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arXiv:1801.00482

Optical Control of Exchange Interaction and Kondo Temperature in cold Atom Gas

Igor Kuzmenko, Tanya Kuzmenko, Y. Avishai

Published Jan 1, 2018• 3 citations
arXivHTMLPDF

Abstract

The relevance of magnetic impurity problems in cold atom systems depends crucially on the nature of exchange interaction between itinerant fermionic atoms and a localized impurity atom. In particular, Kondo physics occurs only if the exchange interaction is anti-ferromagnetic, and strong enough to yield high enough Kondo temperature ($T_K/T_F \ge 0.1$). Focusing, as an example, on the experimentally accessible system of ultra-cold $^{173}$Yb atoms, it is shown that the sign and strength of an exchange interaction between an itinerant Yb($^{1}$S$_{0}$) atom and a trapped Yb($^{3}$P$_{0}$) atom can be optically controlled. Explicitly, as the light intensity increases (from zero), the exchange interaction changes from ferromagnetic to anti-ferromagnetic. When the light intensity is just below a singlet Feshbach resonance, the singlet scattering length $a_S$ is large and negative, and the Kondo temperature increases sharply.

DOI
10.48550/arxiv.1801.00482

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The relevance of magnetic impurity problems in cold atom systems depends crucially on the nature of exchange interaction between itinerant fermionic atoms and a localized impurity atom. In particular, Kondo physics occurs only if the exchange interaction is anti-ferromagnetic, and strong enough to yield high enough Kondo temperature (TK/TF≥0.1T_K/T_F \ge 0.1TK​/TF​≥0.1). Focusing, as an example, on the experimentally accessible system of ultra-cold 173^{173}173Yb atoms, it is shown that the sign and strength of an exchange interaction between an itinerant Yb(1^{1}1S0_{0}0​) atom and a trapped Yb(3^{3}3P0_{0}0​) atom can be optically controlled. Explicitly, as the light intensity increases (from zero), the exchange interaction changes from ferromagnetic to anti-ferromagnetic. When the light intensity is just below a singlet Feshbach resonance, the singlet scattering length aSa_SaS​ is large and negative, and the Kondo temperature increases sharply.
Whereas in the familiar Kondo effect the exchange interaction is dipolar, there are systems in which the exchange interaction is multipolar, as has been realized in a recent experiment. Here, we study multipolar Kondo effect in a Fermi gas of cold 173Yb^{173}\mathrm{Yb}173Yb atoms. Making use of different ac polarizabilities of the electronic ground state Yb(1S0)\mathrm{Yb}(^{1}\mathrm{S}_{0})Yb(1S0​) and the long-lived metastable state Yb∗(3P2){\mathrm{Yb}}^{*}(^{3}\mathrm{P}_{2})Yb∗(3P2​), it is suggested that the latter atoms can be localized and serve as a dilute concentration of magnetic impurities while the former ones remain itinerant. The exchange mechanism between the itinerant Yb and the localized Yb∗{\mathrm{Yb}}^{*}Yb∗ atoms is analyzed and shown to be antiferromagnetic. The quadrupole and octupole interactions act to enhance the Kondo temperature TK{T}_{K}TK​ that is found to be experimentally accessible. The bare exchange Hamiltonian needs to be decomposed into dipole (d)(\text{d})(d), quadrupole (q)(\text{q})(q), and octupole (o)(\text{o})(o) interactions in order to retain its form under renormalization group (RG) analysis, in which the corresponding exchange constants $({\ensuremath{\lambda}}_{\text{d}},{\ensuremath{\lambda}}_{\text{q}}$, and ${\ensuremath{\lambda}}_{\text{o}})$ flow independently. Numerical solution of the RG scaling equations reveals a few finite fixed points. Arguments are presented that the Fermi-liquid fixed point at low temperature is unstable, indicating that the impurity is overscreened, which suggests a non-Fermi-liquid phase. The impurity contributions to the specific heat, entropy, and the magnetic susceptibility are calculated in the weak coupling regime $(T\ensuremath{\gg}{T}_{K})$, and are compared with the analogous results obtained for the standard case of dipolar exchange interaction (the $s\ensuremath{-}d$ Hamiltonian).
