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arXiv:1802.05280 · Physical review. B./Physical review. B

Spin-lattice coupling in U(1) quantum spin liquids

Sangjin Lee, Eun-Gook Moon

Published Jan 10, 2019• 4 citations
arXivHTMLPDF

Abstract

Quantum spin liquids (QSLs) are exotic phases with intrinsic massive entanglements. Instead of microscopic spins, fractionalized particles and gauge fluctuations are emergent, revealing QSLs' exotic natures. Quantum spins with strong spin-orbit coupling on a pyrochlore lattice, for example ${\mathrm{Pr}}_{2}{\mathrm{Zr}}_{2}{\mathrm{O}}_{7}$, are suggested to host a U(1) QSL with emergent photons, gapless excitations, as well as emergent monopoles. One of the key issues in QSLs is an interplay between emergent degrees of freedom of QSLs and conventional degrees of freedom, and we investigate the interplay by constructing a general theory of spin-lattice coupling in U(1) QSLs. We find that the coupling induces characteristic interplay between phonons and photons. For example, photons become qualitatively more stable than phonons at low temperature. We also propose mechanisms to detect emergent photons in experiments such as sound attenuation and thermal transport relying on spin-lattice coupling in U(1) QSLs.

DOI
10.1103/physrevb.99.014412

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Quantum spin liquids (QSLs) are exotic phases with intrinsic massive entanglements. Instead of microscopic spins, fractionalized particles and gauge fluctuations are emergent, revealing QSLs' exotic natures. Quantum spins with strong spin-orbit coupling on a pyrochlore lattice, for example Pr2Zr2O7{\mathrm{Pr}}_{2}{\mathrm{Zr}}_{2}{\mathrm{O}}_{7}Pr2​Zr2​O7​, are suggested to host a U(1) QSL with emergent photons, gapless excitations, as well as emergent monopoles. One of the key issues in QSLs is an interplay between emergent degrees of freedom of QSLs and conventional degrees of freedom, and we investigate the interplay by constructing a general theory of spin-lattice coupling in U(1) QSLs. We find that the coupling induces characteristic interplay between phonons and photons. For example, photons become qualitatively more stable than phonons at low temperature. We also propose mechanisms to detect emergent photons in experiments such as sound attenuation and thermal transport relying on spin-lattice coupling in U(1) QSLs.
Quantum spin liquids (QSLs) have generated considerable excitement as phases of matter with emergent gauge structures and fractionalized excitations. In this context, phase transitions out of QSLs have been widely discussed as Higgs transitions from deconfined to confined phases of a lattice gauge theory. However, the possibility of a wider range of novel phases, occurring between these two limits, has yet to be systematically explored. In this Research Letter, we develop a formalism which allows for interactions between fractionalized quasiparticles coming from the constraint on the physical Hilbert space and can be used to search for exotic, hidden phases. Taking pyrochlore spin ice as a starting point, we show how a U(1) QSL can give birth to abundant daughter phases, without the need for fine-tuning of parameters. These include a (charged) Z2{\mathbb{Z}}_{2}Z2​ QSL and a supersolid. We discuss implications for experiment, and numerical results which support our analysis. These results are of broad relevance to QSLs subject to a parton description and offer a useful perspective in the search for exotic hidden phases in quantum magnets.
A quantum spin liquid (QSL) is an exotic insulating phase with emergent gauge fields and fractionalized excitations. However, the unambiguous demonstration of the existence of a QSL in a “nonengineered” microscopic model (or in any material) remains challenging. Here, using numerically exact sign-problem-free quantum Monte Carlo simulations, we show that a QSL arises in a nonengineered electron–phonon model. Specifically, we investigate the ground-state phase diagram of the bond Su–Schrieffer–Heeger model on a 2D triangular lattice at (one electron per site), which we show includes a QSL phase which is fully gapped, exhibits no symmetry-breaking order, and supports deconfined fractionalized holon excitations. This suggests promising routes for finding QSLs in realistic materials and high- T c superconductivity by lightly doping them.
