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arXiv:1802.00126 · Physical Review Letters

Observation of Discrete-Time-Crystal Signatures in an Ordered Dipolar Many-Body System

Jared Rovny, Robert L. Blum, Sean Barrett

Published May 1, 2018• 287 citations
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Abstract

A discrete time crystal (DTC) is a robust phase of driven systems that breaks the discrete time translation symmetry of the driving Hamiltonian. Recent experiments have observed DTC signatures in two distinct systems. Here we show nuclear magnetic resonance observations of DTC signatures in a third, strikingly different system: an ordered spatial crystal. We use a novel DTC echo experiment to probe the coherence of the driven system. Finally, we show that interactions during the pulse of the DTC sequence contribute to the decay of the signal, complicating attempts to measure the intrinsic lifetime of the DTC.

DOI
10.1103/physrevlett.120.180603

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A discrete time crystal (DTC) is a robust phase of driven systems that breaks the discrete time translation symmetry of the driving Hamiltonian. Recent experiments have observed DTC signatures in two distinct systems. Here we show nuclear magnetic resonance observations of DTC signatures in a third, strikingly different system: an ordered spatial crystal. We use a novel DTC echo experiment to probe the coherence of the driven system. Finally, we show that interactions during the pulse of the DTC sequence contribute to the decay of the signal, complicating attempts to measure the intrinsic lifetime of the DTC.
Periodic driving of an interacting spin system may lead to unusual out-of-equilibrium states of matter, such as the discrete time crystal (DTC). Two recent experiments have reported a key signature of the DTC: for long enough interaction times, the system's response becomes rigidly locked to one half of the driving frequency. Using nuclear magnetic resonance, the authors observe this DTC signature in the most unexpected system to date: a three-dimensional, spatially ordered crystal. This challenges the paradigm that the DTC arises from many-body localization. Furthermore, hidden coherence in the system is revealed by the ``DTC echo'' experiment, and the effect of interactions during drive pulses is demonstrated.
Periodically driven quantum systems host a range of non-equilibrium phenomena which are unrealizable at equilibrium. Discrete time-translational symmetry in a periodically driven many-body system can be spontaneously broken to form a discrete time crystal, a putative quantum phase of matter. We present the observation of discrete time crystalline order in a driven system of paramagnetic PPP -donor impurities in isotopically enriched 28Si^{28}Si28Si cooled below 101010 K. The observations exhibit a stable subharmonic peak at half the drive frequency which remains pinned even in the presence of pulse error, a signature of DTC order. We propose a theoretical model based on the paradigmatic central spin model which is in good agreement with experimental observations, and investigate the role of dissipation in the stabilisation of the DTC. Both experiment and theory indicate that the order in this system is primarily a dissipative effect, and which persists in the presence of spin-spin interactions. We present a theoretical phase diagram as a function of interactions and dissipation for the central spin model which is consistent with the experiments. This opens up questions about the interplay of coherent interaction and dissipation for time-translation symmetry breaking in many-body Floquet systems.
We analyze the quantum dynamics of periodically driven, disordered systems in the presence of long-range interactions. Focusing on the stability of discrete time crystalline (DTC) order in such systems, we use a perturbative procedure to evaluate its lifetime. For 3D systems with dipolar interactions, we show that the corresponding decay is parametrically slow, implying that robust, long-lived DTC order can be obtained. We further predict a sharp crossover from the stable DTC regime into a regime where DTC order is lost, reminiscent of a phase transition. These results are in good agreement with the recent experiments utilizing a dense, dipolar spin ensemble in diamond [Nature (London) 543, 221 (2017)NATUAS0028-083610.1038/nature21426]. They demonstrate the existence of a novel, critical DTC regime that is stabilized not by many-body localization but rather by slow, critical dynamics. Our analysis shows that the DTC response can be used as a sensitive probe of nonequilibrium quantum matter.
Many-body quantum systems, under suitable conditions, exhibit time-translation symmetry breaking and settle in a discrete time crystalline (DTC) phase -- an out-of-equilibrium quantum phase of matter. The defining feature of DTC is a robust subharmonic response. However, the DTC phase is fragile in the presence of environmental dissipation. Here, we propose and exemplify a DTC phase in a noninteracting system that owes its stability to environmental dissipation. The lifetime of this DTC is independent of initial conditions and the size of the system, though it depends on the frequency of the external driver. We experimentally demonstrate this realization of DTC using Nuclear Magnetic Resonance spectroscopy.
Here we provide a theoretical framework to analyze discrete time-crystalline (DTC) phases in the dissipative dipolar systems subjected to a two-pulse excitation scheme. As a particular realization, we choose a quantum many-body system that exhibits prethermalization due to the presence of the quasiconserved quantities. The analysis uses a fluctuation-regulated quantum master equation, which captures the dissipative effects of the drive and dipolar coupling on the dynamics regularized by the thermal fluctuations. We find that the effects of such dissipation lend stability to the dynamics and are directly responsible for the robustness. Specifically, we find that longer fluctuation correlation time enhances the stability of DTC. We also obtain the lifetime of such a robust period-doubling response, a salient feature of the DTC phase, by varying several system parameters. Our results are in good agreement with the recent experimental findings in dipolar systems using nuclear magnetic resonance spectroscopy. Finally, we provide an estimate how the DTC performance degrades with temperature.
The discrete time crystal (DTC) is a nonequilibrium phase of matter that spontaneously breaks time-translation symmetry. Disorder-induced many-body localization can stabilize the DTC phase by breaking ergodicity and preventing thermalization. Here, we observe the hallmark signatures of the many-body–localized DTC using a quantum simulation platform based on individually controllable carbon-13 nuclear spins in diamond. We demonstrate long-lived period-doubled oscillations and confirm that they are robust for generic initial states, thus showing the characteristic time-crystalline order across the many-body spectrum. Our results are consistent with the realization of an out-of-equilibrium Floquet phase of matter and introduce a programmable quantum simulator based on solid-state spins for exploring many-body physics.