Self-Bound Quantum Droplets of Atomic Mixtures in Free Space
Giulia Semeghini, Giovanni Ferioli, L. Masi, Chiara Mazzinghi, L. Wolswijk, F. Minardi, Michele Modugno, Giovanni Carlo Modugno, M. Inguscio, M. Fattori
Self-bound quantum droplets are a newly discovered phase in the context of ultracold atoms. In this Letter, we report their experimental realization following the original proposal by Petrov [Phys. Rev. Lett. 115, 155302 (2015)PRLTAO0031-900710.1103/PhysRevLett.115.155302], using an attractive bosonic mixture. In this system, spherical droplets form due to the balance of competing attractive and repulsive forces, provided by the mean-field energy close to the collapse threshold and the first-order correction due to quantum fluctuations. Thanks to an optical levitating potential with negligible residual confinement, we observe self-bound droplets in free space, and we characterize the conditions for their formation as well as their size and composition. This work sets the stage for future studies on quantum droplets, from the measurement of their peculiar excitation spectrum to the exploration of their superfluid nature.
Self-bound quantum droplets are a newly discovered phase in the context of ultracold atoms. In this Letter, we report their experimental realization following the original proposal by Petrov [Phys. Rev. Lett. 115, 155302 (2015)PRLTAO0031-900710.1103/PhysRevLett.115.155302], using an attractive bosonic mixture. In this system, spherical droplets form due to the balance of competing attractive and repulsive forces, provided by the mean-field energy close to the collapse threshold and the first-order correction due to quantum fluctuations. Thanks to an optical levitating potential with negligible residual confinement, we observe self-bound droplets in free space, and we characterize the conditions for their formation as well as their size and composition. This work sets the stage for future studies on quantum droplets, from the measurement of their peculiar excitation spectrum to the exploration of their superfluid nature.
We revisit the Bogoliubov theory of quantum droplets proposed by Petrov [Phys. Rev. Lett. 115, 155302 (2015)PRLTAO0031-900710.1103/PhysRevLett.115.155302] for an ultracold Bose-Bose mixture, where the mean-field collapse is stabilized by the Lee-Huang-Yang quantum fluctuations. We show that a loophole in Petrov's theory, i.e., the ignorance of the softening complex Bogoliubov spectrum, can be naturally removed by the introduction of bosonic pairing. The pairing leads to weaker mean-field attractions, and also a stronger Lee-Huang-Yang term in the case of unequal intraspecies interactions. As a result, the equilibrium density for the formation of self-bound droplets significantly decreases in the deep droplet regime, in agreement with a recent observation from diffusion Monte Carlo simulations. Our construction of a consistent Bogoliubov theory paves the way to understand the puzzling low critical number of small quantum droplets observed in the experiment [C. Cabrera et al., Science 359, 301 (2018)SCIEAS0036-807510.1126/science.aao5686].
Abstract We study weakly interacting mixtures of ultracold atoms composed of bosonic and fermionic species in 2D and 1D. When interactions between particles are appropriately tuned, self-bound quantum liquids can be formed. We show that while formation of these droplets in 2D is due to the higher order correction terms contributing to the total energy and originating in quantum fluctuations, in 1D geometry the quantum fluctuations have a negligible role on formation of the self-bound systems. The leading mean-field interactions are then sufficient for droplet formation in 1D. We analyze energetic stability for 2D and 1D systems and predict values of equilibrium densities of droplets.
