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arXiv:1708.00906 · Scientific Reports

Ultrastrong coupling probed by Coherent Population Transfer

G. Falci, A. Ridolfo, P. G. Di Stefano, E. Paladino

Published Jun 25, 2019• 29 citations
arXivHTMLPDF

Abstract

Light-matter interaction, and the understanding of the fundamental physics behind, is the scenario of emerging quantum technologies. Solid state devices allow the exploration of new regimes where ultrastrong coupling strengths are comparable to subsystem energies, and new exotic phenomena like quantum phase transitions and ground-state entanglement occur. While experiments so far provided only spectroscopic evidence of ultrastrong coupling, we propose a new dynamical protocol for detecting virtual photon pairs in the dressed eigenstates. This is the fingerprint of the violated conservation of the number of excitations, which heralds the symmetry broken by ultrastrong coupling. We show that in flux-based superconducting architectures this photon production channel can be coherently amplified by Stimulated Raman Adiabatic Passage, providing a unique tool for an unambiguous dynamical detection of ultrastrong coupling in present day hardware. This protocol could be a benchmark for control of the dynamics of ultrastrong coupling architectures, in view of applications to quantum information and microwave quantum photonics.

DOI
10.1038/s41598-019-45187-y

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Light-matter interaction, and the understanding of the fundamental physics behind, is the scenario of emerging quantum technologies. Solid state devices allow the exploration of new regimes where ultrastrong coupling strengths are comparable to subsystem energies, and new exotic phenomena like quantum phase transitions and ground-state entanglement occur. While experiments so far provided only spectroscopic evidence of ultrastrong coupling, we propose a new dynamical protocol for detecting virtual photon pairs in the dressed eigenstates. This is the fingerprint of the violated conservation of the number of excitations, which heralds the symmetry broken by ultrastrong coupling. We show that in flux-based superconducting architectures this photon production channel can be coherently amplified by Stimulated Raman Adiabatic Passage, providing a unique tool for an unambiguous dynamical detection of ultrastrong coupling in present day hardware. This protocol could be a benchmark for control of the dynamics of ultrastrong coupling architectures, in view of applications to quantum information and microwave quantum photonics.
Light-matter interaction and understanding the fundamental physics behind is essential for emerging quantum technologies. Solid-state devices may explore new regimes where coupling strengths are “ultrastrong”, i.e., comparable to the energies of the subsystems. New exotic phenomena occur the common root of many of them being the fact that the entangled vacuum contains virtual photons. They herald the lack of conservation of the number of excitations which is the witness of ultrastrong coupling breaking the U(1) symmetry. Despite more than a decade of research, the detection of ground-state virtual photons still awaits demonstration. In this work, we recognize the “conspiring” set of experimental challenges show how to overcome them, thus providing a solution to this long-standing problem. We find that combining a superinductor-based unconventional “light fluxonium” qudit and coherent control yields a highly efficient, faithful, and selective conversion of virtual photons into real ones. This enables their detection with resources available to present-day quantum technologies. Published by the American Physical Society 2024
Abstract Dynamically probing systems of ultrastrongly coupled light and matter by advanced coherent control have been recently proposed as a unique tool for detecting peculiar quantum features of this regime. Coherence allows in principle on-demand conversion of virtual photons dressing the entangled eigenstates of the system to real ones, with unitary efficiency and remarkable robustness. Here, we study this effect in the presence of decoherence, showing that also in far from ideal regimes is it possible to probe such peculiar features.
Reaching the strong coupling regime of light-matter interaction has led to an impressive development in fundamental quantum physics and applications to quantum information processing. Latests advances in different quantum technologies, like superconducting circuits or semiconductor quantum wells, show that the ultrastrong coupling regime (USC) can also be achieved, where novel physical phenomena and potential computational benefits have been predicted. Nevertheless, the lack of effective decoupling mechanism in this regime has so far hindered control and measurement processes. Here, we propose a method based on parity symmetry conservation that allows for the generation and reconstruction of arbitrary states in the ultrastrong coupling regime of light-matter interactions. Our protocol requires minimal external resources by making use of the coupling between the USC system and an ancillary two-level quantum system.
