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arXiv:1804.06605 · Physical Review Letters

Time-Stretched Spectroscopy by the Quantum Zeno Effect: The Case of Auger Decay

Emil Viñas Boström, Mathieu Gisselbrecht, Tomas Brage, C.‐O. Almbladh, Anders Mikkelsen, Claudio Verdozzi

Published Dec 7, 2018• 6 citations
arXivHTMLPDF

Abstract

A tenet of time-resolved spectroscopy is "faster laser pulses for shorter timescales". Here, we suggest turning this paradigm around, and slowing down the system dynamics via repeated measurements, to do spectroscopy on longer timescales. This is the principle of the quantum Zeno effect. We exemplify our approach with the Auger process, and find that repeated measurements increase the core-hole lifetime, redistribute the kinetic energy of Auger electrons, and alter entanglement formation. We further provide an explicit experimental protocol for atomic Li, to make our proposal concrete.

DOI
10.1103/physrevlett.121.233201

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A tenet of time-resolved spectroscopy is "faster laser pulses for shorter timescales". Here, we suggest turning this paradigm around, and slowing down the system dynamics via repeated measurements, to do spectroscopy on longer timescales. This is the principle of the quantum Zeno effect. We exemplify our approach with the Auger process, and find that repeated measurements increase the core-hole lifetime, redistribute the kinetic energy of Auger electrons, and alter entanglement formation. We further provide an explicit experimental protocol for atomic Li, to make our proposal concrete.
The quantum Zeno effect (QZE) predicts a slow-down of the time development of a system under rapidly repeated ideal measurements, and experimentally this was tested for an ensemble of atoms using short laser pulses for non-selective state measurements. Here we consider such pulses for selective measurements on a single system. Each probe pulse will cause a burst of fluorescence or no fluorescence. If the probe pulses were strictly ideal measurements, the QZE would predict periods of fluorescence bursts alternating with periods of no fluorescence (light and dark periods) which would become longer and longer with increasing frequency of the measurements. The non-ideal character of the measurements is taken into account by incorporating the laser pulses in the interaction, and this is used to determine the corrections to the ideal case. In the limit, when the time between the laser pulses goes to zero, no freezing occurs but instead we show convergence to the familiar macroscopic light and dark periods of the continuously driven Dehmelt system. An experiment of this type should be feasible for a single atom or ion in a trap
The quantum Zeno effect (QZE) predicts a slow-down of the time development of a system under rapidly repeated ideal measurements, and experimentally this was tested for an ensemble of atoms using short laser pulses for non-selective state measurements. Here we consider such pulses for selective measurements on a single system. Each probe pulse will cause a burst of fluorescence or no fluorescence. If the probe pulses were strictly ideal measurements, the QZE would predict periods of fluorescence bursts alternating with periods of no fluorescence (light and dark periods) which would become longer and longer with increasing frequency of the measurements. The non-ideal character of the measurements is taken into account by incorporating the laser pulses in the interaction, and this is used to determine the corrections to the ideal case. In the limit, when the time, , between the laser pulses goes to zero, no freezing occurs but instead we show convergence to the familiar macroscopic light and dark periods of the continuously driven Dehmelt system. An experiment of this type should be feasible for a single atom or ion in a trap.
Abstract We present a time-dependent computational approach to study Auger electron spectroscopy (AES) beyond the ultra-short core-hole relaxation time approximation and, as a test case, we apply it to the paradigmatic example of a one-dimensional Mott insulator represented by a half-filled Hubbard chain. The Auger spectrum is usually calculated by assuming that, after the creation of a core-hole, the system thermalizes almost instantaneously. This leads to a relatively simple analytical expression that uses the ground-state with a core-hole as a reference state and ignores all the transient dynamics related to the screening of the core-hole. In this picture, the response of the system can be associated to the pair spectral function. On the other hand, in our numerical calculations, the core hole is created by a light pulse, allowing one to study the transient dynamics of the system in terms of the pulse duration and in the non-perturbative regime. Time-dependent density matrix renormalization group calculations reveal that the relaxation process involves the creation of a polarization cloud of doublon excitations that have an effect similar to photo-doping. As a consequence, there is a leak of spectral weight to higher energies into what otherwise would be the Mott gap. For longer pulses, these excited states, mostly comprised of doublons, can dominate the spectrum. By changing the duration of the light-pulse, the entire screening process can be resolved in time.
Repeated measurements can slow down (the quantum Zeno effect) or speed up (the quantum anti-Zeno effect) the temporal evolution of a quantum system. In this paper, a general treatment of the quantum Zeno and anti-Zeno effects is presented which is valid for an arbitrary system-environment model in the weak system-environment coupling regime. It is shown that the effective lifetime of a quantum state that is subjected to repeated projective measurements depends on the overlap of the spectral density of the environment and a generalized 'filter function'. This filter function depends on the system-environment Hamiltonian, the state of the environment, and the measurement being performed. Our general framework is then used to study explicitly the Zeno to anti-Zeno crossover behaviour for the spin-boson model where a single two-level system is coupled to a bosonic environment. It is possible to not only reproduce results for the usual population decay case as well as for the pure dephasing model, but to also study the regime where both decay and dephasing take place. These results are then extended to many two-level systems coupled collectively to the bosonic environment to further illustrate the importance of the correct evaluation of the effective decay rate.
Short pulses of a probe laser have been used in the past to measure whether a two-level atom is in its ground or excited state. The probe pulse couples the ground state to a third, auxiliary, level of the atom. The occurrence or absence of resonance fluorescence were taken to mean that the atom was found in its ground or excited state, respectively. In this paper we investigate to what extent this procedure results in an effective measurement to which the projection postulate can be applied, at least approximately. We discuss in detail the complications arising from an additional time development of the two-level system proper during a probe pulse. We extend our previous results for weak probe pulses to the general case and show that one can model an ideal (projection-postulate) measurement much better with a strong than a weak probe pulse. In an application to the quantum Zeno effect we calculate the slow-down of the atomic time development under n repeated probe pulse measurements and determine the corrections compared to the case of n ideal measurements.