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arXiv:1712.05759 · Physical Review Letters

Response Functions as Quantifiers of Non-Markovianity

Philipp Strasberg, Massimiliano Esposito

Published Jul 24, 2018• 27 citations
arXivHTMLPDF

Abstract

Quantum non-Markovianity is crucially related to the study of dynamical maps, which are usually derived for initially factorized system-bath states. We demonstrate that linear response theory also provides a way to derive dynamical maps but for initially correlated (and, in general, entangled) states. Importantly, these maps are always time-translational invariant and allow for a much simpler quantification of non-Markovianity compared to previous approaches. We apply our theory to the Caldeira-Leggett model, for which our quantifier is valid beyond linear response and can be expressed analytically. We find that a classical Brownian particle coupled to an Ohmic bath can already exhibit non-Markovian behavior, a phenomenon related to the initial state preparation procedure. Furthermore, for a peaked spectral density, we show that there is no monotonic relation between our quantifier and the system-bath coupling strength, the sharpness of the peak or the resonance frequency in the bath.

DOI
10.1103/physrevlett.121.040601

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Quantum non-Markovianity is crucially related to the study of dynamical maps, which are usually derived for initially factorized system-bath states. We demonstrate that linear response theory also provides a way to derive dynamical maps but for initially correlated (and, in general, entangled) states. Importantly, these maps are always time-translational invariant and allow for a much simpler quantification of non-Markovianity compared to previous approaches. We apply our theory to the Caldeira-Leggett model, for which our quantifier is valid beyond linear response and can be expressed analytically. We find that a classical Brownian particle coupled to an Ohmic bath can already exhibit non-Markovian behavior, a phenomenon related to the initial state preparation procedure. Furthermore, for a peaked spectral density, we show that there is no monotonic relation between our quantifier and the system-bath coupling strength, the sharpness of the peak or the resonance frequency in the bath.
For many open quantum systems, a master equation approach employing the Markov approximation cannot reliably describe the dynamical behaviour. This is the case, for example, in a number of solid state or biological systems, and it has motivated a line of research aimed at quantifying the amount of non-Markovian behaviour in a given model. Within this framework, we investigate the dynamics of a quantum harmonic oscillator linearly coupled to a bosonic bath. We focus on Gaussian states, which are suitably treated using a covariance matrix approach. Concentrating on an entanglement based non-Markovian behaviour quantifier (NMBQ) proposed by Rivas et. al. [1], we consider the role that near resonant and off-resonant modes play in affecting the NMBQ. By using a large but finite bath of oscillators for both Ohmic and super Ohmic spectral densities we find, by systematically increasing the coupling strength, initially the near resonant modes provide the most significant non-Markovian effects, while after a certain threshold of coupling strength the off-resonant modes play the dominant role. We also consider the NMBQ for two other models where we add a single strongly coupled oscillator to the model in extra bath mode and 'buffer' configurations, which affects the modes that determine non-Markovian behaviour.
We study quantum non-Markovian dynamics of the Caldeira-Leggett model, a prototypical model for quantum Brownian motion describing a harmonic oscillator linearly coupled to a reservoir of harmonic oscillators. Employing the exact analytical solution of this model one can determine the size of memory effects for arbitrary couplings, temperatures, and frequency cutoffs. Here, quantum non-Markovianity is defined in terms of the flow of information between the open system and its environment, which is quantified through the Bures metric as distance measure for quantum states. This approach allows us to discuss quantum memory effects in the whole range from weak to strong dissipation for arbitrary Gaussian initial states. A comparison of our results with the corresponding results for the spin-boson problem show a remarkable similarity in the structure of non-Markovian behavior of the two paradigmatic models.
In this work, we investigate the non-Markovian features of the Adapted Caldeira-Leggett model, a computationally efficient framework recently proposed to capture the essential physics of the standard Caldeira-Leggett model. While this effective model has been previously validated for decoherence and einselection, its ability to reproduce memory effects remains to be explored. By exploiting the model's capability to explicitly track both system and environment degrees of freedom, we provide a detailed characterization of non-Markovianity through the lens of information backflow. We evaluate the buildup of system-environment correlations and the corresponding modifications of the environmental state, assessing a quantitative upper bound for the revival of distinguishability in the reduced dynamics. Our results, obtained by comparing different distinguishability quantifiers such as trace distance and the square root of the Jensen-Shannon divergence, show that while correlations are primarily sensitive to coupling strength, environmental state changes are more heavily influenced by temperature. Our analysis substantiates the physical interpretation of the distinguishability-based approach to non-Markovianity, and confirms this variant of the Caldeira-Leggett model as a reliable tool for exploring the microscopic origins of different fundamental phenomena in quantum mechanics.
By extending the response function approach developed in nonlinear optics, we analytically derive an expression for the non-Markovianity in the time evolution of a system in contact with a quantum mechanical bath, and find a close connection with the directly observable nonlinear optical response. The result indicates that memory in the bath-induced fluctuations rather than in the dissipation causes non-Markovianity. Initial correlations between states of the system and the bath are shown to be essential for a correct understanding of the non-Markovianity. These correlations are included in our treatment through a preparation function.
We determine the frequency-dependent response characteristics of a quantum system to a driven Caldeira-Leggett bath. The bath degrees of freedom are explicitly driven by an external time-dependent force, in addition to the direct time-dependent forcing of the system itself. After general considerations of driven Caldeira-Leggett baths, we consider the Rubin model of a chain of quantum particles coupled by linear springs as an important model of a quantum dissipative system. We show that in the presence of time-dependent driving of the chain, this model can be mapped to a quantum system which couples to a driven Caldeira-Leggett bath. The effect of the bath driving is captured by a time-dependent force on the central system, which is, in principle, non-Markovian in nature. We study two specific examples, the exactly solvable case of a harmonic potential and a quantum two-state system for which we assume a weak system-bath coupling. We evaluate the dynamical response to a periodic driving of the system and the bath. The dynamic susceptibility is shown to be altered qualitatively by the bath drive: The dispersive part is enhanced at low frequencies and acquires a maximum at zero frequency. The absorptive part develops a shoulder-like behavior in this frequency regime. These features seem to be generic for quantum systems in a driven Caldeira-Leggett bath.
Abstract We investigate the dynamics of quantum correlations in bipartite systems initially prepared in a squeezed state, comparing closed-system unitary evolution under the Schrödinger equation with open-system dynamics governed by the Caldeira-Leggett master equation in the high-temperature, weak-coupling regime, all within the Bohmian mechanics framework. Quantum nonlocality is quantified via the sensitivity of the Bohmian velocity of one particle to the position of the other. Our results show that in both distinct (local) and common bath scenarios, nonlocal correlations initially grow from zero, reach a peak, and then decay. In the case of local baths, the decay is smooth and monotonic; although the peak value increases with temperature, its temporal width (measured via the full width at half maximum) decreases, indicating a shorter duration of nonlocal correlations. For a common bath, the initial growth and decay are followed by revivals and oscillations, whose amplitude and timing vary with temperature. These non-monotonic behaviors arise despite the Markovian nature of the underlying dynamics and reflect the nontrivial role of system-bath correlations. We also analyze how both temperature and the squeezing decay parameter affect the structure of Bohmian trajectories and the evolution of nonlocal correlations. This trajectory-based, velocity-sensitivity measure offers an intuitive and quantitative understanding of entanglement degradation, decoherence, and their characteristic time scales. Our findings emphasize how the structure of the environment critically shapes the observable dynamics of quantum correlations, even in Markovian regimes.