Abstract In the field of quantum metrology and sensing, a collection of quantum systems (e.g., spins) are used as a probe to estimate some physical parameter (e.g., magnetic field). It is usually assumed that there are no interactions between the probe systems. We show that strong interactions between them can increase robustness against thermal noise, leading to enhanced sensitivity. In principle, the sensitivity can scale exponentially in the number of probes—even at non-zero temperatures—if there are long-range interactions. This scheme can also be combined with other techniques, such as dynamical decoupling, to give enhanced sensitivity in realistic experiments.
Abstract In the field of quantum metrology and sensing, a collection of quantum systems (e.g., spins) are used as a probe to estimate some physical parameter (e.g., magnetic field). It is usually assumed that there are no interactions between the probe systems. We show that strong interactions between them can increase robustness against thermal noise, leading to enhanced sensitivity. In principle, the sensitivity can scale exponentially in the number of probes—even at non-zero temperatures—if there are long-range interactions. This scheme can also be combined with other techniques, such as dynamical decoupling, to give enhanced sensitivity in realistic experiments.
Quantum sensing utilizes the quantum resources of well-controlled quantum systems to measure small signals with high sensitivity, and has great potential in both fundamental science and concrete applications. Interacting quantum systems have attracted increasing interest in the field of precise measurements, owing to their potential to generate quantum-correlated states and exhibit rich many-body dynamics. These features provide a novel avenue for exploiting quantum resources in sensing applications. Although previous studies have shown that using such systems can improve sensitivity, they mainly focused on measuring individual physical quantities. In experiment, the challenge of using interacting quantum systems to achieve high-precision measurements of multiple physical parameters simultaneously has not been explored to a large extent. In this study, we demonstrate a first realisation of interaction-based multiparameter sensing by using strongly interacting nuclear spins under ultra-low magnetic field conditions. We find that, as the interaction strength among nuclear spins becomes significantly larger than their Larmor frequencies, a different regime emerges where the strongly interacting spins can be simultaneously sensitive to all components of a multidimensional field, such as a three-dimensional magnetic field. Moreover, we observe that the strong interactions between nuclear spins can increase their quantum coherence times to as long as several seconds, thereby improving measurement precision. Our sensor successfully achieves precision measurement of three-dimensional vector magnetic fields with a field sensitivity reaching the order of 10–11 T and an angular resolution as high as 0.2 rad. Importantly, this approach eliminates the need for external reference fields, thereby avoiding calibration errors and technical noise commonly encountered in traditional magnetometry. Experimentally optimized protocol further enhances the sensitivity of the interacting spin-based sensor by up to five orders of magnitude compared with non-interacting or classical schemes. These results demonstrate the enormous potential of interacting spin systems as a powerful platform for high-precision multi-parameter quantum sensing. The techniques developed here pave the way for a new generation of quantum sensors that use intrinsic spin interactions to exceed the traditional sensitivity limits, presenting a promising route toward ultra-sensitive, calibration-free magnetometry in complex environments.
Quantum metrology is a powerful tool for explorations of fundamental physical phenomena and applications in material science and biochemical analysis. While in principle the sensitivity can be improved by increasing the density of sensing particles, in practice this improvement is severely hindered by interactions between them. Here, using a dense ensemble of interacting electronic spins in diamond, we demonstrate a novel approach to quantum metrology to surpass such limitations. It is based on a new method of robust quantum control, which allows us to simultaneously suppress the undesired effects associated with spin-spin interactions, disorder, and control imperfections, enabling a fivefold enhancement in coherence time compared to state-of-the-art control sequences. Combined with optimal spin state initialization and readout directions, this allows us to achieve an ac magnetic field sensitivity well beyond the previous limit imposed by interactions, opening a new regime of high-sensitivity solid-state ensemble magnetometers.
Interacting quantum systems are attracting increasing interest for developing precise metrology. In particular, the realisation that quantum-correlated states and the dynamics of interacting systems can lead to entirely new and unexpected phenomena have initiated an intense research effort to explore interaction-based metrology both theoretically and experimentally. However, the current framework of interaction-based metrology mainly focuses on single-parameter estimations, a demonstration of multiparameter metrology using interactions as a resource was heretofore lacking. Here we demonstrate an interaction-based multiparameter metrology with strongly interacting nuclear spins. We show that the interacting spins become intrinsically sensitive to all components of a multidimensional field when their interactions are significantly larger than their Larmor frequencies. Using liquid-state molecules containing strongly interacting nuclear spins, we demonstrate the proof-of-principle estimation of all three components of an unknown magnetic field and inertial rotation. In contrast to existing approaches, the present interaction-based multiparameter sensing does not require external reference fields and opens a path to develop an entirely new class of multiparameter quantum sensors.
We study the effect of temperature on the ability of a qubit probe to distinguish between different phases in strongly correlated systems. Now to this end, we investigate a spin-1/2 Heisenberg XXZ chain coupled to a qubit probe via a pure dephasing interaction. At zero temperature, as reported previously, the decoherence dynamics exhibit different behavior in the gapped and gapless phases of the chain, with characteristic strong oscillations in the gapped phase and monotonic decay in the gapless phase. These oscillations decay much more slowly than expected with rising temperature in the gapped phase and their remnants are still visible at infinite temperature. In the gapless phase at low temperatures, using Luttinger liquid theory, we predict that the coherence exhibits asymptotic exponential decay in time, with the decay rate sensitive to the sign of the anisotropy parameter. We conclude that probe dynamics continue to carry information about the chain even at finite, reasonably small temperatures, positioning qubit probes as sensitive and robust detectors for quantum phases of correlated spin systems.
The typical bound on parameter estimation, known as the standard quantum limit (SQL), can be surpassed by exploiting quantum resources such as entanglement. To estimate the magnetic probe field, we propose a quantum sensor based on a variable-range many-body quantum spin chain with a moderate transverse magnetic field. We report the threefold benefits of employing a long-range system as a quantum sensor. First, sensors with quasi-long-range interactions can always beat the SQL for all values of the coordination number, while a sensor with long-range interactions does not have this ubiquitous quantum advantage. Second, a long-range Hamiltonian outperforms a nearest-neighbor (NN) Hamiltonian in terms of both estimating precision and system-size scaling. Finally, we observe that the system with long-range interactions can go below the SQL in the presence of a high temperature of the initial state, while sensors having NN interactions cannot. Furthermore, a sensor based on the long-range Ising Hamiltonian proves to be robust against impurities in the magnetic field and when the time-inhomogeneous dephasing noise acts during interaction of the probe with the system.
Dynamical decoupling techniques constitute an integral part of many quantum sensing platforms, often leading to orders-of-magnitude improvements in coherence time and sensitivity. Most ac sensing sequences involve a periodic echolike structure, in which the target signal is synchronized with the echo period. We show that for strongly interacting systems, this construction leads to a fundamental sensitivity limit associated with imperfect interaction decoupling. We present a simple physical picture demonstrating the origin of this limitation, and further formalize these considerations in terms of concise higher-order decoupling rules. We then show how these limitations can be surpassed by identifying a novel sequence building block, in which the signal period matches twice the echo period. Using these decoupling rules and the resulting sequence building block, we experimentally demonstrate significant improvements in dynamical decoupling timescales and magnetic field sensitivity, opening the door for new applications in quantum sensing and quantum many-body physics.