In the last decades, the experimental and theoretical study of light-matter interactions in confined quantum systems has allowed to considerably widen and deepen our understanding of the quantum world.The simplest fully-quantized light-matter interaction is the quantum Rabi model (QRM), where a two-level system is coupled to a single bosonic mode.The implementation of quantum-optical systems in which the interaction strength overcomes losses brought a revolution to this research area.Under this condition, dubbed strong coupling (SC) regime, quantum processes can be observed at the single-photon level, and even exploited to perform Quantum Information tasks.Recent developments in solid-state Quantum Technologies have made possible to push the line further, achieving the ultrastrong coupling (USC) regime of the QRM, in which the interaction strength is comparable with the bare frequencies of the interacting systems.In the USC regime of the QRM, light and matter degrees of freedom merge into collective bound states called polaritons, the system ground state is not the vacuum and excitations are not conserved.The growing interest in USC-related phenomena is mainly motivated by the fundamental counterintuitive modifications to light-matter interactions entailed by this regime.At the same time, the USC regime is also expected to provide computational benefits in terms of operational speed, coherence time, and noise protection.In this Thesis, we theoretically analyze novel quantum phenomena emerging in the USC regime, which can be observed using nowadays technology and can motivate foreseeable improvements.The results here presented have been derived using two conceptually different approaches.On one side, we have analyzed interesting models that can be implemented in superconducting circuits, a quantum platform where the USC regime can be naturally achieved.In particular, we focused on excitation transfer across USC impurities, entanglement generation via modulation of electrical boundary conditions and quantum state engineering in ultrastrongly-coupled systems.On the other hand, we have developed methods to reproduce the physics of light-matter interactions in the USC regime, by tailoring the Hamiltonian of atomic systems, like trapped ions and cold atoms.These proposals take profit of the specific features of such quantum platforms, in order to implement regimes and measurements that are not directly accessible.We believe that this Thesis will contribute to develop a thorough understanding of quantum phenomena related to the USC regime of light-matter interaction, and that it will foster the dialog between experimental and theoretical research in this area.I would like to thank first my PhD supervisor Prof. Enrique Solano, for his constant support and invaluable guidance.Countless thought-provoking discussions held with him during my PhD studies have contributed to develop my critical skills, and his advice has covered all facets of nowadays top-level research.
Ultrastrong coupling between light and matter has, in the past decade, transitioned from a theoretical idea to an experimental reality. It is a new regime of quantum light–matter interaction, which goes beyond weak and strong coupling to make the coupling strength comparable to the transition frequencies in the system. The achievement of weak and strong coupling has led to increased control of quantum systems and to applications such as lasers, quantum sensing, and quantum information processing. Here we review the theory of quantum systems with ultrastrong coupling, discussing entangled ground states with virtual excitations, new avenues for nonlinear optics, and connections to several important physical models. We also overview the multitude of experimental setups, including superconducting circuits, organic molecules, semiconductor polaritons, and optomechanical systems, that have now achieved ultrastrong coupling. We conclude by discussing the many potential applications that these achievements enable in physics and chemistry.
Light-Matter Interaction – from Strong to Ultrastrong Coupling in Superconducting Quantum Circuits Rudolf Gross TU Munchen / Walther-Meisner-Institut fur Tieftemperaturforschung Superconducting quantum circuits imple-mented by nanostructured superconduc-tors allow for the investigation of funda-mental quantum phenomena on a macro-scopic scale and the implementation of solid state quantum information systems. A big advantage of superconducting quantum two-level systems (qubits) over natural atoms is their design flexibility and wide tunability by means of external control parameters such as magnetic fields. We address the coupling of superconducting flux qubits [1,2] to on-chip microwave resonators, giv-ing rise to the prospering field of superconducting circuit quantum electrodynamics (c-QED), which allows us to study the fundamental interaction between artificial solid state atoms and single microwave photons as the basis for communicating quantum information. Recently, we succeeded to realize for the first time c-QED systems operating in the ultra-strong coupling re-gime, where the atom-cavity coupling rate reaches a considerable fraction of the atom transi-tion frequency [3]. In this regime new objects are formed consisting of matter and light. We present spectroscopy data on these new objects providing insight into novel phenomena that could not be studied in atom cavity-QED so far. We also address the interplay of multi-photon processes and symmetries in a qubit-resonator system by spectroscopically analyzing a super-conducting qubit-resonator system under oneand two-photon driving [4]. [1] T. Niemczyk et al., Supercond. Sci. Techn. 22, 034009 (2009). [2] F. Deppe et al., PRB 76, 214503 (2007); K. Kakuyanagi, et al., PRL 98, 047004 (2007). [3] T. Niemczyk et al., Nature Physics 6, 772-776 (2010). [4] F. Deppe et al., Nature Physics 4, 686 (2008); T. Niemczyk et al., arXiv:1107.0810v1 (2011). Gastgeber: Prof. Martin Dressel, Universitat Stuttgart, Telefon: 0711 685-64946