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arXiv:1709.05462 · Journal of Physics Conference Series

Quantum Scattering in an Optical Collider for Ultracold Atoms

Ryan Thomas, Matthew Chilcott, C. S. Chisholm, Amita B. Deb, Milena Horvath, Bianca J. Sawyer, Niels Kjærgaard

Published Nov 1, 2017• 7 citations
arXivHTMLPDF

Abstract

We report on experiments investigating the collisional properties of atoms at ultralow collision energies using an all-optical atom collider. By using a pair of optical tweezers, we can manipulate two ultracold atom clouds and collide them together at energies up to three orders of magnitude larger than their thermal energy. Our experiments measure the scattering of 87 Rb, 40 K, and 40 K- 87 Rb collisions. The versatility of our collider allows us to probe both shape resonances and Feshbach resonances in any partial wave. As examples, we present experiments demonstrating p-wave scattering with indistinguishable fermions, inelastic scattering at non-zero energies near a homonuclear Feshbach resonance, and partial wave interference in heteronuclear collisions.

DOI
10.1088/1742-6596/875/2/012007

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We report on experiments investigating the collisional properties of atoms at ultralow collision energies using an all-optical atom collider. By using a pair of optical tweezers, we can manipulate two ultracold atom clouds and collide them together at energies up to three orders of magnitude larger than their thermal energy. Our experiments measure the scattering of 87 Rb, 40 K, and 40 K- 87 Rb collisions. The versatility of our collider allows us to probe both shape resonances and Feshbach resonances in any partial wave. As examples, we present experiments demonstrating p-wave scattering with indistinguishable fermions, inelastic scattering at non-zero energies near a homonuclear Feshbach resonance, and partial wave interference in heteronuclear collisions.
Ultracold atomic gases have realized numerous paradigms of condensed matter physics, where control over interactions has crucially been afforded by tunable Feshbach resonances. So far, the characterization of these Feshbach resonances has almost exclusively relied on experiments in the threshold regime near zero energy. Here, we use a laser-based collider to probe a narrow magnetic Feshbach resonance of rubidium above threshold. By measuring the overall atomic loss from colliding clouds as a function of magnetic field, we track the energy-dependent resonance position. At higher energy, our collider scheme broadens the loss feature, making the identification of the narrow resonance challenging. However, we observe that the collisions give rise to shifts in the center-of-mass positions of outgoing clouds. The shifts cross zero at the resonance and this allows us to accurately determine its location well above threshold. Our inferred resonance positions are in excellent agreement with theory.Studies on energy-dependent scattering of ultracold atoms were previously carried out near zero collision energies. Here, the authors observe a magnetic Feshbach resonance in ultracold Rb collisions for above-threshold energies and their method can also be used to detect higher partial wave resonances.
This thesis describes experiments investigating the collisions of alkali metal atoms at energies between 10 - 2000 uK, measured in units of the Boltzmann constant. The atoms are accelerated towards each other using a purpose-built collider comprised of a crossed-beam optical dipole trap, which enables us to collide dense ensembles of ultracold atoms in any internal state at relatively high energies. I present the results of two experiments centered around resonant enhancement of the collisions. The first is between homonuclear 40K atoms near a shape resonance where the fermionic nature of the atoms determines the character of multiple scattering effects. The second experiment involves heteronuclear 40K87Rb collisions near a magnetically-tunable Feshbach resonance where we measure parameters describing the resonance as a function of collision energy. Theoretical models are developed that let us describe the collisions using published empirical interaction potentials, and we find good agreement between these models and the experiment.
In this thesis we explore ultracold atomic collisions in the vicinity of a magnetic Feshbach resonance located at 9.1 G, between 87Rb atoms in the |F = 2, mF = 1> and the |F =1, mF = 1> hyperfine states. We experimentally investigate the energy dependence of the enhancement of inelastic interaction in the neighborhood of this Feshbach resonance by analyzing the temperature dependence of a loss spectroscopy feature. An asymmetric widening of the resonance feature with respect to temperature is observed. We develop a simple model which captures these asymmetric line shapes through thermal averaging over the collision energy dependence of the Feshbach resonance. The energy dependence of the Feshbach interactions is further explored by colliding ultracold atomic samples at a fixed energy significantly above threshold using an optical trapping system; the elastic scattering enhancement analyzed by colliding the samples in free space, while for the inelastic measurements the collisions were carried out in trap. No conclusive resonant behavior could obtained for the elastic component of the 9.1 G resonance, however the inelastic scattering enhancement exhibited an anticipated shift.
Abstract Ultracold atomic gases have realized numerous paradigms of condensed matter physics, where control over interactions has crucially been afforded by tunable Feshbach resonances. So far, the characterization of these Feshbach resonances has almost exclusively relied on experiments in the threshold regime near zero energy. Here, we use a laser-based collider to probe a narrow magnetic Feshbach resonance of rubidium above threshold. By measuring the overall atomic loss from colliding clouds as a function of magnetic field, we track the energy-dependent resonance position. At higher energy, our collider scheme broadens the loss feature, making the identification of the narrow resonance challenging. However, we observe that the collisions give rise to shifts in the center-of-mass positions of outgoing clouds. The shifts cross zero at the resonance and this allows us to accurately determine its location well above threshold. Our inferred resonance positions are in excellent agreement with theory.
We describe an implementation of a magnetic collider for investigating cold collisions between ultracold atomic clouds in different spin states, and we use this to study scattering involving both even- and odd-order partial waves. Our method relies on the axial asymmetry of a double-well magnetic trap to selectively prepare the spin state in each cloud. We measure the energy dependence of sss, ppp, and ddd partial-wave phase shifts in collisions up to $300\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{K}$ between 87Rb^{87}\mathrm{Rb}87Rb atoms in the $5{S}_{1∕2},F=1,{m}_{F}=\ensuremath{-}1$ and 5S1∕2,F=2,mF=15{S}_{1∕2},F=2,{m}_{F}=15S1∕2​,F=2,mF​=1 states.
The inherent polarization gradients in tight optical tweezers can be used to couple the atomic spins to the two-body motion under the action of a microwave spin-flip transition, so that such a spin-motion coupling offers an important control knob on the motional states of optically trapped two colliding atoms. Here, after preparing two elastically scattering 85Rb^{85}\mathrm{Rb}85Rb atoms in the three-dimensional ground-state in the optical tweezer, we employed this control in order to probe the colliding energies of elastic and inelastic channels. The combination of microwave spectra and corresponding s-wave pseudopotential model allows us to infer the effect of the state-dependent trapping potentials on the elastic colliding energies, as well as to reveal how the presence of inelastic interactions affects elastic part of the relative potential. Our work shows that the spin-motion coupling in a tight optical tweezer expand the experimental toolbox for fundamental studies of ultracold collisions in the two body systems with reactive collisions, and potentially for that of more complex interactions, such as optically trapped atom-molecule and molecule-molecule interactions.