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arXiv:1712.04312 · Physical Review Letters

Directional Dicke Subradiance with Nonclassical and Classical Light Sources

Daniel Bhatti, Raimund Schneider, Steffen Oppel, Joachim von Zanthier

Published Mar 16, 2018• 37 citations
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Abstract

We investigate Dicke subradiance of N≥2 distant quantum sources in free space, i.e., the spatial emission patterns of spontaneously radiating noninteracting multilevel atoms or multiphoton sources, prepared in totally antisymmetric states. We find that the radiated intensity is marked by a full suppression of spontaneous emission in particular directions. In resemblance to the analogous, yet inverted, superradiant emission profiles of N distant two-level atoms prepared in symmetric Dicke states, we call the corresponding emission patterns directional Dicke subradiance. We further derive that higher-order intensity correlations of the light emitted by statistically independent thermal light sources display the same directional Dicke subradiant behavior and show that it stems from the same interference phenomenon as in the case of quantum sources. We finally present measurements of directional Dicke subradiance for N=2,…,5 distant thermal light sources corroborating the theoretical findings.

DOI
10.1103/physrevlett.120.113603

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We investigate Dicke subradiance of N≥2 distant quantum sources in free space, i.e., the spatial emission patterns of spontaneously radiating noninteracting multilevel atoms or multiphoton sources, prepared in totally antisymmetric states. We find that the radiated intensity is marked by a full suppression of spontaneous emission in particular directions. In resemblance to the analogous, yet inverted, superradiant emission profiles of N distant two-level atoms prepared in symmetric Dicke states, we call the corresponding emission patterns directional Dicke subradiance. We further derive that higher-order intensity correlations of the light emitted by statistically independent thermal light sources display the same directional Dicke subradiant behavior and show that it stems from the same interference phenomenon as in the case of quantum sources. We finally present measurements of directional Dicke subradiance for N=2,…,5 distant thermal light sources corroborating the theoretical findings.
Superradiance has been an outstanding problem in quantum optics since Dicke introduced the concept of enhanced directional spontaneous emission by an ensemble of identical two-level atoms. The effect is based on the correlated collective Dicke states which turn out to be highly entangled. Here we show that enhanced directional emission of spontaneous radiation can be produced also with statistically independent incoherent sources, via the measurement of higher-order correlation functions of the emitted radiation. Our analysis is applicable to a wide variety of quantum emitters, like trapped atoms, ions, quantum dots, or nitrogen-vacancy centers, and is also valid for incoherent classical emitters. This is experimentally confirmed with up to eight statistically independent thermal light sources. The arrangement to measure the higher-order correlation functions corresponds to a generalized Hanbury Brown-Twiss setup, demonstrating that the two phenomena, superradiance and the Hanbury Brown-Twiss effect, stem from the same interference phenomenon.
Dicke superradiance, i.e., the enhanced spontaneous emission of coherent radiation, is often attributed to radiation emitted by synchronized dipoles coherently oscillating in phase. At the same time, Dicke derived superradiance assuming atoms in entangled Dicke states which do not display any dipole moment. To shed light on this apparent paradox, we study the intensity distribution arising from two identical two-level atoms prepared either in an entangled Dicke state or in a separable atomic state with a nonvanishing dipole moment. We find that the two configurations produce similar far-field intensity patterns, although they stem from fundamentally distinct types of coherence: while in the second case the atoms display coherence among the individual particles, leading to Young-type interference like that known from classical dipoles, atoms in Dicke states possess collective quantum coherence stemming from entanglement and quantum correlations of the state, leading to an interference pattern resulting from enhanced spontaneous emission. This demonstrates that the radiation generated by synchronized dipoles and Dicke superradiance---even if they do produce the same interference pattern---are fundamentally distinct phenomena and have to be interpreted in different ways.
Fully excited two-level atoms separated by less than the transition wavelength cooperatively emit light in a short burst, a phenomenon called superradiance by R. Dicke in 1954 [Phys. Rev. 93, 99 (1954)]. The burst is characterized by a maximum intensity scaling with the square of the number of atoms NNN and a temporal width reduced by NNN compared to the single atom spontaneous decay time. Both effects are usually attributed to a synchronization of the electric dipole moments of the atoms occurring during the process of light emission. Contrary to this explanation, it was recently shown by use of a quantum path description that the peak intensity results from the quantum correlations among the atoms when occupying symmetric Dicke states. Here we investigate from this perspective the temporal evolution of the ensemble, starting in the small sample limit, i.e., when the atoms have mutual separations much smaller than the transition wavelength $\ensuremath{\lambda}$ and pass down the ladder of symmetric Dicke states. In addition, we explore the temporal evolution for the case of distant noninteracting atoms with mutual separations much larger than $\ensuremath{\lambda}$. We show that in this case a similar superradiant burst of the emitted radiation is observed if the quantum correlations of the atoms are generated by conditional photon measurements retaining the atomic ensemble within or close to the symmetric subspace.
In this paper we investigate the close relationship between Dicke superradiance, originally predicted for an ensemble of two-level atoms in entangled states, and the Hanbury Brown and Twiss effect, initially established in astronomy to determine the dimensions of classical light sources such as stars. By studying the state evolution of the fields produced by classical sources---defined by a positive Glauber-Sudarshan PPP function---when recording intensity correlations of higher order in a generalized Hanbury Brown and Twiss setup we find that the angular distribution of the last detected photon, apart from an offset, is identical to the superradiant emission pattern generated by an ensemble of two-level atoms in entangled symmetric Dicke states. We show that the phenomenon derives from projective measurements induced by the measurement of photons in the far field of the sources and the permutative superposition of quantum paths identical to those leading to superradiance in the case of single photon emitters. We thus point out an important similarity between classical sources and quantum emitters upon detection of photons if the particular photon source remains unknown. We finally present a compact result for the characteristic functional which generates intensity correlations of arbitrary order for any kind of light source.
We calculate the radiative characteristics of emission from a system of entangled atoms which can have a relative distance larger than the emission wavelength. We develop a quantum multipath interference approach which explains both super- and subradiance though the entangled states have zero dipole moment. We derive a formula for the radiated intensity in terms of different interfering pathways. We further show how the interferences lead to directional emission from atoms prepared in symmetric WWW states. As a byproduct of our work we show how Dicke's classic result can be understood in terms of interfering pathways. In contrast to the previous works on ensembles of atoms, we focus on finite numbers of atoms prepared in well characterized states.
Superradiance, i.e., spontaneous emission of coherent radiation by an ensemble of two-level atoms in collective states introduced by Dicke in 1954, is one of the enigmatic problems of quantum optics. The startling gist is that even though the atoms have no dipole moment they radiate with increased intensity in particular directions. Following the advances in our understanding of superradiant emission by atoms in entangled W-states we examine the quantum statistical properties of superradiance. Such investigations require the system to have at least two excitations in order to explore the photon-photon correlations of the radiation emitted by such states. We present specifically results for the spatially resolved photon-photon correlations of systems prepared in doubly excited W-states and give conditions when the atomic system emits nonclassial light. Equally, we derive the conditions for the occurrence of bunching and even of superbunching, a rare phenomenon otherwise known only from nonclassical states of light like the squeezed vacuum. We finally investigate the photon-photon cross correlations of the spontaneously scattered light and highlight the nonclassicalty of such correlations. The theoretical findings can be implemented with current technology, e.g., using ions in a linear rf-trap, atoms in an optical lattice or quantum dots in a cavity.