Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1709.03428 · Physical Review A

Coherent metamaterial absorption of two-photon states with 40% efficiency

Ashley Lyons, Dikla Oren, Thomas Roger, Vassili Savinov, João Valente, Stefano Vezzoli, Nikolay I. Zheludev, Mordechai Segev, Daniele Faccio

Published Jan 14, 2019• 41 citations
arXivHTMLPDF

Abstract

Multiphoton absorption processes have a nonlinear dependence on the amplitude of the incident optical field, i.e., the number of photons. However, multiphoton absorption is generally weak and multiphoton events occur with extremely low probability. Consequently, it is extremely challenging to engineer quantum nonlinear devices that operate at the single photon level and the majority of quantum technologies have to rely on single photon interactions. Here we demonstrate experimentally and theoretically that exploiting coherent absorption of $N=2$ NOON states makes it possible to enhance the number of two-photon states that are absorbed by at most a factor of 2 with respect to a linear absorption process. An absorbing metasurface placed inside a Sagnac-style interferometer into which we inject an $N=2$ NOON state, exhibits two-photon absorption with $40.5%$ efficiency, close to the theoretical maximum. This high probability of simultaneous absorption of two photons holds the promise for applications in fields that require multiphoton upconversion but are hindered by high peak intensities.

DOI
10.1103/physreva.99.011801

Related papers

Coherent absorption of two-photon states in metamaterials

Thomas Roger, Ashley Lyons, Dikla Oren +6 more

Multiple photon absorption processes typically have a nonlinear dependence on the amplitude of the incident optical field. On the other hand, quantum technologies rely on single photon events. It has therefore been of great technical difficulty to achieve nonlinear devices using single photons. This is due to the small cross-section of absorption in room temperature devices, with multi-photon absorption events occurring with extremely low probability. The lack of access to nonlinear processes severely inhibits the use of optics for a large number of applications surrounding quantum technologies. We demonstrate experimentally that by exploiting a coherent absorption mechanism for N=2 N00N states, outlined theoretically by Jeffers in 2000 [1] and experimentally explored by Roger et. al. in 2016 [2], that it is possible to determine and enhance the number of two photon states that are absorbed. Here a 50% absorbing metasurface is placed inside a Sagnac interferometer into which we inject a N00N state. We show that by tuning the phase φ of the input state, |2,0〉 + exp(-ί2φ) |0,2〉, we can selectively tune the output state. For an input phase of φ = π/2 or 3π/2 we find that a single photon is absorbed with 100% probability. However, when we tune the input phase to φ = 0 or π we see that either 0 or 2 photons are absorbed with equal probability. We have developed a theoretical model that, with no free parameters, fits the experimentally measured two-photon contribution and finds the maximum contribution of |0,0) (0,0| to the output state to be 40.5%.

Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)•Jun 1, 2017•0 citations

Non-Hermitian Quantum Nonlinear Optics with Single Photons

Samuel Napoli, Andrea Zappalá, Franco Nori +2 more

Quantum nonlinear optics seeks to harness strong photon-photon interactions for scalable quantum technologies, although dissipative losses still pose a major barrier to near-unity conversion efficiency. Here, we bridge non-Hermitian physics with the quantum nonlinear domain by exploiting perfect absorption to identify and optimize few-photon nonlinear processes. We theoretically investigate two circuit QED systems, operating in the light-matter ultrastrong coupling regime. The first (i) enables simultaneous two-atom excitations by single photons, while the second (ii) realizes the strong coupling between a single-photon and a two-photon Fock states. We demonstrate that, since the strong optical nonlinearities cause quantum spectral features to emerge already at the level of linear response theory, the perfect absorption condition in $|S_{11}|$ enables near-deterministic single-photon down-conversion into (i) a qubit-qubit-correlated pair and (ii) a two-photon pair. We show that the conversion efficiency can be systematically optimized through experimentally accessible parameters, both linked to the emergence of Hermitian subspaces within the effective non-Hermitian Hamiltonians. These findings position non-Hermitian engineering as a broadly applicable route to optimizing quantum devices at the single-photon level, even beyond circuit-QED platforms.

quant-pharXiv:2607.29313•Aug 3, 2026•0 citations

Nonlinear Interferometry for Quantum-Enhanced Measurements of Multiphoton Absorption

S. Panahiyan, Carlos Sánchez Muñoz, Maria V. Chekhova +1 more

Multiphoton absorption is of vital importance in many spectroscopic, microscopic, or lithographic applications. However, given that it is an inherently weak process, the detection of multiphoton absorption signals typically requires large field intensities, hindering its applicability in many practical situations. In this Letter, we show that placing a multiphoton absorbent inside an imbalanced nonlinear interferometer can enhance the precision of multiphoton cross section estimation with respect to strategies based on photon-number measurements using coherent or even squeezed light directly transmitted through the medium. In particular, the power scaling of the sensitivity with photon flux can be increased by 1 order compared with transmission measurements of the sample with coherent light, such that the measurement precision at any given intensity can be greatly enhanced. Furthermore, we show that this enhanced measurement precision is robust against experimental imperfections leading to photon losses, which usually tend to degrade the detection sensitivity. We trace the origin of this enhancement to an optimal degree of squeezing which has to be generated in a nonlinear SU(1,1) interferometer.

