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arXiv:1708.01840

Quantum difference parametric amplification and oscillation

M. K. Olsen

Published Aug 6, 2017• 0 citations
arXivHTMLPDF

Abstract

A recent article [W.C.W. Huang and H. Batelaan, arXiv:1708.0057v1] analysed the dualism between optical and difference parametric amplification, performing a classical analysis of a system where two electromagnetic fields are produced by another of a frequency which is the difference of the frequency of the other two. The authors claimed that this process would not violate energy conservation at the classical level, but that a quantum description would necessarily require a non-Hermitian Hamiltonian and therefore would not exist. In this work we show that the process can proceed quantum mechanically if described by the correct Hamiltonian, that energy conservation is not violated, and that fields are produced with interesting quantum statistics. Furthermore, we show that the process can be thought of as different types of already known three-wave mixing processes, with the actual type depending on either initial conditions or personal preference.

DOI
10.48550/arxiv.1708.01840

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A recent article [W.C.W. Huang and H. Batelaan, arXiv:1708.0057v1] analysed the dualism between optical and difference parametric amplification, performing a classical analysis of a system where two electromagnetic fields are produced by another of a frequency which is the difference of the frequency of the other two. The authors claimed that this process would not violate energy conservation at the classical level, but that a quantum description would necessarily require a non-Hermitian Hamiltonian and therefore would not exist. In this work we show that the process can proceed quantum mechanically if described by the correct Hamiltonian, that energy conservation is not violated, and that fields are produced with interesting quantum statistics. Furthermore, we show that the process can be thought of as different types of already known three-wave mixing processes, with the actual type depending on either initial conditions or personal preference.
The amplification of electromagnetic fields is analyzed in a quantum-mechanical context by discussing the behavior of a simple theoretical model of the parametric amplifier. The statistical properties of the amplifier fields are described by means of the time-dependent density operator for the system. In doing this, extensive use is made of the coherent states and the PPP representation of the density operator, which provide a quantum-mechanical description of the fields closely resembling their classical description. Explicit solutions are obtained for the density operator for either of the two field modes for a variety of initial states of the modes. Initial states considered include combinations of coherent states, chaotic mixtures, and nnn-quantum states. Particular attention is given the behavior of the amplifier fields in the limit of large amplification. The conditions are established under which the amplification process leads in this limit to the existence of a non-negative PPP representation for the density operator for a single mode of oscillation.
A large number of "molecules," which are taken to be angular momentum oscillators of frequency $\ensuremath{\nu}$, are considered to interact through their dipole moment with two electromagnetic cavity modes of frequencies ${\ensuremath{\omega}}_{1}$ and ${\ensuremath{\omega}}_{2}$, respectively, where $\ensuremath{\nu}={\ensuremath{\omega}}_{1}\ifmmode\pm\else\textpm\fi{}{\ensuremath{\omega}}_{2}$. The behavior of the combined system is analyzed up to fourth order in perturbation theory. Phenomena known as two-photon emission or absorption, parametric amplification, various types of Raman emission, and frequency conversion are exhibited. The analytical method used is applicable to both a quantum-mechanical and a classical description of the modes and molecules; it displays explicitly the resulting differences. Expressions for the rate of energy change of the modes and molecules indicate resonance in second and fourth order. The second-order results are the same for the classical and quantum-mechanical treatments, while the fourth-order results show certain differences, which are examined in detail. The conditions under which each of the above phenomena occurs are discussed in a self-consistent manner, both classically and quantum-mechanically. It is shown that the second-order expression and the most significant part of the fourth-order expression can be derived very simply from a resonance interaction Hamiltonian that consists of a sum of products of three variables---two referring to the two modes, and the third to the molecules. The relationship between this resonance Hamiltonian and the fundamental dipole-moment Hamiltonian is examined, and the approximations by which the resonance Hamiltonian may be derived are considered. Arguments concerning the applicability of perturbation theory to steady-state situations are presented; it is pointed out that the second-order expressions for the energy transfer between molecules and field may be applicable to such a situation, in which case the classical and quantum-mechanical treatments are equivalent.
The description of the statistical dynamics of quantum oscillators is formulated in terms of the Wigner distribution, analogous to the more commonly used PPP distribution, with explicit formulas being obtained for its time evolution and for average values. This formulation is desirable because, e.g., the Wigner distribution always exists whereas the PPP distribution does not. The formalism is applied to the process of parametric amplification in a single mode, which may be considered as the degenerate form of the well-known two-mode case. This degeneracy gives rise to significantly different properties; for example, the PPP distribution for the single mode of interest evolves from a circularly symmetric two-dimensional Gaussian into an elliptically symmetric form and ceases to exist after a finite time, even for amplification in the presence of losses. This is contrary to the two-mode case. The corresponding Wigner distribution is found to exist as a well-behaved function for all time as expected, regardless of the amount of losses, and is used to calculate average values of various quantities of interest. It is found, e.g., that in the lossless case the average number of photons in the signal mode always becomes infinite as $t\ensuremath{\rightarrow}\ensuremath{\infty}$. This is in contrast to the corresponding classical result for the lossless case which allows the signal to decay rather than to grow with time, depending on the relative phase between the signal and the pump. Field fluctuations are discussed and found to have some unusual properties. The combination of frequency up-conversion with single-mode amplification is also described briefly. The effect of the quantization of the pump oscillator is considered in an Appendix.
Breaking the symmetry in a coupled wave system can result in unusual amplification behavior. In the case of difference parametric amplification the resonant pump frequency is equal to the difference, instead of the sum, frequency of the normal modes. We show that sign reversal in the symmetry relation of parametric coupling give rise to difference parametric amplification as a dual of optical parametric amplification. For optical systems, our result can potentially be used for efficient XUV amplification.
Recent proposed ``loophole-free'' Bell tests are discussed in the light of classical models for the relevant features of optical parametric amplification and homodyne detection. The Bell tests themselves are uncontroversial: there are no obvious loopholes that might cause bias and hence, if the world does, after all, obey local realism, no violation of a Bell inequality will be observed. Interest centres around the question of whether or not the proposed criterion for ``non-classical'' light is valid. If it is not, then the experiments will fail in their initial concept, since both quantum theorists and local realists will agree that we are seeing a purely classical effect. The Bell test, though, is not the only criterion by which the quantum-mechanical and local realist models can be judged. It is suggested that the quantum-mechanical models given in the proposals will also fail in their detailed predictions. If the experiments are extended by including a range of parameter values and by analysing, in addition to the proposed digitised voltage differences, the raw voltages, the models can be compared in their overall performance and plausibility.
A quantum theory of parametric amplification and frequency conversion of an optical image in coupled nonlinear optical processes that include one parametric amplification process at high-frequency pumping and two up-conversion processes in the same pump field is developed. The field momentum operator that takes into account the diffraction and group velocities of the waves is used to derive the quantum equations related to the spatial dynamics of the images during the interaction. An optical scheme for the amplification and conversion of a close image is considered. The mean photon number density and signal-to-noise ratio are calculated in the fixed-pump-field approximation for images at various frequencies. It has been established that the signal-to-noise ratio decreases with increasing interaction length in the amplified image and increases in the images at the generated frequencies, tending to asymptotic values for all interacting waves. The variance of the difference of the numbers of photons is calculated for various pairs of frequencies. The quantum entanglement of the optical images formed in a high-frequency pump field is shown to be converted to higher frequencies during the generation of sum frequencies. Thus, two pairs of entangled optical images are produced in the process considered.