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arXiv:1710.10562 · Scientific Reports

Photon antibunching control in a quantum dot and metallic nanoparticle hybrid system with non-Markovian dynamics

Tara Moradi, M. Bagheri Harouni, M. H. Naderi

Published Aug 14, 2018• 11 citations
arXivHTMLPDF

Abstract

Photon-number statistics of the emitted photons from a quantum dot placed in the vicinity of a metallic nanoparticle driven by a laser in the non-Markovian regime is investigated theoretically. In the model scheme, the quantum dot is considered as an InAs three-level system in L-type configuration with two transition channels. We aim to introduce the hybrid system as a nonclassical photon source and control the antibunching behavior of the emitted photons by the geometrical as well as the physical parameters of the hybrid system. Our approach is based on the classical Green's function technique and time convolution master equation. The results reveal that the emitted photons from the hybrid system under consideration are antibunched and energy is exchanged between the QD and nanoshell. By increasing the QD-MNP separation distance, the detuning frequency between the QD transitions and surface plasmon modes, and the Rabi frequency the antibunching time increases while the backaction of the reservoir on the QD decreases. To sum up, we conclude that the studied system has the potential to be a highly controllable single-photon source.

DOI
10.1038/s41598-018-29799-4

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Photon-number statistics of the emitted photons from a quantum dot placed in the vicinity of a metallic nanoparticle driven by a laser in the non-Markovian regime is investigated theoretically. In the model scheme, the quantum dot is considered as an InAs three-level system in L-type configuration with two transition channels. We aim to introduce the hybrid system as a nonclassical photon source and control the antibunching behavior of the emitted photons by the geometrical as well as the physical parameters of the hybrid system. Our approach is based on the classical Green's function technique and time convolution master equation. The results reveal that the emitted photons from the hybrid system under consideration are antibunched and energy is exchanged between the QD and nanoshell. By increasing the QD-MNP separation distance, the detuning frequency between the QD transitions and surface plasmon modes, and the Rabi frequency the antibunching time increases while the backaction of the reservoir on the QD decreases. To sum up, we conclude that the studied system has the potential to be a highly controllable single-photon source.
We theoretically study the dissipative dynamics of a quantum emitter placed near the planar surface of a metal supporting surface-plasmon excitations. The emitter-metal coupling regime can be tuned by varying some control parameters such as the qubit-surface separation and/or the detuning between characteristic frequencies. By using a Green's-function approach jointly with a time-convolutionless master equation, we analyze the non-Markovian dissipative features on the qubit time evolution in two cases of interest: (i) an undriven qubit initially prepared in its excited state and (ii) the evolution toward a steady state for a system driven by a laser field. For weak to moderate qubit-metal coupling strength, and on time scales large compared to the surface plasmon oscillation time, a Markovian approximation for the master-equation results to be adequate to describe the qubit main optical properties: surface enhancements of rate emission, optical spectra, and time-dependent photon-photon correlation functions. The qubit decay shows a crossover passing from being purely dissipative for small qubit-surface distances to plasmon emission for larger separations.
We study the spectrum and statistical properties of photons scattered from a semiconductor-quantum-dot--metal-nanoparticle system under monochromatic and bichromatic excitations. We rely on the Bloch equation to describe the evolution of the density matrix of the quantum dot. We pay attention to the self-interaction of the quantum dot in the presence of the nanoparticle. Going beyond the dipole approximation, we show that the system exhibits optical responses of different character in different regions of the quantum dot dipole moment versus the nanoparticle radius phase diagram. In the strong transition and bistability regions, upon changing the initial state, a pronounced fluorescence spectrum may become a faint one, and an oscillatory intensity-intensity correlation may become a monotonically increasing one. The amplitudes, frequencies, and phases of the laser fields tailor the number, position, height, and width of the peaks of the fluorescence spectrum. The antibunched light as well as the sub-Poissonian light can be generated. Our results suggest that in view of solid-state-based sources of nonclassical light, a hybrid quantum-dot--nanoparticle system may be superior to an isolated quantum dot.
Abstract In this paper, we study the tunneling induced optical bistability (OB) in a quantum dot (QD)-metallic nanoparticle (MNP) hybrid system via surface plasmon effects. We realized that in the presence of the tunneling effect, OB arises when the probe light is parallel to the major axis of the hybrid system. We realized the threshold of OB can be controlled by controlling the distance parameter between the QD and MNP. For appropriate distance between the QD and MNP, we find that optical multistability (OM) appears in the system. We find that the threshold of OM can be adjusted when we consider the radius effect of the MNP, respectively.
In the present work, we theoretically/numerically study the optical second-order sideband generation in a hybrid structure consisting of a semiconductor quantum dot (QD) conjugated with DNA molecules, and coupled to a solid metallic nanoparticle (MNP) or a metallic nanoshell (MNS) with core-shell geometry. The hybrid system is driven by a strong control (pump) laser field and a weak signal (probe) field. The dynamics of the system is analyzed using the Heisenberg equation of motion in the frame of rotating wave approximation. We discuss the role of plasmon-exciton interaction in enhancing third- and fifth-order nonlinear susceptibilities through the nonlinear optical response of the system and the effects of the presence of a MNP or a MNS near the QD-DNA system on the nonlinear optical absorption spectrum is investigated. We demonstrate that the second-order sideband is generated, and the hybrid system considered here enables robust control and tunability of the second-order sidebands. It is shown that the second-order sideband spectrum (or absorption) is significantly affected by plasmonic nanoparticle size, the interparticle distance, the control field (Rabi frequency ), and the control-exciton detuning.
Plasmonic nanocomposites have the ability to enhance light-matter interaction due to the 1 plasmonic effects leading to promising potential applications. In this paper, we theoretically study the 2 group index of the silver nanoparticle-gold nanoparticle-quantum dot plasmonic hybrid system in 3 the optical region of the electromagnetic spectrum using the density matrix approach. The quantum 4 dot is considered to be a three-level atomic system of a lambda configuration, interacting with strong 5 control and weak probe fields. We find that the plasmonic hybrid system exhibits at near resonance a 6 strong switching between slow and fast light, which can be controlled by the inclination angle of the 7 gold nanoparticle and the size of the metals nanoparticles, in addition to the strength and detuning 8 of the control field. Thus, the silver nanoparticle-gold nanoparticle-quantum dot could potentially be 9 used in optoelectronic devices.10
Plasmonic nanocomposites have the ability to enhance light-matter interaction due to the plasmonic effects leading to promising potential applications. In this paper, we theoretically study the group index of the silver nanoparticle-gold nanoparticle-quantum dot plasmonic hybrid system in the optical region of the electromagnetic spectrum using the density matrix approach. The quantum dot is considered to be a three-level atomic system of a lambda configuration, interacting with strong control and weak probe fields. We find that the plasmonic hybrid system exhibits at near resonance a strong switching between slow and fast light, which can be controlled by the inclination angle of the gold nanoparticle and the size of the metals nanoparticles, in addition to the strength and detuning of the control field. Thus, the silver nanoparticle-gold nanoparticle-quantum dot could potentially be used in optoelectronic devices.