arXiv:2209.02697•Physical Review Letters•May 19, 2023•22 citations

Quantum Metasurfaces for Enhancement of Reverse Saturable Absorption

Ioannis Katsantonis, Maria Kafesaki

Reverse saturable absorption (RSA) occurs in nonlinear materials where the excited state exhibits higher absorption than the ground state. This study presents a full-wave spatio-temporal numerical model that accurately simulates coherent RSA by coupling quantum systems with Maxwell’s equations. The model enables the design of complex photonic metamaterials and metasurfaces beyond the capabilities of conventional absorption models. To demonstrate its effectiveness, we analyze a metasurface-enhanced optical absorber, achieving over twice the absorption enhancement compare to the bare layer. This approach paves the way for highly efficient low-power optical absorption devices, with applications in protective optics and photonic elements.

International Congress on Artificial Materials for Novel Wave Phenomena (Metamaterials)•Sep 1, 2025•0 citations

Integrable high-efficiency generation of three-photon entangled states by a single incident photon

Yunning Lu, Zeyang Liao, Fuli Li +1 more

Generation of multi-photon entangled states with high efficiency in integrated photonic quantum systems is still a big challenge. The usual three-photon generation efficiency based on the third-order nonlinear effect is extremely low. Here, we propose a scheme to generate three-photon correlated states, which are entangled states in frequency space and bound states in real space, with high efficiency. This method relies on two crucial processes. On one hand, by employing a Sagnac interferometer, an incident photon can be transformed into a symmetric superposition of the clockwise and counterclockwise modes of the Sagnac loop, which can then be perfectly absorbed by the emitter. On the other hand, the coupling strengths of the two transition paths of the emitter to the Sagnac loop are set to be equal, under which the absorbed photon can be emitted completely from the cascaded transition path due to quantum interference. By adjusting the coupling strengths among the three transition paths of the emitter and the waveguide modes, we can control the spectral entanglement and spatial separation among the three photons. Our proposal can be used to generate three-photon entangled states on demand, and the efficiency can be higher than 90% with some practical parameters, which can find important applications in integrated quantum information processing.

Photonics Research•Nov 30, 2021•8 citations

Coherent Absorption of N00N States

Thomas Roger, Sara Restuccia, Ashley Lyons +5 more

Recent results in deeply subwavelength thickness films demonstrate coherent control and logical gate operations with both classical and single-photon light sources. However, quantum processing and devices typically involve more than one photon and nontrivial input quantum states. Here we experimentally investigate two-photon N00N state coherent absorption in a multilayer graphene film. Depending on the N00N state input phase, it is possible to selectively choose between single- or two-photon absorption of the input state in the graphene film. These results demonstrate that coherent absorption in the quantum regime exhibits unique features, opening up applications in multiphoton spectroscopy and imaging.

