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arXiv:1802.00942 · Physical Review A

Angle-dependent magic wavelengths for the 4s1/2→3d5/2,3/2 transitions of Ca+ ions

Jun Jiang, Li Jiang, Zhongwen Wu, Denghong Zhang, Lu-You Xie, Chenzhong Dong

Published Mar 22, 2019• 9 citations
arXivHTMLPDF

Abstract

The dynamic polarizabilities of the atomic states with angular momentum $j>1/2$ are sensitive to the angle between the quantization axis ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{e}}_{z}$ and the polarization vector $\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\ensuremath{\epsilon}}$ owing to the contribution of anisotropic tensor polarizabilities. The magic wavelength at which the differential Stark shift of an atomic transition nullifies depends on this angle. We identified the magic wavelengths for the $4{s}_{1/2}\ensuremath{\rightarrow}3{d}_{3/2,5/2}$ transitions of ${\mathrm{Ca}}^{+}$ ions at different angles between ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{e}}_{z}$ and $\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\ensuremath{\epsilon}}$ in the case of linearly polarized light. The magic wavelengths near 395.79 nm, which lie between the $4{s}_{1/2}\ensuremath{\rightarrow}4{p}_{1/2}$ and $4{s}_{1/2}\ensuremath{\rightarrow}4{p}_{3/2}$ transition wavelengths, remain insensitive to the angle, while the longest magic wavelength, which is around 1000 nm, for each of the magnetic sublevel transitions is very sensitive to the angle. We suggest that accurate measurements on the longest magic wavelengths for the $4{s}_{1/2}\ensuremath{\rightarrow}3{d}_{5/2}$ and $4{s}_{1/2}\ensuremath{\rightarrow}3{d}_{3/2}$ transitions can be used to determine the oscillator strengths for the $4{s}_{1/2}\ensuremath{\rightarrow}4{p}_{1/2,3/2}, 3{d}_{5/2}\ensuremath{\rightarrow}4{p}_{3/2}$, and $3{d}_{3/2}\ensuremath{\rightarrow}4{p}_{1/2,3/2}$ transitions, and the difference of the static polarizabilities of the $4{s}_{1/2}$ and $3{d}_{5/2}$ states, and the tensor polarizability of the $3{d}_{5/2}$ state.

DOI
10.1103/physreva.99.032510

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Measurement of infrared magic wavelength for an all-optical trapping of 40^{40}40Ca+^{+}+ ion clock
For the first time, we experimentally determine the infrared magic wavelength for the 40^{40}40Ca+^{+}+ 4s 2 ⁣S1/2→3d 2 ⁣D5/24s\, ^{2}\!S_{1/2} \rightarrow 3d\,^{2}\!D_{5/2}4s2S1/2​→3d2D5/2​ electric quadrupole transition by observation of the light shift canceling in 40^{40}40Ca+^{+}+ optical clock. A "magic" magnetic field direction is chosen to make the magic wavelength insensitive to both the linear polarization purity and the polarization direction of the laser. The determined magic wavelength for this transition is 1056.37(9)~nm, which is not only in good agreement with theoretical predictions but also more precise by a factor of about 300. Using this measured magic wavelength we also derive the differential static polarizability to be −44.32(32)-44.32(32)−44.32(32)~a.u., which will be an important input for the evaluation of the blackbody radiation shift at room temperatures. Our work paves a way for all-optical-trapping of 40^{40}40Ca+^{+}+ optical clock.
The wave functions, energy levels and matrix elements of Yb+ ions are calculated using the relativistic configuration interaction plus core polarization (RCICP) method. The static and dynamic electric dipole polarizabilities of the ground state and low-lying excited states are determined. Then, the magic wavelengths of the magnetic sublevel 6s1/2,m = 1/2 → 5d3/2,m = ±3/2,±1/2 and 6s1/2,m = 1/2 → 5d5/2,m = ±5/2,±3/2,±1/2 transitions in the linearly, right-handed, and left-handed polarized light are further determined. The dependence of the magic wavelengths upon the angle between the direction of magnetic field and the direction of laser polarization is analyzed.
The relativistic configuration interaction plus many-body perturbation (RCI +++ MBPT) method is utilized to calculate the wave functions, energy levels, and reduced E1E1E1 transition matrix elements of Ca atoms in detail. The static and dynamic polarizabilities of the 4s21S0,4s4p1P14{s}^{2}\phantom{\rule{0.16em}{0ex}}^{1}S_{0}, 4s4p\phantom{\rule{0.16em}{0ex}}^{1}P_{1}4s21S0​,4s4p1P1​, and 4s4p3P0,1,24s4p\phantom{\rule{0.16em}{0ex}}^{3}P_{0,1,2}4s4p3P0,1,2​ states are determined by the sum-over-states method. A number of magic-zero wavelengths for the ground and 4s4p3P04s4p\phantom{\rule{0.16em}{0ex}}^{3}P_{0}4s4p3P0​ states, as well as magic wavelengths for the $4{s}^{2}\phantom{\rule{0.16em}{0ex}}^{1}S_{0}\ensuremath{\rightarrow}4s4p\phantom{\rule{0.16em}{0ex}}^{3}P_{0}$ and $4{s}^{2}\phantom{\rule{0.16em}{0ex}}^{1}S_{0}\ensuremath{\rightarrow}4s4p\phantom{\rule{0.16em}{0ex}}^{3}P_{1}$ transitions, are obtained. We suggest that the measurements of the magic-zero wavelengths of the 4s4p3P04s4p\phantom{\rule{0.16em}{0ex}}^{3}P_{0}4s4p3P0​ states can be used to determine oscillator strengths with high precision. In addition, the angle-dependent magic wavelengths of each magnetic sublevel transition of the $4{s}^{2}\phantom{\rule{0.16em}{0ex}}^{1}S_{0}\ensuremath{\rightarrow}4s4p\phantom{\rule{0.16em}{0ex}}^{3}P_{1}$ transition are provided, which are of particular interest for optical frequency measurements, Bose-Einstein condensate generation, and superradiant laser technology.
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We demonstrate experimentally the existence of magic wavelengths and determine the ratio of oscillator strengths for a single trapped ion. For the first time, two magic wavelengths near 396 nm for the ^{40}Ca^{+} clock transition are measured simultaneously with high precision. By tuning the applied laser to an intermediate wavelength between transitions 4s_{1/2}→4p_{1/2} and 4s_{1/2}→4p_{3/2}, the sensitivity of the clock transition Stark shift to the oscillator strengths is greatly enhanced. Furthermore, with the measured magic wavelengths, we determine the ratio of the oscillator strengths with a deviation of less than 0.5%. Our experimental method may be applied to measure magic wavelengths for other ion clock transitions. Promisingly, the measurement of these magic wavelengths paves the way to building all-optical trapped ion clocks.