Among settings which have recently been elaborated for the creation of stable multidimensional solitons, most advanced, as concerns the theory and experiment alike, is the work with quantum droplets (QDs) in atomic BEC. Important theoretical predictions for fundamental and topologically structured soliton-like (stably self-trapped) QDs have been published in many papers, starting from the pioneering work of Petrov [Phys. Rev. Lett. 115, 155302 (2015)]. Simultaneously, the experimental advancement in the making of QDs in binary BECs, as well as in single-component BECs of atoms carrying magnetic dipole moments, have been really remarkable and unique. Successful experiments followed the first theoretical prediction of the QDs very quickly, and the progress in the experimental work was much faster than in other areas of physics where stable multidimensional solitons were predicted. The basis of these works is a correction to the MF (mean-field) BEC dynamics produced by quantum fluctuations around MF states. The correction was first predicted in 1957 by Lee, Huang, and Yang (LHY). The breakthrough proposal made by Petrov [Phys. Rev. Lett. 115, 155302 (2015)] was to use the effective higher-order (quartic) self-repulsion, produced by the LHY effect in the atomic BEC, as a mechanism arresting the collapse driven by mutual attraction of two self-repulsive components in a binary quantum bosonic gas. The balance between the inter-species attraction and LHY-induced self-repulsion gives rise to stable 3D and quasi-2D (pancake-shaped) localized bound states in the form of the quantum droplets (QDs). In single-component condensates of magnetic atoms, the attraction is provided by the long-range dipole–dipole interaction (Chomaz et al., 2016; Schmitt et al., 2016). The competition between the MF attraction and LHY repulsion maintains a superfluid state whose density (taking very low values) cannot exceed a certain maximum, thus making it effectively incompressible. This is a reason why this quantum macroscopic state of matter is identified as a superfluid. Accordingly, localized states filled by this quantum fluid are called “droplets.” In addition to the 3D QDs, droplets in the effectively 2D setting, which may exist under the action of tight confinement in one direction, imposed by an external potential, were theoretically predicted [Petrov and Astrakharchik, Phys. Rev. Lett. 117, 100401 (2016)] and experimentally created [Cabrera et al., Science 359, 301-304 (2018)] too. This chapter provides a condensed review of basic theoretical results for stable QDs in binary BECs, maintained through the stable balance between the inter-species attraction and intra-species LHY repulsion. Both fundamental modes and ones with embedded vorticity are considered. The presentation is partly based on a review article by Luo et al. [Front. Phys. 16, 32501 (2021)]. In addition to 2D and 3D self-trapped QDs in free space, the present chapter addresses 2D fundamental and vortex modes trapped in a singular attractive potential, ∼−1/r2, which are stabilized by the LHY repulsion. Two subsequent chapters present a summary of experimental findings for QDs in binary BECs and for QDs in single-component BECs of magnetic atoms.
These lecture notes contain an introduction to quantum simulation of bosonic systems in the continuum, focusing on weakly interacting Bose-Bose mixtures with competing mean-field interactions. When the values of such interactions are fine-tuned to almost completely cancel the mean-field energy, quantum fluctuations become apparent and dominate the behavior of the system, stabilizing an ultradilute quantum liquid phase. An analogous situation appears in single-component dipolar quantum gases. We review the mechanism that gives rise to this exotic quantum liquid, which can form droplets that are self-bound in the absence of any external confinement, and discuss their properties and dynamics in both the mixture and the dipolar cases. In dipolar gases, arrays of dipolar droplets stabilized by quantum fluctuations can establish global phase coherence and form supersolids. In bosonic mixtures, supersolidity can emerge already at the mean-field level through spin-orbit coupling. We discuss the properties of such spin-orbit-coupled supersolids, comparing them to their dipolar counterparts. Specifically, we focus on their periodic density modulation, phase coherence, and peculiar excitation spectrum, which hosts both superfluid and crystal excitations. Finally, we conclude by discussing open research directions in the areas of quantum liquid droplets and spin-orbit-coupled supersolids, in particular at the interface of the two research topics.
While quantum fluctuations in binary mixtures of bosonic atoms with short-range interactions can lead to the formation of a self-bound droplet, for equal intracomponent interactions but an unequal number of atoms in the two components, there is an excess part that cannot bind to the droplet. Imposing confinement, as here through periodic boundary conditions in a one-dimensional setting, the droplet becomes amalgamated with a residual condensate. The rotational properties of this compound system reveal simultaneous rigid-body and superfluid behavior in the ground state and uncover that the residual condensate can carry angular momentum even in the absence of vorticity. In contradiction to the intuitive idea that the superfluid fraction of the system would be entirely made up of the excess atoms not bound by the droplet, we find evidence that this fraction is higher than what one would expect in such a picture. Our findings are corroborated by an analysis of the elementary excitations in the system, and shed new light on the coexistence of localization and superfluidity.