We propose an experimental protocol to directly observe the Kondo effect by scattering ultracold atoms. We propose using an optical Feshbach resonance to engineer Kondo-type spin-dependent interactions in a system with ultracold 6Li^{6}\mathrm{Li}6Li and 87Rb^{87}\mathrm{Rb}87Rb gases. We calculate the momentum transferred from the 87Rb^{87}\mathrm{Rb}87Rb gas to the 6Li^{6}\mathrm{Li}6Li gas in a scattering experiment and show that it has a logarithmically enhanced temperature dependence, characteristic of the Kondo effect, and analogous to the resistivity of alloys with magnetic impurities. Experimentally detecting this enhancement will give a different perspective on the Kondo effect, and allow us to explore a rich variety of problems such as the Kondo lattice problem and heavy-fermion systems.
We propose a simple but novel scheme to realize the Kondo effect with ultracold atoms. Our system consists of a Fermi sea of spinless fermions interacting with an impurity atom of different species which is confined by an isotropic potential. The interspecies attraction can be tuned with an s-wave Feshbach resonance so that the impurity atom and a spinless fermion form a bound dimer that occupies a threefold-degenerate p orbital of the confinement potential. Many-body scatterings of this dimer and surrounding spinless fermions occur with exchanging their angular momenta and thus exhibit the SU(3) orbital Kondo effect. The associated Kondo temperature has a universal leading exponent given by TK∝exp[-π/(3apkF3)] that depends only on an effective p-wave scattering volume ap and a Fermi wave vector kF. We also elucidate a Kondo singlet formation at zero temperature and an anisotropic interdimer interaction mediated by surrounding spinless fermions. The Kondo effect thus realized in ultracold atom experiments may be observed as an increasing atom loss by lowering the temperature or with radio-frequency spectroscopy. Our scheme and its extension to a dense Kondo lattice will be useful to develop new insights into yet unresolved aspects of Kondo physics.
The research described in this thesis is part of an international effort with the aim of studying ultracold quantum degenerate gas samples like Bose-Einstein condensates and Fermi degenerate systems, consisting of atoms confined in magnetic or optical traps. The behavior of such samples is governed by the inter-atomic interactions and the resulting properties of the atom-atom scattering. At the relevant temperatures of 1nK to 10µK a key property is the atom-atom scattering length a. In chapter 2 a theoretical method is presented which enables one to describe the interaction and scattering of (ultra)cold atoms to unprecedented precision. It is also unparalleled in comprehensiveness: it allows the prediction of a large and varied set of experimental data for all isotopes of the same element. The method relies on the extraction from experiments of a few (phase) parameters which completely summarize the behavior of the atoms in the (ultra)cold regime. In chapter 3 the method is applied to the "workhorses" of cold-atom physics: the atomic species 85Rb and 87Rb. We extract the foregoing parameters to a very high precision from several recent high precision experiments, allowing us to predict e.g. the 87Rb spinor condensate to be ferromagnetic: a prediction for which the scattering length has to be calculated with a precision better than 1%. We also predict Feshbach resonances at experimentally accessible magnetic field strengths; resonances searched for and found by the experimental group of Rempe. In close collaboration with his group we "fine-tune" the interaction parameters found previously, by making use of only one of the observed resonances. We then obtain agreement with 42 out of the observed 43 resonance field strengths and are able to identify bound states inducing the Feshbach resonances at these locations. Chapter 4 describes the results of this research. With a thorough understanding of the rubidium interactions, we then switch to lithium which has a fermionic (6Li) and a bosonic (7Li) isotope. Both are being used in cold-atom experiments. In chapter 5 we evaluate the interaction parameters for lithium allowing us to predict magnetic field strengths for which a sample of fermionic 6Li atoms can be regarded as strongly interacting. Furthermore, a three-level method for measuring mean-field shifts, based on