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arXiv:1707.03836 · Physical review. B./Physical review. B

Thermal transport in a two-dimensional Z 2 spin liquid

Alexandros Metavitsiadis, Angelo Pidatella, Wolfram Brenig

Published Nov 13, 2017• 34 citations
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Abstract

We study the dynamical thermal conductivity of the two-dimensional Kitaev spin model on the honeycomb lattice. We find a strongly temperature dependent low-frequency spectral intensity as a direct consequence of fractionalization of spins into mobile Majorana matter and a static ${\mathbb{Z}}_{2}$ gauge field. The latter acts as an emergent thermally activated disorder, leading to the appearance of a pseudogap which closes in the thermodynamic limit, indicating a dissipative heat conductor. Our analysis is based on complementary calculations of the current correlation function, comprising exact diagonalization by means of a complete summation over all gauge sectors, as well as a phenomenological mean-field treatment of thermal gauge fluctuations, valid at intermediate and high temperatures. The results will also be contrasted against the conductivity discarding gauge fluctuations.

DOI
10.1103/physrevb.96.205121

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We study the dynamical thermal conductivity of the two-dimensional Kitaev spin model on the honeycomb lattice. We find a strongly temperature dependent low-frequency spectral intensity as a direct consequence of fractionalization of spins into mobile Majorana matter and a static Z2{\mathbb{Z}}_{2}Z2​ gauge field. The latter acts as an emergent thermally activated disorder, leading to the appearance of a pseudogap which closes in the thermodynamic limit, indicating a dissipative heat conductor. Our analysis is based on complementary calculations of the current correlation function, comprising exact diagonalization by means of a complete summation over all gauge sectors, as well as a phenomenological mean-field treatment of thermal gauge fluctuations, valid at intermediate and high temperatures. The results will also be contrasted against the conductivity discarding gauge fluctuations.
We study the dynamical thermal conductivity of the Kitaev spin model on a two-leg ladder. In contrast to the majority of conventional one-dimensional spin systems, we show the ladder to exhibit no ballistic channel and a zero-frequency pseudogap. This is a direct consequence of the fractionalization of spins into mobile Majorana matter and a static Z2{\mathbb{Z}}_{2}Z2​ gauge field, which acts as an emergent thermally activated disorder. Our finding rests on complementary calculations of the current correlation function, comprising a phenomenological mean-field treatment of thermal gauge fluctuations, a complete summation over all gauge sectors, as well as exact diagonalization of the original spin model. The results will also be contrasted against the conductivity discarding gauge fluctuations.
We study the self-energy of phonons, magnetoelastically coupled to the two-dimensional Kitaev spin model on the honeycomb lattice. Fractionalization of magnetic moments into mobile Majorana matter and a static Z2{\mathbb{Z}}_{2}Z2​ gauge field lead to a continuum of relaxation processes comprising two channels. Thermal flux excitations, which act as an emergent disorder, strongly affect the phonon renormalization. Above the flux proliferation temperature, the dispersion of a narrow quasiparticle-hole channel is suppressed in favor of broad and only weakly momentum-dependent features, covering large spectral ranges. Our analysis is based on complementary calculations in the low-temperature homogeneous gauge and a mean-field treatment of thermal gauge fluctuations, valid at intermediate and high temperatures.
We study the energy-density dynamics at finite momentum of the two-dimensional Kitaev spin model on the honeycomb lattice. Due to fractionalization of magnetic moments, the energy relaxation occurs through mobile Majorana matter, coupled to a static Z2{\mathbb{Z}}_{2}Z2​ gauge field. At finite temperatures, the Z2{\mathbb{Z}}_{2}Z2​ flux excitations act as a thermally induced disorder, which strongly affects the energy dynamics. We show that sufficiently far above the flux proliferation temperature, but not yet in the high-temperature classical regime, disordered gauge configurations modify the coherent low-temperature energy-density dynamics into a form which is almost diffusive, with a diffusion kernel that is nearly momentum independent, but which remains retarded, primarily due to the presence of two distinct relaxation channels of particle-hole and particle-particle nature. Relations to the thermal conductivity are clarified. Our analysis is based on complementary calculations in the low-temperature homogeneous gauge configuration and a mean-field treatment of thermal gauge fluctuations, valid above the flux proliferation temperature.
