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arXiv:1710.07124 · Physical Review A

Lindblad formalism based on fermion-to-qubit mapping for nonequilibrium open quantum systems

Fabricio Macedo de Souza, L. Sanz

Published Nov 8, 2017• 8 citations
arXivHTMLPDF

Abstract

We present an alternative form of master equation, applicable to the analysis of nonequilibrium dynamics of fermionic open quantum systems. The formalism considers a general scenario, composed by a multipartite quantum system in contact with several reservoirs, each one with a specific chemical potential and in thermal equilibrium. With the help of Jordan-Wigner transformation, we perform a fermion-to-qubit mapping to derive a set of Lindblad superoperators that can be straightforwardly used on a wide range of physical setups. To illustrate our approach, we explore the effect of a charge sensor, acting as a probe, over the dynamics of electrons on coupled quantum molecules. The probe consists of a quantum dot attached to source and drain leads, that allows a current flow. The dynamics of populations, entanglement degree, and purity show how the probe is behind the sudden deaths and rebirths of entanglement, at short times. Then, the evolution leads the system to an asymptotic state being a statistical mixture. Those are signatures that the probe induces dephasing, a process that destroys the coherence of the quantum system.

DOI
10.1103/physreva.96.052110

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We present an alternative form of master equation, applicable to the analysis of nonequilibrium dynamics of fermionic open quantum systems. The formalism considers a general scenario, composed by a multipartite quantum system in contact with several reservoirs, each one with a specific chemical potential and in thermal equilibrium. With the help of Jordan-Wigner transformation, we perform a fermion-to-qubit mapping to derive a set of Lindblad superoperators that can be straightforwardly used on a wide range of physical setups. To illustrate our approach, we explore the effect of a charge sensor, acting as a probe, over the dynamics of electrons on coupled quantum molecules. The probe consists of a quantum dot attached to source and drain leads, that allows a current flow. The dynamics of populations, entanglement degree, and purity show how the probe is behind the sudden deaths and rebirths of entanglement, at short times. Then, the evolution leads the system to an asymptotic state being a statistical mixture. Those are signatures that the probe induces dephasing, a process that destroys the coherence of the quantum system.
We present the Born-Markov approximated Redfield quantum master equation (RQME) description for an open system of noninteracting particles (bosons or fermions) on an arbitrary lattice of NNN sites in any dimension and weakly connected to multiple reservoirs at different temperatures and chemical potentials. The RQME can be reduced to the Lindblad equation, of various forms, by making further approximations. By studying the N=2N=2N=2 case, we show that RQME gives results which agree with exact analytical results for steady-state properties and with exact numerics for time-dependent properties over a wide range of parameters. In comparison, the Lindblad equations have a limited domain of validity in nonequilibrium. We conclude that it is indeed justified to use microscopically derived full RQME to go beyond the limitations of Lindblad equations in out-of-equilibrium systems. We also derive closed-form analytical results for out-of-equilibrium time dynamics of two-point correlation functions. These results explicitly show the approach to steady state and thermalization. These results are experimentally relevant for cold atoms, cavity QED, and far-from-equilibrium quantum dot experiments.
Quantum systems are inherently open to their environment and thus they evolve under the influence of dissipation, decoherence and driving from external fields. This poses a significant theoretical challenge: how to track the dynamics of the system of interest while tracing out environmental degrees of freedom. Markovian master equations offer a longstanding solution to this problem, where under a series of assumptions the reduced density matrix of the system can be obtained. These flexible approaches provide a conceptually and numerically simple framework for describing complex many-body systems. However, the assumptions enforced by Markovian master equations create a gap in the availability of generic, simple, and analytical techniques capable of treating open quantum systems beyond the regimes of standard Markovian master equations. In this thesis, we introduce three studies addressing three regimes that are inaccessible to standard Markovian master equations and investigate their consequences in quantum thermodynamics-inspired applications. We begin by developing a Markovian embedding technique to tackle non-Markovian dynamics induced by the long correlation times of a qubit coupled to a structured environment. Subsequently, we propose an "effective" Hamiltonian theory enabling the study of equilibrium properties of strong coupling to a thermal reservoir through a dressed version of the Gibbs state. This framework can also be applied to address problems of equilibration, transport, quantum thermal machines, and quantum dynamics. Lastly, we showcase the importance of including non-secular terms in the quantum master equation, which results in a drastic separation of timescales leading to rich metastable dynamics. We apply this quantum master equation approach to temperature sensing in a nonequilibrium setting offering an alternative to standard equilibrium probes. Overall, this thesis contributes novel theoretical techniques for tackling open quantum systems beyond standard approximations with applications in quantum thermodynamics.