radio-frequency techniques, is introduced. For weak interactions we find proportionality of resonance shifts to interaction strengths. In the strongly interacting regime, however, these shifts become very small reflecting the quantum unitarity limit and many-body effects. Most interesting is the fact that in this regime the shifts are small both for large positive a and for large negative a, likely reflecting the universality of the interaction energy. In chapters 6 and 7 the interactions between lithium atoms are reinvestigated, making use of newly available experimental data and with the updated interaction parameters special attention is paid to locating field strengths at which magnetically tunable Feshbach resonances occur in the scattering of lithium atoms. In chapter 6 scattering events in a gas of (fermionic) 6Li atoms are studied. In chapter 7 we show that a consistent description of the 6Li+6Li system can be given. We discuss theoretical uncertainties for the position of the wide 6Li Feshbach resonance and present an analytic scattering model for this resonance, based on the inclusion of a field-dependent virtual open-channel state. We predict new Feshbach resonances for the 6Li-7Li system, and their importance for different types of crossover superfluidity models is discussed. Molecules created by magnetically sweeping over these resonances will have a fermionic character. One magnetic field strength is predicted at which two different fermionic molecules can be created simultaneously.
The feasibility of realizing the overscreened Kondo effect in ultracold Fermi gas of atoms with spin $s\ensuremath{\ge}\frac{3}{2}$ in the presence of a localized magnetic impurity atom is proved realistic. Specifying (as a mere example) a system of ultracold 22Na^{22}\mathrm{Na}22Na Fermi gas and a trapped 6Li^{6}\mathrm{Li}6Li impurity, the mechanism of exchange interaction between the Na and Li atoms is elucidated and the exchange constant is found to be positive (antiferromagnetic). The corresponding exchange Hamiltonian is derived, and the Kondo temperature is estimated at the order of 500 nK. Within a weak-coupling renormalization group scheme, it is shown that the coupling renormalizes to the non-Fermi-liquid fixed point. An observable displaying multichannel features even in the weak-coupling regime is the impurity magnetization that is negative for $T\ensuremath{\gg}{T}_{K}$ and becomes positive with decreasing temperature.
Ultracold gases of fermionic alkaline-earth(-like) atoms are hopeful candidates for the quantum simulation of many-body physics induced by magnetic impurities (e.g., the Kondo physics), because there are spin-exchange interactions (SEIs) between two atoms in the electronic ground (1S0^{1}\mathrm{S}_{0}1S0​) and metastable (3P^{3}\mathrm{P}3P) state, respectively. Nevertheless, this SEI cannot be tuned via magnetic Feshbach resonance. In this paper, we propose three methods to control the SEI between one atom in the 1S0^{1}\mathrm{S}_{0}1S0​ state and another atom in the 3P2^{3}\mathrm{P}_{2}3P2​ states or $^{3}\mathrm{P}_{2}\text{\ensuremath{-}}^{3}\mathrm{P}_{0}$ dressed states, with one or two laser beams. These methods are based on the spin-dependent ac-Stark shifts of the 3P2^{3}\mathrm{P}_{2}3P2​ states or the $^{3}\mathrm{P}_{2}\text{\ensuremath{-}}^{3}\mathrm{P}_{0}$ Raman coupling. We show that due to the structure of alkaline-earth (like) atoms, the heating effects induced by the laser beams of our methods are very weak. For instance, for ultracold Yb atoms, ac-Stark-shift difference of variant spin states of the 3P2(F=3/2)^{3}\mathrm{P}_{2}(F=3/2)3P2​(F=3/2) level, or the strength of the $^{3}\mathrm{P}_{2}\text{\ensuremath{-}}^{3}\mathrm{P}_{0}$ Raman coupling, could be of the order of $(2\ensuremath{\pi})\phantom{\rule{0.28em}{0ex}}\mathrm{MHz}$, while the heating rate (photon scattering rate) is only of the order of Hz. As a result, the Feshbach resonances, with which one can efficiently control the SEI by changing the laser intensity, may be induced by the laser beams with a low-enough heating rate, even if the scattering lengths of the bare interatomic interaction are so small that they are comparable with the length scale associated with the van der Waals interaction.