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arXiv:1803.05884 · Optics Letters

Lineshape-asymmetry elimination in weak atomic transitions driven by an intense standing wave field

D. Antypas, Anne M. Fabricant, Dmitry Budker

Published May 2, 2018• 7 citations
arXivHTMLPDF

Abstract

Owing to the ac-Stark effect, the lineshape of a weak optical transition in an atomic beam can become significantly distorted when driven by an intense standing wave field. We use an Yb atomic beam to study the lineshape of the 6s2S10→5d6sD31 transition, which is excited with light circulating in a Fabry–Perot resonator. We demonstrate two methods to avoid the distortion of the transition profile. Of these, one relies on the operation of the resonator in multiple longitudinal modes, and the other in multiple transverse modes.

DOI
10.1364/ol.43.002241

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Owing to the ac-Stark effect, the lineshape of a weak optical transition in an atomic beam can become significantly distorted when driven by an intense standing wave field. We use an Yb atomic beam to study the lineshape of the 6s2S10→5d6sD31 transition, which is excited with light circulating in a Fabry–Perot resonator. We demonstrate two methods to avoid the distortion of the transition profile. Of these, one relies on the operation of the resonator in multiple longitudinal modes, and the other in multiple transverse modes.
We report on an experimental and theoretical study of the dynamic (ac) Stark effect on a forbidden transition. A general framework for parametrizing and describing off-resonant ac-Stark shifts is presented. A model is developed to calculate spectral line shapes resulting from resonant excitation of atoms in an intense standing light wave in the presence of off-resonant ac-Stark shifts. The model is used in the analysis and interpretation of a measurement of the ac-Stark shifts of the static-electric-field-induced $6{s}^{2}\phantom{\rule{0.2em}{0ex}}^{1}S_{0}\ensuremath{\rightarrow}5d6s^{3}D_{1}$ transition at 408nm408\phantom{\rule{0.3em}{0ex}}\mathrm{nm}408nm in atomic Yb. The results are in agreement with estimates of the ac-Stark shift of the transition under the assumption that the shift is dominated by that of the 6s21S06{s}^{2}\phantom{\rule{0.2em}{0ex}}^{1}S_{0}6s21S0​ ground state. A detailed description of the experiment and analysis is presented. A biproduct of this work is an independent determination (from the saturation behavior of the 408-nm transition) of the Stark transition polarizability, which is found to be in agreement with our earlier measurement. This work is part of the ongoing effort aimed at a precision measurement of atomic parity-violation effects in Yb.
The influence of ac Stark shifts on the three-photon ionization of cesium in a moderate-intensity laser beam is investigated. The ionization process involves a two-photon resonance with the 8d8d8d fine-structure levels. The work consists of two related parts. In the first part, atomic parameters, such as the two-photon Rabi rate and the ac Stark shift, are calculated in the nonrelativistic Hartree-Fock approximation. In the second part, the atomic parameters thus obtained are used as coefficients in a system of coupled differential equations representing the time evolution of the density matrix. Ionization line shapes are generated for a transform-limited pulsed laser of moderate intensity with a single-mode transverse structure. As the time history of the intensity profile is varied from square to smooth, the ionization line shape becomes asymmetric due to the time dependence of the ac Stark shift. The effects of varying the spatial intensity distribution of the laser light to include transverse centering and longitudinal focusing are also studied.
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The interaction of a beam of two level atoms with a standing wave laser field has been the subject of extensive investigation in recent times. A standing wave perpendicular to an atomic beam allows the manipulation of the transverse velocity distribution. The interaction of an atomic beam with a strong standing wave laser field has been systematically investigated by both theoretical simulation and experiment in this thesis. We have developed a numerical model based on a continued fraction solution for the light pressure forces to simulate the near perpendicular interaction of an atomic beam with a strong standing wave laser field. The reshaping of the transverse spatial profile of an atomic beam by a perpendicular, near resonant, standing wave laser field is investigated for red detunings using a longitudinal velocity selective detection system. The experimental dependence of the reshaped profile on the longitudinal and transverse atomic velocities agrees well with a continued fraction solution for the light force. In particular, a regime is found where channelling of the atoms near the antinodes of the standing wave produces a central peak in the spatial distribution of the atomic beam in the far field which have also been observed elsewhere.
Atoms moving in an intense, near resonant standing wave (SW) experience a force along the direction of the SW. This force has been investigated by observing its effect on the transverse velocities of atoms in a thermal beam. When the standing wave is tuned above resonance the atomic beam is collimated and has an increased intensity at the center of the beam. Below resonance, the SW anti-collimates the atomic beam, reducing the central intensity. These effects are due to the interaction between the induced atomic dipole and the inhomogeneous field of the SW. Further investigation shows structure in the transverse velocity distribution of the atomic beam. This structure is due to multiphoton (Doppleron) resonances in the force. Calculations reproduce the dipole force and multiphoton resonance effects and are in good agreement with the data.