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arXiv:1803.03194 · Physical review. B./Physical review. B

Universal dielectric response across a continuous metal-insulator transition

Prosenjit Haldar, M. S. Laad, Syed R. Hassan

Published Mar 26, 2019• 8 citations
arXivHTMLPDF

Abstract

A wide range of disordered materials, including disordered correlated systems, show universal dielectric response (UDR), followed by a superlinear power-law increase in their optical responses over exceptionally broad frequency regimes. While extensively used in various contexts over the years, the microscopics underpinning UDR remains controversial. Here, we investigate the optical response of the simplest model of correlated fermions, the Falicov-Kimball model, across the continuous metal-insulator transition (MIT) and analyze the associated quantum criticality in detail using cluster extension of dynamical mean-field theory. Surprisingly, we find that UDR naturally emerges in the quantum critical region associated with the continuous MIT. We tie the emergence of these novel features to a many-body orthogonality catastrophe accompanying the onset of strongly correlated electronic glassy dynamics close to the MIT, providing a microscopic realization of Jonscher's time-honored proposal as well as a rationale for similarities in optical responses between correlated electronic matter and canonical glass formers.

DOI
10.1103/physrevb.99.125147

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The ground-state phase diagrams of the Falicov-Kimball model with local disorder are derived within the dynamical mean-field theory and using the geometrically averaged (``typical'') local density of states. Correlated metal, Mott insulator, and Anderson insulator phases are identified. The metal-insulator transitions are found to be continuous. The interaction and disorder compete with each other stabilizing the metallic phase against the occurring one of the insulators. The Mott and Anderson insulators are found to be continuously connected.

