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arXiv:1709.04837 · Optica

Extended Wiener–Khinchin theorem for quantum spectral analysis

Rui‐Bo Jin, Ryōsuke Shimizu

Published Jan 23, 2018• 56 citations
arXivHTMLPDF

Abstract

The classical Wiener-Khinchin theorem (WKT), which can extract spectral information by classical interferometers through Fourier transform, is a fundamental theorem used in many disciplines. However, there is still need for a quantum version of WKT, which could connect correlated biphoton spectral information by quantum interferometers. Here, we extend the classical WKT to its quantum counterpart, i.e., extended WKT (e-WKT), which is based on two-photon quantum interferometry. According to the e-WKT, the difference-frequency distribution of the biphoton wavefunctions can be extracted by applying a Fourier transform on the time-domain Hong-Ou-Mandel interference (HOMI) patterns, while the sum-frequency distribution can be extracted by applying a Fourier transform on the time-domain NOON state interference (NOONI) patterns. We also experimentally verified the WKT and e-WKT in a Mach-Zehnder interference (MZI), a HOMI and a NOONI. This theorem can be directly applied to quantum spectroscopy, where the spectral correlation information of biphotons can be obtained from time-domain quantum interferences by Fourier transform. This may open a new pathway for the study of light-matter interaction at the single photon level.

DOI
10.1364/optica.5.000093

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The classical Wiener-Khinchin theorem (WKT), which can extract spectral information by classical interferometers through Fourier transform, is a fundamental theorem used in many disciplines. However, there is still need for a quantum version of WKT, which could connect correlated biphoton spectral information by quantum interferometers. Here, we extend the classical WKT to its quantum counterpart, i.e., extended WKT (e-WKT), which is based on two-photon quantum interferometry. According to the e-WKT, the difference-frequency distribution of the biphoton wavefunctions can be extracted by applying a Fourier transform on the time-domain Hong-Ou-Mandel interference (HOMI) patterns, while the sum-frequency distribution can be extracted by applying a Fourier transform on the time-domain NOON state interference (NOONI) patterns. We also experimentally verified the WKT and e-WKT in a Mach-Zehnder interference (MZI), a HOMI and a NOONI. This theorem can be directly applied to quantum spectroscopy, where the spectral correlation information of biphotons can be obtained from time-domain quantum interferences by Fourier transform. This may open a new pathway for the study of light-matter interaction at the single photon level.
The Wiener-Khinchin theorem, the fact that the autocorrelation function of a time process has a spectral decomposition given by its power-spectrum intensity, can be used in many disciplines. However, the applications based on a quantum counterpart of the Wiener-Khinchin theorem that provides a translation between time-energy degrees of freedom of biphoton wave function still remains relatively unexplored. Here, we use a quantum Wiener-Khinchin theorem (QWKT) to state that two-photon joint spectral intensity and the cross-correlation of two-photon temporal signal can be connected by making a Fourier transform. The mathematically defined QWKT is experimentally demonstrated in frequency-entangled two-photon Hong-Ou-Mandel (HOM) interference with the assistance of spectrally resolved detection. We apply this method to spectral-domain quantum optical coherence tomography that detects thickness-induced optical delays in a transparent sample, and show that our method suffices to achieve great advantages in measurement precision within a wide dynamic range and capturing time over the conventional HOM interferometric schemes. These results may significantly facilitate the use of QWKT for quantum information processing and quantum interferometric spectroscopy.
We propose theoretically a quantum interferometer in which the NOON state interferometer is combined with the Hong-Ou-Mandel interferometer. With this interferometer, the temporal interference patterns associated with biphoton frequency sum and difference can be shown in different parts of a single interferogram. It is thus possible to simultaneously obtain the spectral correlation information of biphotons in both frequency sum and difference by taking the Fourier transform from such an interferogram. This provides a method for complete spectral characterization of an arbitrary two-photon state with exchange symmetry and might be useful in quantum Fourier-transform spectroscopy where direct spectral measurement is difficult. Furthermore, as it can realize the measurement of time intervals on three scales at the same time, we expect that it can provide a method in quantum metrology. Finally, we discuss another potential application of such an interferometer in the generation and characterization of high-dimensional and phase-controlled frequency entanglement.
Fourier transform spectroscopy with classical interferometry corresponds to the measurement of a single-photon intensity spectrum from the viewpoint of the particle nature of light. In contrast, the Fourier transform of two-photon quantum interference patterns provides the intensity spectrum of the two photons as a function of the sum or difference frequency of the constituent photons. This unique feature of quantum interferometric spectroscopy offers a different type of spectral information from the classical measurement and may prove useful for nonlinear spectroscopy with two-photon emission. Here, we report the first experimental demonstration of two-photon quantum interference of photon pairs emitted via biexcitons in the semiconductor CuCl. Besides applying Fourier transform to quantum interference patterns, we reconstruct the intensity spectrum of the biexciton luminescence in the two-photon sum or difference frequency. We discuss the connection between the reconstructed spectra and exciton states in CuCl as well as the capability of quantum interferometry in solid-state spectroscopy.
Fourier transform spectroscopy with classical interferometry corresponds to the measurement of a single-photon intensity spectrum from the viewpoint of the particle nature of light. In contrast, the Fourier transform of two-photon quantum interference patterns provides the intensity spectrum of the two photons as a function of the sum- or difference frequency of the constituent photons. This unique feature of quantum interferometric spectroscopy offers a different type of spectral information from the classical measurement and may prove useful for nonlinear spectroscopy with two-photon emission. Here, we report the experimental demonstration of two-photon quantum interference of biphotons emitted via biexcitons in the semiconductor CuCl. Besides applying Fourier transform to quantum interference patterns, we reconstruct the intensity spectrum of the biexciton luminescence in the two-photon sum- or difference frequency. We discuss the connection between the reconstructed spectra and exciton states in CuCl as well as the capability of quantum interferometry in solid-state spectroscopy.
The paper proposes a spectral-domain version of a biphoton (Hong–Ou–Mandel) interferometry. The operation principle is based on measuring the coincidence rate of entangled photons while scanning the difference between their central frequencies. A theoretical apparatus describing the operation principle and the resolution limits of the proposed spectral-domain biphoton interferometry is developed. The analysis is based on quantum and classical Cramer–Rao bounds. It was shown that the proposed spectral-domain biphoton interferometry approach enables the mitigation of the fringe number counting errors, often encountered in classical spectral interferometry. A comparison with a conventional Hong–Ou–Mandel biphoton interferometry is also presented.