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arXiv:1802.06172 · Physical Review A

Controlling rare-earth ions in a nanophotonic resonator using the ac Stark shift

John G. Bartholomew, Tian Zhong, Jonathan M. Kindem, Raymond Lopez‐Rios, Jake Rochman, Ioana Craiciu, Evan Miyazono, Andrei Faraon

Published Jun 28, 2018• 11 citations
arXivHTMLPDF

Abstract

Rare-earth ions in crystals are one of the most promising platforms for building quantum technologies, such as quantum memories. Now, through the miniaturization of such systems in an on-chip nanophotonic resonator, the ac Stark shift due to a single photon can be used as a versatile way to control the ions.
DOI
10.1103/physreva.97.063854

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•Jun 1, 2020•1 citation
I present quantum nano-photonic devices based on nanophotonic resonators coupled to rare-earth-ions in crystals. The rare-earth ions exhibit long coherence times on optical transitions, which makes them suitable for optical quantum memories. We demonstrate a high-fidelity nanophotonic quantum memory based on a mesoscopic rare-earth ensemble coupled to a photonic crystal cavity. The nanocavity enables >95% spin polarization for efficient initialization of the atomic frequency comb memory, and time-bin-selective readout via enhanced optical Stark shift of the comb frequencies. Besides ensemble memories, single rare-earth-ions coupled to nano-resonators can be used as single optically addressable quantum bits where the quantum state is mapped on their Zeeman or hyperfine levels with long coherence time. Our solid-state nano-photonic quantum light-matter interfaces can be integrated with other chip-scale photon source and detector devices for multiplexed quantum and classical information processing at the nodes of quantum networks.
Quantum interconnects allow disparate quantum systems to be entangled, leading to more powerful integrated quantum technology and increases in scalability. The foundation for such technology, including photonic quantum memories and coherent microwave-to-optical (M2O) transducers, have already been developed in rare-earth ion (REI) crystals. Here we demonstrate improved REI quantum device functionality in an on-chip platform that dramatically strengthens the ions’ interactions with optical fields and integrates with planar microwave technology. Using a photonic crystal nanobeam fabricated in a Nd-doped yttrium vanadate (YVO) crystal, we harness the enhanced ion-photon interactions that create single photon Rabi frequencies as large as 60 MHz. In particular, the large AC Stark shift is used to control an ensemble of approximately 4000 ions for photonic quantum memory applications. We demonstrate AC Stark shift control of the storage time in the atomic frequency comb protocol as well as the possibility of memories based on an all-optical variation of the hybrid photon echo rephasing protocol. The spin state of the REIs can also be addressed directly through the integration of microwave striplines and coplanar waveguide cavities. The achievement of optically detected magnetic resonance in on-chip waveguides and nanophotonic cavities in Nd:YVO will be presented along with the initial progress of achieving coherent M2O conversion using Raman heterodyne spectroscopy. With photonic quantum memories and sources, single ion qubits, and quantum M2O all feasible in the one integrated platform, REI technology is a promising platform for enabling large scale integration of diverse quantum resources.
This thesis presents on-chip quantum storage of telecommunication wavelength light using nanophotonic resonators coupled to erbium ions. Storage of light in an optical quantum memory has applications in quantum information and quantum communication. For example, long distance quantum communication using quantum repeater protocols is enabled by quantum memories. Efficient and broadband quantum memories can be made from resonators coupled to ensembles of atoms. Like other rare earth ions, erbium is appealing for quantum applications due to its long optical and hyperfine coherence times in the solid state at low temperatures. However, erbium is unique among rare earth ions in having an optical transition in the telecommunication C band (1540 nm), making it particularly appealing for quantum communication applications. In this work, we use nano-scale resonators coupled to erbium-167 ions in yttrium orthosilicate crystals (167Er 3+:Y2SiO5). We demonstrate quantum storage in two types of resonators. In a nanobeam photonic crystal resonator milled directly in 167Er 3+:Y2SiO5, we show storage of weak coherent states using the atomic frequency comb protocol. The storage fidelity for single photon states is estimated to be at least 93.7% ± 2.4% using decoy state analysis, Storage of up to 10 μs and multimode storage are demonstrated. Using a hybrid amorphous silicon 167Er 3+:Y2SiO5 resonator and on-chip electrodes, we demonstrate a multifunctional memory using the atomic frequency comb protocol with DC Stark shift control. In addition dynamic control of memory time, Stark shift control allows modifications to the frequency and bandwidth of stored light. We show tuning of the output pulse by ± 20 MHz relative to the input pulse, and broadening of the pulse bandwidth by more than a factor of three. The storage efficiency in both devices was limited to < 1%. On the way to these results, we describe 167Er 3+:Y2SiO5 spectroscopy measurements including optical coherence times and hyperfine lifetimes below 1 K, and we estimate the linear DC stark shift along two crystal directions. The design and fabrication of the on-chip resonators is presented. We discuss the limitations to storage time and efficiency, including superhyperfine coupling and resonator parameters, and we outline a path forward for improving the storage efficiency in these types of devices.