Ultrafast electronic dynamics are typically studied using pulsed lasers. Here we demonstrate a complementary experimental approach: quantum simulation of ultrafast dynamics using trapped ultracold atoms. Counter-intuitively, this technique emulates some of the fastest processes in atomic physics with some of the slowest, leading to a temporal magnification factor of up to 12 orders of magnitude. In these experiments, time-varying forces on neutral atoms in the ground state of a tunable optical trap emulate the electric fields of a pulsed laser acting on bound charged particles. We demonstrate the correspondence with ultrafast science by a sequence of experiments: nonlinear spectroscopy of a many-body bound state, control of the excitation spectrum by potential shaping, observation of sub-cycle unbinding dynamics during strong few-cycle pulses, and direct measurement of carrier-envelope phase dependence of the response to an ultrafast-equivalent pulse. These results establish cold-atom quantum simulation as a complementary tool for studying ultrafast dynamics.
Ultrafast electronic dynamics are typically studied using pulsed lasers. Here we demonstrate a complementary experimental approach: quantum simulation of ultrafast dynamics using trapped ultracold atoms. Counter-intuitively, this technique emulates some of the fastest processes in atomic physics with some of the slowest, leading to a temporal magnification factor of up to 12 orders of magnitude. In these experiments, time-varying forces on neutral atoms in the ground state of a tunable optical trap emulate the electric fields of a pulsed laser acting on bound charged particles. We demonstrate the correspondence with ultrafast science by a sequence of experiments: nonlinear spectroscopy of a many-body bound state, control of the excitation spectrum by potential shaping, observation of sub-cycle unbinding dynamics during strong few-cycle pulses, and direct measurement of carrier-envelope phase dependence of the response to an ultrafast-equivalent pulse. These results establish cold-atom quantum simulation as a complementary tool for studying ultrafast dynamics.
Abstract Ultrafast electronic dynamics are typically studied using pulsed lasers. Here we demonstrate a complementary experimental approach: quantum simulation of ultrafast dynamics using trapped ultracold atoms. Counter-intuitively, this technique emulates some of the fastest processes in atomic physics with some of the slowest, leading to a temporal magnification factor of up to 12 orders of magnitude. In these experiments, time-varying forces on neutral atoms in the ground state of a tunable optical trap emulate the electric fields of a pulsed laser acting on bound charged particles. We demonstrate the correspondence with ultrafast science by a sequence of experiments: nonlinear spectroscopy of a many-body bound state, control of the excitation spectrum by potential shaping, observation of sub-cycle unbinding dynamics during strong few-cycle pulses, and direct measurement of carrier-envelope phase dependence of the response to an ultrafast-equivalent pulse. These results establish cold-atom quantum simulation as a complementary tool for studying ultrafast dynamics.
We demonstrate a physical quantum simulator of ultrafast phenomena, in which
time-varying forces on neutral atoms in a tunable optical trap emulate the
electric fields of a pulsed laser acting on electrons or nuclei in a binding
potential. The simulator operates in regimes equivalent to those of ultrafast
and strong-field pulsed-laser experiments, opening up a hitherto unexplored
application of quantum simulation techniques and a complementary path towards
investigating open questions in ultrafast science. Counter-intuitively, this
approach emulates some of the fastest processes in atomic physics with some of
the slowest, giving rise to a temporal magnification factor of up to twelve
orders of magnitude which greatly simplifies experimental access to the
dynamics. The correspondence with ultrafast science is demonstrated by a
sequence of experiments: we perform nonlinear spectroscopy of a many-body bound
state, control the excitation spectrum by shaping the potential, observe
sub-cycle unbinding dynamics during strong few-cycle pulses, and directly
measure carrier-envelope phase dependence of the response to an
ultrafast-equivalent pulse.