arXiv:1603.04363•Physical Review Letters•Jul 6, 2016•64 citations
Multiphoton absorption processes have a nonlinear dependence on the amplitude of the incident optical field, i.e., the number of photons. However, multiphoton absorption is generally weak and multiphoton events occur with extremely low probability. Consequently, it is extremely challenging to engineer quantum nonlinear devices that operate at the single photon level and the majority of quantum technologies have to rely on single photon interactions. Here we demonstrate experimentally and theoretically that exploiting coherent absorption of N=2N=2N=2 NOON states makes it possible to enhance the number of two-photon states that are absorbed by at most a factor of 2 with respect to a linear absorption process. An absorbing metasurface placed inside a Sagnac-style interferometer into which we inject an N=2N=2N=2 NOON state, exhibits two-photon absorption with 40.540.5%40.5 efficiency, close to the theoretical maximum. This high probability of simultaneous absorption of two photons holds the promise for applications in fields that require multiphoton upconversion but are hindered by high peak intensities.
Multiple photon absorption processes typically have a nonlinear dependence on the amplitude of the incident optical field. On the other hand, quantum technologies rely on single photon events. It has therefore been of great technical difficulty to achieve nonlinear devices using single photons. This is due to the small cross-section of absorption in room temperature devices, with multi-photon absorption events occurring with extremely low probability. The lack of access to nonlinear processes severely inhibits the use of optics for a large number of applications surrounding quantum technologies. We demonstrate experimentally that by exploiting a coherent absorption mechanism for N=2 N00N states, outlined theoretically by Jeffers in 2000 [1] and experimentally explored by Roger et. al. in 2016 [2], that it is possible to determine and enhance the number of two photon states that are absorbed. Here a 50% absorbing metasurface is placed inside a Sagnac interferometer into which we inject a N00N state. We show that by tuning the phase φ of the input state, |2,0〉 + exp(-ί2φ) |0,2〉, we can selectively tune the output state. For an input phase of φ = π/2 or 3π/2 we find that a single photon is absorbed with 100% probability. However, when we tune the input phase to φ = 0 or π we see that either 0 or 2 photons are absorbed with equal probability. We have developed a theoretical model that, with no free parameters, fits the experimentally measured two-photon contribution and finds the maximum contribution of |0,0) (0,0| to the output state to be 40.5%.
Quantum nonlinear optics seeks to harness strong photon-photon interactions for scalable quantum technologies, although dissipative losses still pose a major barrier to near-unity conversion efficiency. Here, we bridge non-Hermitian physics with the quantum nonlinear domain by exploiting perfect absorption to identify and optimize few-photon nonlinear processes. We theoretically investigate two circuit QED systems, operating in the light-matter ultrastrong coupling regime. The first (i) enables simultaneous two-atom excitations by single photons, while the second (ii) realizes the strong coupling between a single-photon and a two-photon Fock states. We demonstrate that, since the strong optical nonlinearities cause quantum spectral features to emerge already at the level of linear response theory, the perfect absorption condition in ∣S11∣|S_{11}|∣S11​∣ enables near-deterministic single-photon down-conversion into (i) a qubit-qubit-correlated pair and (ii) a two-photon pair. We show that the conversion efficiency can be systematically optimized through experimentally accessible parameters, both linked to the emergence of Hermitian subspaces within the effective non-Hermitian Hamiltonians. These findings position non-Hermitian engineering as a broadly applicable route to optimizing quantum devices at the single-photon level, even beyond circuit-QED platforms.
Multiphoton absorption is of vital importance in many spectroscopic, microscopic, or lithographic applications. However, given that it is an inherently weak process, the detection of multiphoton absorption signals typically requires large field intensities, hindering its applicability in many practical situations. In this Letter, we show that placing a multiphoton absorbent inside an imbalanced nonlinear interferometer can enhance the precision of multiphoton cross section estimation with respect to strategies based on photon-number measurements using coherent or even squeezed light directly transmitted through the medium. In particular, the power scaling of the sensitivity with photon flux can be increased by 1 order compared with transmission measurements of the sample with coherent light, such that the measurement precision at any given intensity can be greatly enhanced. Furthermore, we show that this enhanced measurement precision is robust against experimental imperfections leading to photon losses, which usually tend to degrade the detection sensitivity. We trace the origin of this enhancement to an optimal degree of squeezing which has to be generated in a nonlinear SU(1,1) interferometer.
Reverse saturable absorption (RSA) occurs in nonlinear materials where the excited state exhibits higher absorption than the ground state. This study presents a full-wave spatio-temporal numerical model that accurately simulates coherent RSA by coupling quantum systems with Maxwell’s equations. The model enables the design of complex photonic metamaterials and metasurfaces beyond the capabilities of conventional absorption models. To demonstrate its effectiveness, we analyze a metasurface-enhanced optical absorber, achieving over twice the absorption enhancement compare to the bare layer. This approach paves the way for highly efficient low-power optical absorption devices, with applications in protective optics and photonic elements.
Generation of multi-photon entangled states with high efficiency in integrated photonic quantum systems is still a big challenge. The usual three-photon generation efficiency based on the third-order nonlinear effect is extremely low. Here, we propose a scheme to generate three-photon correlated states, which are entangled states in frequency space and bound states in real space, with high efficiency. This method relies on two crucial processes. On one hand, by employing a Sagnac interferometer, an incident photon can be transformed into a symmetric superposition of the clockwise and counterclockwise modes of the Sagnac loop, which can then be perfectly absorbed by the emitter. On the other hand, the coupling strengths of the two transition paths of the emitter to the Sagnac loop are set to be equal, under which the absorbed photon can be emitted completely from the cascaded transition path due to quantum interference. By adjusting the coupling strengths among the three transition paths of the emitter and the waveguide modes, we can control the spectral entanglement and spatial separation among the three photons. Our proposal can be used to generate three-photon entangled states on demand, and the efficiency can be higher than 90% with some practical parameters, which can find important applications in integrated quantum information processing.
Recent results in deeply subwavelength thickness films demonstrate coherent control and logical gate operations with both classical and single-photon light sources. However, quantum processing and devices typically involve more than one photon and nontrivial input quantum states. Here we experimentally investigate two-photon N00N state coherent absorption in a multilayer graphene film. Depending on the N00N state input phase, it is possible to selectively choose between single- or two-photon absorption of the input state in the graphene film. These results demonstrate that coherent absorption in the quantum regime exhibits unique features, opening up applications in multiphoton spectroscopy and imaging.