coupling to make the coupling strength comparable to the transition frequencies in the system. The achievement of weak and strong coupling has led to increased control of quantum systems and to applications such as lasers, quantum sensing, and quantum information processing. Here we review the theory of quantum systems with ultrastrong coupling, discussing entangled ground states with virtual excitations, new avenues for nonlinear optics, and connections to several important physical models. We also overview the multitude of experimental setups, including superconducting circuits, organic molecules, semiconductor polaritons, and optomechanical systems, that have now achieved ultrastrong coupling. We conclude by discussing the many potential applications that these achievements enable in physics and chemistry.
The interaction of light and matter at the single-photon level is of central importance in various fields of physics, including, e.g., condensed matter physics, astronomy, quantum optics, and quantum information. Amplification of such quantum light–matter interaction can be highly beneficial to, e.g., improve device performance, explore novel phenomena, and understand fundamental physics, and has therefore been a long-standing goal. Furthermore, simulation of light–matter interaction in the regime of ultrastrong coupling, where the interaction strength is comparable to the bare frequencies of the uncoupled systems, has also become a hot research topic, and considerable progress has been made both theoretically and experimentally in the past decade. In this review, we provide a detailed introduction of recent advances in amplification of quantum light–matter interaction and simulation of ultrastrong light–matter interaction, particularly in cavity and circuit quantum electrodynamics and in cavity optomechanics.
Abstract This article reviews theoretical methods developed in the last decade to understand cavity quantum electrodynamics in the ultrastrong‐coupling regime, where the strength of the light–matter interaction becomes comparable to the photon frequency. Along with profound modifications of fundamental quantum optical effects giving rise to a rich phenomenology, this regime introduces significant theoretical challenges. One of the most important is the break‐down of the rotating‐wave approximation which neglects all non‐resonant terms in light–matter interaction Hamiltonians. Consequently, a large part of the quantum optical theoretical framework has to be revisited in order to accurately account for all interaction terms in this regime. In this article, a broad overview of the recent progress is given, ranging from analytical estimates of ground‐state properties to proper derivations of master equations and computation of photodetection signals. For each aspect of the theory, the basic principles of the methods are illustrated on paradigmatic models such as quantum Rabi and spin‐boson models. The validity of effective Hamiltonians for the different experimental platforms is discussed in the last part of the article, addressing recent debates on fundamental issues related to gauge invariance in the ultrastrong‐coupling regime.
Abstract Light-matter interactions are an established field that is experiencing a renaissance in recent years due to the introduction of exotic coupling regimes. These include the ultrastrong and deep-strong coupling regimes, where the coupling constant is smaller and of the order of the frequency of the light mode, or larger than this frequency, respectively. In the past few years, quantum simulations of light-matter interactions in all possible coupling regimes have been proposed and experimentally realized, in quantum platforms such as trapped ions, superconducting circuits, cold atoms, and quantum photonics. We review this fledgling field, illustrating the benefits and challenges of the quantum simulations of light-matter interactions with quantum technologies.
The prototypical system constituted by a two-level atom interacting with a quantized single-mode electromagnetic field is described by the quantum Rabi model (QRM). The QRM is potentially valid at any light-matter interaction regime, ranging from the weak (where the decay rates exceeds the coupling rate) to the deep strong coupling (where the interaction rate exceeds the bare transition frequencies of the subsystems). However, when reaching the ultrastrong coupling regime, several theoretical issues may prevent the correct description of the observable dynamics of such a system: (i) the standard quantum optics master equation fails to correctly describe the interaction of this system with the reservoirs; (ii) the correct output photon rate is no longer proportional to the intracavity photon number; and (iii) they appear to violate gauge invariance. Here, we study the photon flux emission rate of this system under the incoherent excitation of the two-level atom for any light-matter interaction strength and consider different effective temperatures. The dependence of the emission spectra on the coupling strength is the result of the interplay between energy levels, matrix elements of the observables, and the density of states of the reservoirs. Within this approach, we also study the occurrence of light-matter decoupling in the deep strong-coupling regime and show how all of the obtained results are gauge invariant.