Weakly-interacting atoms in a Bose-Einstein condensate coherently occupy the ground-state of their container. This phenomenon, coupled with the technical ability to produce precise, isolated and dynamically-tunable trapping potentials, makes ultracold atoms a versatile platform for simulating quantum mechanical systems. This thesis details the construction of two apparatus at the University of California, Santa Barbara for the production of Bose-Einstein condensates of lithium and strontium atoms respectively. Results of the first experiment performed on the strontium apparatus, a quantum simulation of ultrafast dynamics, are presented. In this experiment, driven cold atoms simulate ultrafast ionization dynamics in attosecond laser pulses, counter-intuitively emulating some of the fastest processes in atomic physics with some of the slowest. A sequence of experiments which demonstrate the correspondence with ultrafast science are described, including the direct observation of carrier-envelope-phase dependent sub-cycle unbinding dynamics. Preliminary results from a second experiment, studying phasonic excitations in a quasiperiodic lattice, are also discussed.
The demanding experimental access to the ultrafast dynamics of materials challenges our understanding of their electronic response to applied strong laser fields. For this purpose, trapped ultracold atoms with highly controllable potentials have become an enabling tool to describe phenomena in a scenario in which some effects are more easily accessible and 12 orders of magnitude slower. In this work, we introduce a mapping between the parameters of attoscience platforms and atomic cloud simulators and propose an experimental protocol to access the emission spectrum of high-harmonic generation, a regime that has so far been elusive to cold-atom simulation. As we illustrate, the benchmark offered by these simulators can provide new insights into the conversion efficiency of extended and short nuclear potentials, as well as the response to applied elliptical polarized fields or ultrashort few-cycle pulses. Published by the American Physical Society 2024
Ultracold matter offers a unique capability to reach the best high-precision spectroscopy measurements and leads to exciting perspectives in many different areas of science and technology. Molecules, thanks to their complex spectra, couple with a broader range of photons compared to atoms, so they are extremely attractive for fundamental science or to design new quantum technologies. However, to date, only a few molecular species have been brought to temperatures of the order of the microkelvin. This was done by laser cooling, a process that has been demonstrated only for species featuring an unpaired electron that does not participate to the chemical bond. \n \nA different approach, which is indifferent to the molecule electronic structure and thus potentially universal, is sympathetic cooling, where neutral molecules are cooled in a bath of ultracold atoms. However, inelastic collisions between molecules and the coolant is a major obstacle that has hindered the advances of this method thus far. Trapping the molecules in their absolute ground state would circumvent this problem or at least greatly simplify it. In this thesis we simulate the feasibility of an experiment in which metastable CO molecules are first slowed down to a few m/s with a microstructured Stark decelerator, then they are stopped by a strong DC electrical barrier and finally they are transferred irreversibly to their absolute ground state and captured in an optical trap. \nUnfortunately, the results of the simulations indicate that the total number of molecules that can be accumulated in the optical trap is rather low, far behind the observation threshold. Therefore, we concluded that other approaches to produce ultracold molecules must to be searched.
Ultracold quantum gases offer a versatile platform to study a wide range of open questions in condensed matter physics and beyond. In particular, their controllability, isolation from noisy thermal environments, and evolution on experimentally-accessible timescales make them a natural choice to probe the effects of driving on time evolution and energy. This thesis details the construction of two cold-atom apparatuses, a lithium machine and a strontium machine, for quantum emulation experiments studying driven systems. Initial numerical simulations along two experimental lines are briefly discussed, and results from the first two experiments on the strontium machine are then presented. In the first, a strontium Bose-Einstein condensate in an optical trap is strongly driven to emulate ultrafast photoionization processes; in a series of proof-of-principle experiments measuring the momenta and energy of particles ejected from the trap, we demonstrate the viability of this technique to study open questions in strong-field physics. The second experiment realizes a tunable quasicrystal, the energy structure for which is described by the multifractal Hofstadter butterfly. Quasiperiodic structures host not only phonons, but also a higher-dimension analogue called phasons. In the experiment, we demonstrate phasonic spectroscopy for the first time by directly driving one of these modes; we characterize the coupling to the resulting excitations, and directly map a slice of the Hofstadter energy spectrum.