An atom interferometer is a ubiquitous tool for measuring fundamental constants and inertial sensing. While it has been extremely useful in measuring inertial rotations, the fine-structure constant, gravity gradients, and local gravity, the measurement process lacks the ability to probe continuously due to its single-shot nature. In this work, we experimentally demonstrate the diffraction of an atom laser in the Raman-Nath regime, a key step towards the development of an atom-laser-based interferometer. The diffraction orders can be precisely controlled, and momenta up to $\ifmmode\pm\else\textpm\fi{}18\ensuremath{\hbar}k$ can be imparted to the atom laser. We form the ``atom laser'' by outcoupling a quasicontinuous beam of coherent atoms from a reservoir of $^{87}\mathrm{Rb}$ Bose-Einstein condensate lasting up to 400 ms. This atom laser then interacts with a grating formed by a standing wave of far-detuned laser light. By controlling the interaction time, the strength of diffraction into various orders can be controlled. Such diffraction would allow for the construction of an atom-interferometer to probe changes in physical environments continuously up to a few hundred milliseconds.
An atom interferometer is a ubiquitous tool for measuring fundamental constants and inertial sensing. While it has been extremely useful in measuring inertial rotations, the fine-structure constant, gravity gradients, and local gravity, the measurement process lacks the ability to probe continuously due to its single-shot nature. In this work, we experimentally demonstrate the diffraction of an atom laser in the Raman-Nath regime, a key step towards the development of an atom-laser-based interferometer. The diffraction orders can be precisely controlled, and momenta up to \ifmmode±\else\textpm\fi18\ensuremathℏk can be imparted to the atom laser. We form the ``atom laser'' by outcoupling a quasicontinuous beam of coherent atoms from a reservoir of 87Rb Bose-Einstein condensate lasting up to 400 ms. This atom laser then interacts with a grating formed by a standing wave of far-detuned laser light. By controlling the interaction time, the strength of diffraction into various orders can be controlled. Such diffraction would allow for the construction of an atom-interferometer to probe changes in physical environments continuously up to a few hundred milliseconds.
We report the experimental realization of a multibeam atom laser. A single continuous atom laser is outcoupled from a Bose-Einstein condensate via an optical Raman transition. The atom laser is subsequently split into up to five atomic beams with slightly different momenta, resulting in multiple, nearly copropagating, coherent beams which could be of use in interferometric experiments. The splitting process itself is a realization of Bragg diffraction, driven by each of the optical Raman laser beams independently. This presents a significantly simpler implementation of an atomic beam splitter, one of the main elements of coherent atom optics.
This cumulative thesis consists of four publications [1-4], presented as three contributions (I) - (III), where the second one (II) consists of the joint publications [2,3]. All publications were written during the author's research activities at the Institute of Quantum Physics under the supervision of Prof. Dr. W. P. Schleich. All of the presented publications consider light-matter interactions and their potential application in atom interferometry, a comparatively young and rapidly evolving technique. Atom interferometers find application in high-precision measurements, the determination of physical constants, the testing of fundamental physics, and the provision of gravimeters and gyroscopes. The advancement of technology and science has led to significant improvements in performance and the development of ambitious mobile and space-based devices. The recent success of several experiments has led to the proposal of further experiments with the aim of opening up new frontiers. However, the construction of future devices necessitates a decision regarding the employed diffraction mechanism and geometry, depending on the specific technical and scientific requirements. Furthermore, it is necessary to enhance the sensitivity of future devices. The contributions in this dissertation address these issues. The first contribution (I) focuses on the diffraction of atoms by laser pulses which can be employed to generate atom-optical diffraction elements like beam splitters and mirrors. These diffraction elements can be combined to construct atom interferometers, which have been successfully employed for precision measurements regarding fundamental physics as well as practical applications. The article presents a numerical comparison of two distinct diffraction mechanisms (Bragg and Raman) and diffraction geometries (single and double diffraction) in microgravity. It discusses the fundamental differences between the mechanisms and geometries with respect to the diffraction efficiency, taking