The Leggett-Garg inequalities serve to test whether or not quantum correlations in time can be explained within a classical macrorealistic framework. We apply this test to thermodynamics and derive a set of Leggett-Garg inequalities for the statistics of fluctuating work done on a quantum system unitarily driven in time. It is shown that these inequalities can be violated in a driven two-level system, thereby demonstrating that there exists no general macrorealistic description of quantum work. These violations are shown to emerge within the standard Two-Projective-Measurement scheme as well as for alternative definitions of fluctuating work that are based on weak measurement. Our results elucidate the influences of temporal correlations on work extraction in the quantum regime and highlight a key difference between quantum and classical thermodynamics.
The Leggett-Garg inequalities serve to test whether or not quantum correlations in time can be explained within a classical macrorealistic framework. We apply this test to thermodynamics and derive a set of Leggett-Garg inequalities for the statistics of fluctuating work done on a quantum system unitarily driven in time. It is shown that these inequalities can be violated in a driven two-level system, thereby demonstrating that there exists no general macrorealistic description of quantum work. These violations are shown to emerge within the standard Two-Projective-Measurement scheme as well as for alternative definitions of fluctuating work that are based on weak measurement. Our results elucidate the influences of temporal correlations on work extraction in the quantum regime and highlight a key difference between quantum and classical thermodynamics.
Macrorealistic description governing the classical realm is known to get uprooted in the quantum domain. The Leggett-Garg inequality [A. J. Leggett and A. Garg, Phys. Rev. Lett. 54, 857 (1985)] proposes to probe the macrorealistic limit emerging from the quantum scenario. It places a bound on the linear combinations of temporal correlations of observables measured sequentially at different time intervals. Violation of the Leggett-Garg inequality, up to the so-called temporal Tsirelson bound (TTB), has been realized in the quantum domain. It is important to understand whether quantum theory permits larger violation beyond the TTB and up to the algebraic maximum value of the Leggett-Garg inequality. To this end, it has been shown [C. Budroni and C. Emary, Phys. Rev. Lett. 113, 050401 (2014)] that a three-term Leggett-Garg inequality can be violated beyond the TTB 3/2 in the time evolution of N>2 level quantum systems by choosing suitable measurement schemes and state-update rules. Furthermore, it is revealed that the algebraic maximum value 3 can be realized in the limit $N\ensuremath{\rightarrow}\ensuremath{\infty}$. Their measurement scheme rules out violation of the Leggett-Garg inequality beyond the TTB by a qubit. Being genuinely quantum in nature, we ask whether such enhanced violation of the Leggett-Garg inequality could be witnessed in a qubit itself. Here, we show that a qubit undergoing time evolution generated by a non-Hermitian PT-symmetric Hamiltonian indeed violates the three-term Leggett-Garg inequality beyond the TTB and up to its algebraic maximum value 3.
We study the fluctuations of the work performed on a driven quantum system, defined as the difference between subsequent measurements of energy eigenvalues. These work fluctuations are governed by statistical theorems with similar expressions in classical and quantum physics. We show that we can distinguish quantum and classical work fluctuations, as the latter can be described by a macrorealistic theory and hence obey Leggett-Garg inequalities. We show that these inequalities are violated by quantum processes in a driven two-level system and in a harmonic oscillator subject to a squeezing transformation.
Nonclassicality of temporal correlations pertaining to noncommutative sequential measurements is defined through the violation of macrorealistic inequalities, known as Leggett-Garg inequalities (LGI). We investigate the energy cost of the process associated with the Leggett-Garg test in the context of noiseless and Markovian noise for arbitrary initial states. We prove that in noiseless and in certain noisy scenarios, the maximal violations of LGI under the energy constraint occurs when the average energy of the process is equal to the negative of the energy of the initial state. Such a dependence of LGI on the choice of the initial state is not seen in the unconstrained case. Moreover, we find that in the presence of a moderate amount of Markovian noise, the amount of violation of LGI remains almost unaltered with a suitable choice of the evolution and dephasing operators in the neighborhood of the maximal violation line, thereby showing the robustness of temporal correlations under environmental effects.
I study several aspects of tests of macrorealism (MR), which for a given data set serves to give a quantitative signal of the presence of a specific notion of non-classical behaviour. The insufficiency of classical understanding underpins both the paradoxes of quantum mechanics, its future technological promise, and so these tests are of interest both foundationally and pragmatically. I derive generalisations of the Leggett-Garg (LG) inequalities and Fine's theorem, which together establish the necessary and sufficient conditions for macrorealism. First, I extend these conditions to tests involving an arbitrary number of measurement times. Secondly, I generalise them beyond the standard dichotomic variable, to systems described by many-valued variables. I also perform a quantum mechanical analysis examining the interplay of different conditions of MR. I then develop the theoretical framework to support tests of macrorealism in continuous variable systems, where I define variables based on coarse-grainings of position. I calculate temporal correlators for general bound systems, and analyse LG violations within the quantum harmonic oscillator (QHO), in its energy eigenstates and coherent states. I analyse the precise physical mechanisms underpinning the violations in terms of probability currents, Bohm trajectories. Staying within continuous variable systems, we outline a different approach to meeting the invasiveness requirement of LG tests. Reasoning that we may approximately non-invasively measure whether a particle crosses the axis, we measure an object which is related to the standard correlators, and derive a set of macrorealistic inequalities for these modified correlators. We demonstrate violations of these modified LG inequalities for several states within the QHO.
It remains an open question how a realist view of the macroscopic world emerges from a quantum formalism. For testing the macrorealism in the quantum domain, an interesting approach was put forward by Leggett and Garg in 1985, by formulating a suitable inequality valid for any macrorealistic theory. Recently, by following the Wigner idea of local realist inequality, a probabilistic version of standard Leggett-Garg inequalities has also been proposed. While the Wigner form of local realist inequalities is equivalent to the two-party, two-measurements and two-outcomes CHSH inequalities, in this paper we provide a generic proof to demonstrate that the Wigner form of Leggett-Garg inequalities is not only inequivalent to the standard ones, but also stronger than the latter. This is demonstrated by quantifying the amount of disturbance caused by a priori measurement to the subsequent measurements. In this connection, the relation between LGIs and another formulation of macrorealism known as no-signaling in time is examined.
In contrast to the spatial Bell's inequalities which probe entanglement between spatially separated systems, the Leggett–Garg inequalities test the correlations of a single system measured at different times. Violation of a genuine Leggett–Garg test implies either the absence of a realistic description of the system or the impossibility of measuring the system without disturbing it. Quantum mechanics violates the inequalities on both accounts and the original motivation for these inequalities was as a test for quantum coherence in macroscopic systems. The last few years has seen a number of experimental tests and violations of these inequalities in a variety of microscopic systems such as superconducting qubits, nuclear spins, and photons. In this article, we provide an introduction to the Leggett–Garg inequalities and review these latest experimental developments. We discuss important topics such as the significance of the non-invasive measurability assumption, the clumsiness loophole, and the role of weak measurements. Also covered are some recent theoretical proposals for the application of Leggett–Garg inequalities in quantum transport, quantum biology and nano-mechanical systems.