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arXiv:1803.08523 · Science

Imaging the electronic Wigner crystal in one dimension

I. Shapir, A. Hamo, S. Pecker, Cătălin Paşcu Moca, Ö. Legeza, Gergely Zaránd, Shahal Ilani

Published May 30, 2019• 125 citations
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Abstract

The quantum crystal of electrons, predicted more than 80 years ago by Eugene Wigner, remains one of the most elusive states of matter. In this study, we observed the one-dimensional Wigner crystal directly by imaging its charge density in real space. To image, with minimal invasiveness, the many-body electronic density of a carbon nanotube, we used another nanotube as a scanning-charge perturbation. The images we obtained of a few electrons confined in one dimension match the theoretical predictions for strongly interacting crystals. The quantum nature of the crystal emerges in the observed collective tunneling through a potential barrier. These experiments provide the direct evidence for the formation of small Wigner crystals and open the way for studying other fragile interacting states by imaging their many-body density in real space.

DOI
10.1126/science.aat0905

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The quantum crystal of electrons, predicted more than 80 years ago by Eugene Wigner, remains one of the most elusive states of matter. In this study, we observed the one-dimensional Wigner crystal directly by imaging its charge density in real space. To image, with minimal invasiveness, the many-body electronic density of a carbon nanotube, we used another nanotube as a scanning-charge perturbation. The images we obtained of a few electrons confined in one dimension match the theoretical predictions for strongly interacting crystals. The quantum nature of the crystal emerges in the observed collective tunneling through a potential barrier. These experiments provide the direct evidence for the formation of small Wigner crystals and open the way for studying other fragile interacting states by imaging their many-body density in real space.
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The collective tunneling of a Wigner necklace---a crystal-like state of a small number of strongly interacting electrons confined to a suspended nanotube and subject to a double-well potential---is theoretically analyzed and compared with experiments in Shapir et al. [Science 364, 870 (2019)]. Density matrix renormalization group computations, exact diagonalization, and instanton theory provide a consistent description of this very strongly interacting system, and show good agreement with experiments. Experimentally extracted and theoretically computed tunneling amplitudes exhibit a scaling collapse. Collective quantum fluctuations renormalize the tunneling, and substantially enhance it as the number of electrons increases.
The simplest possible structural transition that an electronic system can undergo is Wigner crystallization. The aim of this short review is to discuss the main aspects of three recent experimets on the one-dimensional Wigner molecule, starting from scratch. To achieve this task, the Luttinger liquid theory of weakly and strongly interacting fermions is briefly addressed, together with the basic properties of carbon nanotubes that are required. Then, the most relevant properties of Wigner molecules are addressed, and finally the experiments are described. The main physical points that are addressed are the suppression of the energy scales related to the spin and isospin sectors of the Hamiltonian, and the peculiar structure that the electron density acquires in the Wigner molecule regime.
The physics of interacting quantum wires has attracted a lot of attention recently. When the density of electrons in the wire is very low, the strong repulsion between electrons leads to the formation of a Wigner crystal. We review the rich spin and orbital properties of the Wigner crystal, in both the one-dimensional and the quasi-one-dimensional regimes. In the one-dimensional Wigner crystal the electron spins form an antiferromagnetic Heisenberg chain with exponentially small exchange coupling. In the presence of leads, the resulting inhomogeneity of the electron density causes a violation of spin-charge separation. As a consequence the spin degrees of freedom affect the conductance of the wire. Upon increasing the electron density, the Wigner crystal starts deviating from the strictly one-dimensional geometry, forming a zigzag structure instead. Spin interactions in this regime are dominated by ring exchanges, and the phase diagram of the resulting zigzag spin chain has a number of unpolarized phases as well as regions of complete and partial spin polarization. Finally we address the orbital properties in the vicinity of the transition from a one-dimensional to a quasi-one-dimensional state. Due to the locking between chains in the zigzag Wigner crystal, only one gapless mode exists. Manifestations of Wigner crystal physics at weak interactions are explored by studying the fate of the additional gapped low-energy mode as a function of interaction strength.
A one-dimensional gas of electrons interacting with long-range Coulomb forces [V(r)\ensuremath{\approxeq}1/r] is investigated. The excitation spectrum consists of separate collective charge and spin modes. For arbitrarily weak Coulomb repulsion density correlations at wave vector 4kF{\mathit{k}}_{\mathit{F}}kF​ decay extremely slowly and are best described as those of a one-dimensional Wigner crystal. Pinning of the Wigner crystal then leads to the nonlinear transport properties characteristic of charge density waves. The results allow a consistent interpretation of the plasmon and spin excitations observed in one-dimensional semiconductor structures, and suggest an interpretation of some of the observed features in terms of ``spinons.''
Moiré systems have emerged as an exciting tunable platform for engineering and probing quantum matter. A large number of exotic states have been observed, stimulating intense efforts in experiment, theory, and simulation. Utilizing a neural-network-based quantum Monte Carlo approach, we discover a new ground state of the two-dimensional electron gas in a honeycomb moire potential at a filling factor of νm=1/4ν_m =1/4νm​=1/4 (one electron every four moiré minima). In this state, two opposite-spin electrons pair to form a singlet-like valence bond state which restores local C6C_6C6​ symmetry in hexagonal molecules each spanning 666 moiré minima. These molecules of pairs then form a molecular Wigner crystal, leaving one quarter of the moiré minima mostly depleted. The formation of such a paired Wigner crystal, absent any confining potential or attractive interaction to facilitate "pre-assembling" the molecule, provides a fascinating case of collective phenomena in strongly interacting quantum many-body systems, and opportunities to engineer exotic properties.