into account the width of the initial wave function and the duration of the light pulse. Additionally, it explores the transition between the two diffraction geometries when starting from an atom initially at rest and increasing its momentum. The results may serve as a reference for experimentalists in selecting the most suitable configuration, based on their aims and requirements in the realization of more advanced atom interferometers. The second contribution (II) is a follow-up to the previous one, but focuses exclusively on a single diffraction type in microgravity, namely the so-called double Raman diffraction. In contrast to the previous article, where we only discussed single two-photon processes, we consider in this article a six-photon process, also known as third-order diffraction, as well as three subsequent two-photon processes, which both lead to the same amount of transferred momentum and can both be used to realize large-momentum transfer (LMT). We demonstrate that third-order double Raman diffraction is a viable and advantageous method for the diffraction of small momentum distributions like Bose-Einstein condensates (BECs) compared to a sequence of three two-photon processes. Furthermore, we show that third-order Raman pulses can be successfully applied to create higher-order Raman atom interferometers. Third-order diffraction can be perfectly combined with other LMT techniques and, moreover, allows for a reduction in the overall duration of the diffraction process and the complexity of the experimental set-up, as only two distinct laser frequencies are required. Moreover, we present a third-order Mach-Zehnder interferometer with spurious paths being disregarded. As demonstrated later on in [3], this interferometer generates optimal contrast and a substantial amplitude. The third contribution (III) extends the semi-classical λ-scheme of single Raman diffraction, as discussed in detail in contribution (I), into a fully quantized multi-atom multi-λ configuration with center-of-mass motion inside a cavity. Therefore, the incorporation of an internal structure allows for a more realistic modeling of the atoms, which is relevant for multi-photon interaction or cooling processes. We use for our analysis the framework of second quantization, i.e., we take into account the field-theoretical nature of the multi-particle atomic field as well as of the diffracting light field. We reduce this model with a Hamiltonian averaging theory applied to the atomic field operators and obtain an effective Hamiltonian, which determines the time evolution of the system. We demonstrate the efficiency of our model by the application of a typical initial state. Moreover, for a specific input state, we obtain the Hong-Ou-Mandel effect simultaneously in the atomic and the optical system. Our many-body formalism is perfectly suited to theoretically describe contemporary high-precision atom interferometric experiments based on entanglement between the atoms, that aim to surpass the shot-noise limit.
Our ability to manipulate the coherence properties of light has been at the heart of many of the most important scientific and technological innovations of this century. There can hardly be a home in this country that does not possess a laser in the form of a compact disc player or a CDROM. When we talk on the phone, or send messages on the Internet, there is a high probability that our message will be encoded by a laser into pulses of light to be passed through optical fibres. In the last few years physicists have been discovering that it is possible to control the coherence properties of atoms, and are now developing tools analogous to those which have been developed to take advantage of the coherence properties of light. In the next decade we can look forward to seeing the application of lasers, fibres, mirrors and waveguides for atoms. Already we have been able to construct interferometry experiments using beams of atoms and these have proved to be extremely sensitive measurement devices, allowing us to test physical theories and measure fundamental constants to a level of precision not previously possible. Will these developing technologies ever be as ubiquitous as their optical forebears? In this paper we discuss the anticipated uses of this technology for both fundamental science and industrial applications. Starting from an explanation of the meaning of coherence and a comparison of the properties of photons and atoms, we describe the development of the science of atom optics. The tortuous route towards the great achievement of producing a Bose–Einstein condensate is described, and we explain why this is the most important step towards a laser–like source of atoms. Numerous other optical elements for atoms have been built or are on the drawing board, and we describe how these may be used to manipulate atoms with a precision that has never before been achieved, and look ahead to what we can learn about physics using these tools and at how they can be put to practical use.