Quantum spin liquids (QSLs) are exotic phases of matter exhibiting long-range entanglement and supporting emergent gauge fields. A vigorous search for experimental realizations of these states has identified several materials with properties hinting at QSL physics. A key issue in understanding these QSL candidates is often the interplay of weak disorder of the crystal structure with the spin liquid state. It has recently been pointed out that in at least one important class of candidate QSLs-pyrochlore magnets based on non-Kramers ions such as Pr^{3+} or Tb^{3+}-structural disorder can actually promote a U(1) QSL ground state. Here we set this proposal on a quantitative footing by analyzing the stability of the QSL state in the minimal model for these systems: a random transverse field Ising model. We consider two kinds of instability, which are relevant in different limits of the phase diagram: condensation of spinons and confinement of the U(1) gauge fields. Having obtained stability bounds on the QSL state, we apply our results directly to the disordered candidate QSL Pr_{2}Zr_{2}O_{7}. We find that the available data for currently studied samples of Pr_{2}Zr_{2}O_{7} are most consistent with it a ground state outside the spin liquid regime, in a paramagnetic phase with quadrupole moments near saturation due to the influence of structural disorder.
An emergent SU(4) symmetry discovered in the microscopic model for d1 honeycomb materials [M. G. Yamada, M. Oshikawa, and G. Jackeli, ] has enabled us to tailor exotic SU(4) models in real materials. In the honeycomb structure, the emergent SU(4) Heisenberg model would potentially have a quantum spin-orbital liquid ground state due to the , and we can also expect similar spin-orbital liquids in three-dimensional versions of the honeycomb lattice. In such quantum spin-orbital liquids, both the spin and orbital degrees of freedom become fractionalized and entangled together due to the strong frustrated interactions between them. Similarly to spinons in pure quantum spin liquids, quantum spin-orbital liquids can host not only spinon excitations, but also fermionic excitations at low temperature.
Dynamics and stability of U(1) spin liquids beyond mean-field theory: Triangular-lattice J1J_1J1​-J2J_2J2​ Heisenberg model
Quantum spin liquids (QSLs) are long-range entangled phases of frustrated magnets exhibiting fractionalised spin excitations. In two dimensions, there is limited analytical understanding of their excitation spectra beyond parton mean-field theories, which fail to capture many features of the finite frequency dynamical response. We use a self-consistent mean-field theory combined with the random phase approximation (RPA) for the J1J_1J1​-J2J_2J2​ Heisenberg model on the triangular lattice to describe the strong spinon-spinon interactions of the U(1) Dirac QSL. We obtain quantitative results for the dynamical spin structure factor and phase diagram compatible with comprehensive numerical efforts. We show the continuum response at the Brillouin zone corners is described by a spinon-exciton hybridised with monopole gauge excitations. We further show that the transition from the QSL to 120-degree coplanar order is in the QED3_33​ O(3)-GN universality class. We extend the method to chiral QSLs and XXZ anisotropy, and discuss its broad range of applicability to other models and for describing inelastic neutron scattering experiments in KYbSe2_22​.
Gapless fracton quantum spin liquids are exotic phases of matter described by higher-rank U(1) gauge theories, which host gapped and immobile fracton matter excitations as well as gapless photons. Despite well-known field theories, no spin models beyond purely classical systems have been identified to realize these phases. Using error-controlled Green function Monte Carlo, here we investigate a square lattice spin-1 model that shows precise signatures of a fracton quantum spin liquid without indications of conventional ordering. Specifically, the magnetic response exhibits characteristic patterns of suppressed pinch points that accurately match the prediction of a rank-2 U(1) field theory and reveals the existence of emergent photon excitations in 2+1 spacetime dimensions. Remarkably, this type of fracton quantum spin liquid is not only identified in the system's ground state but also in generic low-energy sectors of a strongly fragmented Hilbert space.