We present a study of longitudinal thermal transport in the Kitaev spin model on the honeycomb lattice, focusing on the role of anisotropic exchange to cover both gapless and gapped phases. Employing a complementary combination of exact diagonalization on small systems and an average gauge configuration approach for up to $\ensuremath{\sim}O({10}^{4})$ spinful sites, we report results for the dynamical energy current autocorrelation function as well as the dc thermal conductivity over a wide range of temperatures and exchange anisotropies. Despite a pseudogap in the current correlation spectra, induced by emergent thermal gauge disorder on any finite system, we find that in the thermodynamic limit, gapless and gapful phases both feature normal dissipative transport, with a temperature dependence crossing over from power law to exponentially activated behavior upon gap opening.
Thermal Fractionalization of Quantum Spins in a Kitaev Model: Coherent Transport of Majorana Fermions and TTT-linear Specific Heat
Finite-temperature (TTT) properties of a Kitaev model defined on a honeycomb lattice are investigated by a quantum Monte Carlo simulation, from the viewpoint of fractionalization of quantum S=1/2S=1/2S=1/2 spins into two types of Majorana fermions, itinerant and localized. In this system, the entropy is released successively at two well-separated TTT scales, as a clear indication of the thermal fractionalization. We show that the high-TTT crossover, which is driven by itinerant Majorana fermions, is closely related with the development of nearest-neighbor spin correlations. On the other hand, the low-TTT crossover originates in thermal fluctuations of fluxes composed of localized Majorana fermions, by which the spectrum of itinerant Majorana fermions is significantly disturbed. As a consequence, in the intermediate-TTT range, the system exhibits coherent transport of Majorana fermions and TTT-linear behavior in the specific heat, despite the Dirac semimetallic spectrum in the low-TTT limit. We also show that the flux fluctuations affect the gapless-gapped phase boundary. Our results indicate that the fractionalization is experimentally observable in spin correlations, specific heat, and transport properties.
The long-sought quantum spin liquid is a quantum-entangled magnetic state leading to the fractionalization of spin degrees of freedom. Quasiparticles emergent from the fractionalization affect not only the ground-state properties but also thermodynamic behavior in a peculiar manner. Here we investigate how the spin dynamics evolves from the high-temperature paramagnet to the quantum spin-liquid ground state, for the Kitaev spin model describing the fractionalization into itinerant matter fermions and localized Z2{Z}_{2}Z2​ fluxes. Beyond the previous studies [J. Yoshitake, J. Nasu, and Y. Motome, Phys. Rev. Lett. 117, 157203 (2016); J. Yoshitake, J. Nasu, Y. Kato, and Y. Motome, Phys. Rev. B 96, 024438 (2017)], in which the mean-field nature of the cluster dynamical mean-field theory prevented us from studying low-temperature properties, we develop a numerical technique by applying the continuous-time quantum Monte Carlo (CTQMC) method to statistical samples generated by the quantum Monte Carlo (QMC) method in a Majorana fermion representation. This QMC+CTQMC method is fully unbiased and enables us to investigate the low-temperature spin dynamics dominated by thermally excited Z2{Z}_{2}Z2​ fluxes, including the unconventional phase transition caused by Z2{Z}_{2}Z2​ flux loops in three dimensions, which was unreachable by the previous methods. We apply this technique to the Kitaev model in both two and three dimensions. Our results clearly distinguish two cases: while the dynamics changes smoothly through the crossover in the two-dimensional honeycomb case, it exhibits singular behaviors at the phase transition in the three-dimensional hyperhoneycomb case. We show that the low-temperature spin dynamics is a sensitive probe for thermally fluctuating Z2{Z}_{2}Z2​ fluxes that behave very differently between two and three dimensions.