We investigate the diffraction of a three-level atom from a "walking" light wave composed of counterpropagating traveling waves of different frequencies. The coupling of the two nondegenerate internal ground states by means of an off-resonant Raman transition resonantly couples the initial external momentum state to only one other momentum state. This happens even in the Raman-Nath regime, where the interaction time is short enough that momentum transfer is not constrained by phase-matching conditions. The final momentum state depends on the initial internal state of the atom and the relative directions of the two traveling waves. By using multiple diffraction regions, this process can be used to coherently split a beam of atoms into two beams that are widely separated in momentum space. This type of beam splitter would be useful in the building an atom interferometer.
We have used an echo-type atom interferometer that manipulates laser-cooled atoms in a single ground state to investigate the effect of light scattering from pulsed and continuous-wave light. The interferometer uses two off-resonant standing-wave pulses applied at times t=0 and t=T to diffract and recombine momentum states separated by $2\ensuremath{\hbar}k$ at t=2T. Matter wave interference is associated with the formation of a density grating with period $\ensuremath{\lambda}/2$ in the vicinity of this echo time. The grating contrast is measured by recording the intensity of coherently backscattered light. The interferometer is perturbed by an additional pulse applied at $t=2T\ensuremath{-}\ensuremath{\delta}T$ or by continuous-wave background light. If the additional pulse is a standing wave, the momentum states interfering at t=2T are displaced and the grating contrast can be completely recovered due to constructive interference. In this case, the contrast shows a periodic modulation at the atomic recoil frequency as a function of $\ensuremath{\delta}T$. In a recent work, it was shown that the atomic recoil frequency can be measured easily and precisely when using coherence functions to model the signal shape. This paper provides an alternative description of the signal shape through an analytical calculation of echo formation in the presence of an additional standing-wave pulse. Using this treatment, it is possible to model the effects of spontaneous emission and spatial profile of the laser beam on the signal shape. Additionally, the theory predicts scaling laws as a function of the pulse area and the number of additional standing-wave pulses. These scaling laws are investigated experimentally and can be exploited to improve precision measurements of the atomic recoil frequency. We also show that coherence functions can be used to make a direct measurement of the populations of momentum states associated with the ground state under conditions where the Doppler-broadened velocity distribution of the sample is much larger than the recoil velocity. These measurements are consistent with Monte Carlo wave-function simulations. If the additional pulse is a traveling wave, we find that the grating contrast measured as a function of $\ensuremath{\delta}T$ can be modeled by a quasiperiodic coherence function as in previous experiments that utilized atomic beams. In this work, we investigate the dependence of the photon scattering rate on the intensity and detuning of the traveling wave. We also study the effects of perturbing the interferometer with continuous-wave light and find that the dependence of the photon scattering rate on the intensity and detuning of the perturbing field is consistent with expectations.
We study the transient dynamics that arise during the formation of an atom laser beam in a tight waveguide. The time dependent density profile develops a series of wiggles which are related to the diffraction in time phenomenon. The apodization of matter waves, which relies on the use of smooth aperture functions, allows to suppress such oscillations in a time interval, after which there is a revival of the diffraction in time. The revival time scale is directly related to the inverse of the harmonic trap frequency for the atom reservoir. PACS numbers: Atom lasers have recently been created in the laboratory and stand up for their applications in atom lithography and interferometry. Similar to their light analogues, they consist in coherent and directed (matter-) wave beams, which are extracted from a Bose-Einstein condensate (BEC). Different schemes have been proposed to out-couple the atoms from the BEC reservoir. One of the prototypes uses two-photon Raman excitation to create “output coupled ” atomic pulses with well defined mean momentum which overlap and form a quasi-continuous beam [1, 2] (For other approaches see e.g. [3] or [4]). The features of the beam profile are of outmost importance for applications [5, 6, 7], and depend on the pulse shape, duration, emission frequency, and initial phase [8]. We study the dynamics of a beam created by multiple overlapping pulses, transversely confined in a tight waveguide and with negligible interactions between the out-coupled atoms. It is found that an oscillatory pattern appears in the density profile of the beam which is closely related to the diffraction in time phenomenon. If the switching process is slow, such oscillations are suppressed on a time window after which there is a revival of the diffraction in time. The time scale in which the spatial fringes appear is related to the the spatial width of the out-coupled pulses.