arXiv:cond-mat/0412590•Physical Review B•May 6, 2005•37 citations
A wide range of disordered materials, including disordered correlated systems, show universal dielectric response (UDR), followed by a superlinear power-law increase in their optical responses over exceptionally broad frequency regimes. While extensively used in various contexts over the years, the microscopics underpinning UDR remains controversial. Here, we investigate the optical response of the simplest model of correlated fermions, the Falicov-Kimball model, across the continuous metal-insulator transition (MIT) and analyze the associated quantum criticality in detail using cluster extension of dynamical mean-field theory. Surprisingly, we find that UDR naturally emerges in the quantum critical region associated with the continuous MIT. We tie the emergence of these novel features to a many-body orthogonality catastrophe accompanying the onset of strongly correlated electronic glassy dynamics close to the MIT, providing a microscopic realization of Jonscher's time-honored proposal as well as a rationale for similarities in optical responses between correlated electronic matter and canonical glass formers.
In contrast to the first-order correlation-driven Mott metal-insulator transition, continuous disorder-driven transitions are intrinsically quantum critical. Here, we investigate transport quantum criticality in the Falicov-Kimball model, a representative of the latter class in the strong disorder category. Employing cluster-dynamical mean-field theory, we find clear and anomalous quantum critical scaling behavior manifesting as perfect mirror symmetry of scaling curves on both sides of the MIT. Surprisingly, we find that the beta function $\ensuremath{\beta}(g)$ scales as log(g)log(g)log(g) deep into the bad-metallic phase as well, providing a sound unified basis for these findings. We argue that such strong localization quantum criticality may manifest in real three-dimensional systems where disorder effects are more important than electron-electron interactions.
The Falicov-Kimball model (FKM) is long known to be the simplest model of correlated fermions exhibiting a novel Mott-like quantum critical point (QCP) assocaited with a {\it continuous} MIT in dimensions D≥3D \geq 3D≥3. It is also known to be isomorphic to an {\it annealed} binary-alloy disorder model. Notwithstanding extensive numerical studies for the FKM, analytic insight into the microscopic processes spawning novel Mott-like quantum criticality is scarce. Here, we develop a fully analytic theory for the Mott-like quantum criticality in the FKM on a hierarchical Cayley tree (Bethe lattice) by utilizing a single input from a 2-site cluster-dynamical mean-field theory (CDMFT). We find that density fluctuation modes acquire anomalous dimensions, originating from infra-red power-law singular cluster self-energies. Interestingly, we uncover, at T=0T=0T=0, that this {\it sub-diffusive} metal with glassy dynamics separating a weakly ergodic metal from a non-ergodic insulator shrinks to a single point, namely the Mott-like QCP, at least on the Bethe lattice. We detail the consequences of this anomalous quantum criticality for a range of thermal and dynamical responses in a variety of physical systems that can be effectively modelled by the FKM.
This chapter focuses on studies of the critical behavior of conductivity in two-dimensional electron systems (2DES) with different amounts and types of disorder as well as different ranges of Coulomb interactions, in order to identify possible universality classes of the 2D metal-insulator transition (MIT). It discusses the manifestations of glassiness in both low- and high-disorder samples. The chapter examines the critical region near the 2D MIT in particular on describing conductivity measurements that have demonstrated dynamical scaling, the main signature of the MIT as a quantum phase transition. It also focuses on experiments that probe the nature of the insulating state, as well as charge dynamics across the MIT, in both high- and low-disorder 2DESs. There is substantial evidence that in many materials near the MIT both strong electronic correlations and disorder play an important role, and thus their competition is expected to lead to glassy behavior of electrons, in analogy with other frustrated systems.
Abstract: The metal–insulator transition (MIT) constitutes one of the most profound and persistent problems in condensed matter physics, sitting at the intersection of electronic structure theory, many-body physics, and emergent quantum phenomena. Conventional band theory, which successfully classifies materials as metals or insulators according to the filling of their electronic bands, fails dramatically when confronted with a class of compounds transition metal oxides chief among them that ought to be metallic by band-counting arguments yet are robustly insulating in the laboratory. The resolution of this paradox required abandoning the independent-electron picture entirely and recognizing that strong Coulomb repulsion between electrons can, by itself, drive localization. This insight, formalized by Mott and later distilled into the Hubbard model, established correlation-driven insulation as a phenomenon distinct from band insulation. The present paper offers a theoretical exploration of the MIT problem, tracing its conceptual development from the Mott criterion through the Hubbard Hamiltonian, the Brinkman–Rice scenario of quasiparticle mass divergence, and the watershed development of dynamical mean-field theory (DMFT), which rendered the Mott transition quantitatively tractable for the first time. We argue that the competition between the electronic bandwidth and the on-site interaction encoded in the ratio U/W provides the unifying organizing principle for the field. Building toward the modern frontier, we examine how the Mott transition connects to quantum phase transitions and quantum criticality, where zero-temperature instabilities governed by quantum rather than thermal fluctuations produce non-Fermi-liquid behavior and anomalous scaling. Case studies of vanadium oxides, rare-earth nickelates, and doped cuprates illustrate the diversity and subtlety of real correlated materials. We conclude that the MIT remains a central and unresolved problem whose continued study is increasingly entangled with the development of quantum materials and quantum technologies. Keywords: Metal–Insulator Transition; Mott Insulator; Strongly Correlated Electrons; Hubbard Model; DMFT; Quantum Criticality; Quantum Materials; Condensed Matter Physics
The celebrated Wiedemann-Franz (WF) law is believed to be robust in metals as long as interactions between electrons preserve their fermion-quasiparticle character. We study thermal transport and the fate of the WF law close to a continuous metal-insulator transition (MIT) in the Falicov-Kimball model (FKM) using cluster-dynamical mean-field theory (CDMFT). Surprisingly, as for electrical transport, we find robust and novel quantum critical scaling in thermal transport across the MIT. We unearth the deeper reasons for these novel findings in terms of (i) the specific structure of energy-current correlations for the FKM and (ii) the microscopic electronic processes which facilitate energy transport while simultaneously blocking charge transport close to the MIT. However, within (C)DMFT, we also find that the WF law survives at $T\ensuremath{\longrightarrow}0$ in the incoherent metal right up to the MIT, even in absence of Landau quasiparticles.
The ground-state phase diagrams of the Falicov-Kimball model with local disorder are derived within the dynamical mean-field theory and using the geometrically averaged (``typical'') local density of states. Correlated metal, Mott insulator, and Anderson insulator phases are identified. The metal-insulator transitions are found to be continuous. The interaction and disorder compete with each other stabilizing the metallic phase against the occurring one of the insulators. The Mott and Anderson insulators are found to be continuously connected.