Abstract We consider the transition from the description of a closed quantum system consisting of an open quantum system and a reservoir to the description of the open quantum system alone by eliminating the reservoir degrees of freedom by averaging over them. An approach based on the Lindblad master equation for the density matrix is used. A general scheme is developed for deriving the Lindblad superoperator that emerges after averaging the von Neumann equation over the reservoir degrees of freedom. This scheme is illustrated with the cases of radiation of a two-level atom into free space and the dynamics of the transition of a two-level atom from a pure state to a mixed state due to interaction with a dephasing reservoir. Special attention is paid to the open system consisting of several subsystems each of which independently interacts with the reservoir. In the case of noninteracting subsystems, the density matrix is a tensor product of the subsystem density matrices, and the Lindblad superoperator of the system is a sum of Lindblad superoperators of those subsystems. The interaction between the subsystems results not only in the emergence of the corresponding term in the Hamiltonian of the combined system but also in the nonadditivity of the Lindblad superoperators. This is often overlooked in modern literature, possibly leading, as is shown in this methodological note, to serious errors; for example, the second law of thermodynamics could be violated.
We develop a superoperator coupled cluster method for nonequilibrium open many-body quantum systems described by the Lindblad master equation. The method is universal and applicable to systems of interacting fermions, bosons or their mixtures. We present a general theory and consider its application to the problem of quantum transport through the system with electron–phonon correlations. The results are assessed against the perturbation theory and nonequilibrium configuration interaction theory calculations.
Reservoir engineering has proven to be a practical approach to control open quantum systems, preserving quantum coherence by appropriately manipulating the reservoir and system-reservoir interactions. In this context, for systems comprised of different parts, it is common to describe the dynamics of a subsystem of interest by making an adiabatic elimination of the remaining components of the system. This procedure often leads to an effective master equation for the subsystem that is not in the well-known Gorini-Kossakowski-Lindblad-Sudarshan form (here called standard Lindblad form). Instead, it has a more general structure (here called generalized Lindblad form), which explicitly reveals the dissipative coupling between the various components of the subsystem. In this work, we present a set of dynamical equations for the first and second moments of the canonical variables for linear systems, bosonic and fermionic, described by master equations in a generalized Lindblad form. Our method is efficient and allows one to obtain analytical solutions for the steady state. Further, we include as a review some covariance matrix methods for which our results are particularly relevant, paying special attention to those related to the measurement of entanglement. Finally, we prove that the Duan criterion for entanglement is also applicable to fermionic systems.
The celebrated Lindblad equation governs the nonunitary time evolution of density operators used in the description of open quantum systems. It is usually derived from the von Neumann equation for a large system, at given physical conditions, when a small subsystem is explicitly singled out and the rest of the system acts as an environment whose degrees of freedom are traced out. In the specific case of a subsystem with variable particle number, the equilibrium density operator is given by the well-known grand canonical Gibbs state. Consequently, solving the Lindblad equation in this case should automatically yield, without any additional assumptions, the corresponding density operator in the limiting case of statistical equilibrium. Current studies of the Lindblad equation with varying particle number assume, however, the grand canonical Gibbs state a priori: the chemical potential is externally imposed rather than derived from first principles, and hence the corresponding density operator is not obtained as a natural solution of the equation. In this work, we investigate the compatibility of grand canonical statistical mechanics with the derivation of the Lindblad equation. We propose an alternative and complementary approach to the current literature that consists in using a generalized system Hamiltonian which includes a term μN. In a previous paper, this empirically well-known term has been formally derived from the von Neumann equation for the specific case of equilibrium. Including μN in the system Hamiltonian leads to a modified Lindblad equation which yields the grand canonical state as a natural solution, meaning that all the quantities involved are obtained from the physics of the system without any external assumptions.