We study the quantum correlations induced by spontaneous parametric down-conversion of a frequency comb. We derive a theoretical method to find the output state corresponding to a pump with an arbitrary spectral profile. After applying it to the relevant example of a spectrally chirped pump, we run an optimization algorithm to numerically find the pump profiles maximizing some target functions. These include the number of independently squeezed modes and the variances of nullifiers defining cluster states used in many continuous-variable quantum information protocols. To assess the advantages of pump shaping in real experiments, we take into account the physical limitations of the pulse shaper.
We study the quantum correlations induced by spontaneous parametric down-conversion of a frequency comb. We derive a theoretical method to find the output state corresponding to a pump with an arbitrary spectral profile. After applying it to the relevant example of a spectrally chirped pump, we run an optimization algorithm to numerically find the pump profiles maximizing some target functions. These include the number of independently squeezed modes and the variances of nullifiers defining cluster states used in many continuous-variable quantum information protocols. To assess the advantages of pump shaping in real experiments, we take into account the physical limitations of the pulse shaper.
Quantum optics has been, from its beginning, a driving force both for the exploration of fundamental limits of the quantum world and for conceiving seminal ideas and applications of the so-called quantum technologies. The last 20 years have seen a rapid development of ideas and proof-of-principle experiments involving the fields of quantum communication, quantum computation, quantum metrology and quantum simulation. The so called continuous variable (CV) approach to quantum optics, which uses many photon in collective states, and continuous observables like the quadratures of the electric field to encode information, has many interesting properties, especially from a communications perspective. It is inherently broadband and compatible with standard telecom infrastructures. Moreover, in CV, entanglement, one of the fundamental resource of quantum optics, can be generated deterministically. One of the main challenges for all quantum information technologies is scalability, being able to generate and manipulate a large number of quantum resources to achieve practical tasks efficiently. One approach to solve the issue of scalability is to use highly multimode quantum states. The quantum description of the electromagnetic field associate each photon (particle of light) with a mode (way for light to propagate). In a mutlimodal approach, we look at the quantum state bases and optical modes bases conjointly and tailor quantum fields not only in given modes, but also optimize the spatio-temporal shapes of the modes in which the state is defined. This opens wide perspectives for treating complex quantum states. In particular, using ultra-fast pulses of light which contain many temporal/spectral modes, we are able to generate large and complex entangled states of light using simple resources. In this thesis, we used an optical parametric oscillator pumped synchronously (SPOPO) with a frequency comb to generate multimode squeezed vacuum states which can be used to form cluster states: a large collection of modes (the nodes) entangled to each other in a certain way. These state are the basic resource for Measurement Based Quantum Computation (MBQC). This set-up has the advantage to generate entanglement in many mode with a single device. It is also highly tunable. Indeed, by tuning the spectrum of the OPO pump with a pulse shaper, one can tailor the properties of the generated quantum state. In this work, we focus on the optimization of the pump spectral shape to generate specific states. Using simulations based on Machine Learning Algorithms (MLA), we find optimal pump profile for typical target states. We then implement those shapes on the experimental set-up and measure the resulting states using multipixel homodyne detection. We also study intra-cavity dispersion effects. Dispersion inside the SPOPO cavity is indeed one of the main factor that limits the number of entangled modes in the generated quantum states. A systematic study of dispersion effects is therefore necessary to model the SPOPO output accurately. This works paves the way toward a fully tunable device that can be optimized in real time to generate specific quantum resources tailored for specific tasks.
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables, for example, in cluster state computation. We report in this Letter the first experimental evidence of a multimode nonclassical frequency comb in a femtosecond synchronously pumped optical parametric oscillator. In addition to a global reduction of its quantum intensity fluctuations, the system features quantum correlations between different parts of its frequency spectrum. This allows us to show that the frequency comb is composed of several uncorrelated eigenmodes having specific spectral shapes, two of them at least being squeezed, and to characterize their spectral shapes.
Squeezed states are a versatile class of quantum states with applications ranging from quantum computing to high-precision detection. We propose a method for generating tunable squeezed vacuum states of light with multiple modes encoded in frequency bins. Our method uses custom-engineered spontaneous parametric down-conversion pumped by a pulse-shaped pump field. The multimode squeezed states are generated in a single pass and can be tuned in real time by adjusting the properties of the pump field. Exploring new quantum states of light, encoded in new degrees of freedom, can be a fruitful path toward discovering new quantum applications.
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables [1]. They can be generated either by mixing different squeezed light sources using linear optical operations [2], or directly in a multimode optical device [3, 4]. Synchronously Pumped Optical Parametric Oscillators (SPOPO) — which correspond to an OPO pumped by a train of ultrashort pulses that are synchronized with the cavity round-trip time — have been theoretically shown to be promising devices for the generation of multimode nonclassical frequency combs, since a SPOPO is a sole optical cavity acting as an assembly of independent squeezers in a particular basis called the supermodes basis [5]. The supermodes are optical frequency combs with specific spectrum and phase profiles that are determined by the length of the intracavity nonlinear crystal and the pulse shape of the pump.
Continuous-variable quantum networks constitute a valuable resource for a wide range of quantum communication and information protocols. While frequency- and fast time-multiplexing enable the implementation of scalable quantum architectures, a precise characterization of multimode squeezed-light sources is essential. In this work, we increase both the spectral resolution and the measured squeezing values. Both parameters are relevant for the improved generation of so-called cluster states, a key resource for measurement-based quantum computing. Our source is based on parametric down-conversion in a periodically poled KTP waveguide pumped by a pulsed laser. The source produces squeezed states over a specific set of optical spectra. Increased spectral resolution in spectrally resolved homodyne detection allowed us to enhance the squeezing per spectral mode, increasing it from 1 dB to more than 2.4 dB in the first mode when measuring with a homodyne detector with a bandwidth of a few MHz. Secondly, we implemented a pulse-by-pulse characterization of the resource using a fast homodyne detector with an electronic bandwidth on the order of the laser repetition rate (100 MHz). Using this approach, the fast measurements revealed squeezing values of up to 1.5 dB in the first few spectral modes. To fully access the multimode quantum resource and ultimately improve the amount of squeezing, a high quantum efficiency is required. To avoid limitations imposed by poor spatial mode matching between the quantum resource and the local oscillator in homodyne detection, we implemented a wavefront-shaping scheme to characterize and control both the intensity profile and phase of the local oscillator. In preliminary tests this approach increased the mode-matching between the reference beam and the quantum signal by more than 8% while simultaneously providing a detailed characterization of the beam shape and of the influence of waveguide transmission on the beam profile. To achieve a genuine advantage in quantum information processing over classical protocols, the generation of non-Gaussian states is necessary. We therefore present a complete scheme for the creation of non-Gaussian states in a multimode system via mode-selective single-photon addition and subtraction, implemented through nonlinear optical processes in second-order nonlinear materials. We introduce a simulation framework applied to our squeezing source, which can be adapted to other regimes as well. Based on this framework, we are able to predict specific waveguide configurations that enable full control over the generated quantum states while maintaining high purity, with each process exhibiting a Schmidt number close to K=1, corresponding to effective single-mode addressing. generated quantum states while maintaining high purity, with each process exhibiting a Schmidt number close to K=1, corresponding to effective single-mode addressing.
Multimode bright squeezed vacuum is a non-classical state of light hosting a macroscopic photon number while offering promising capacity for encoding quantum information in its spectral degree of freedom. Here, we employ an accurate model for parametric down-conversion in the high-gain regime and use nonlinear holography to design quantum correlations of bright squeezed vacuum in the frequency domain. We propose the design of quantum correlations over two-dimensional lattice geometries that are all-optically controlled, paving the way toward continuous-variable cluster state generation on an ultrafast timescale. Specifically, we investigate the generation of a square cluster state in the frequency domain and calculate its covariance matrix and the quantum nullifier uncertainties, that exhibit squeezing below the vacuum noise level.