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arXiv:1707.03681 · Physical Review A

Polariton spectrum of the Dicke-Ising model

Erika Cortese, Luigi Garziano, Simone De Liberato

Published Nov 28, 2017• 19 citations
arXivHTMLPDF

Abstract

The Dicke-Ising model describes cavity quantum electrodynamics setups in which dipoles couple not only with the photonic cavity field but also with each other through dipole-dipole interaction. In this work we diagonalize such a model in terms of bosonic polaritonic operators for arbitrarily large values of the light-matter coupling and for values of the dipole-dipole interaction until the onset of the ferromagnetic Ising phase transition. In order to accomplish this task we exploit higher-order terms of the Holstein-Primakoff transformation, developing a general method which allows us to solve the normal phase of the Ising model in terms of bosonic excitations for large values of the dipole-dipole interaction. Our results shed light on the interplay between the dipole-dipole and light-matter coupling strengths and their effect on the virtual excitations which populate the ground state when the interactions become comparable with the bare transition frequency.

DOI
10.1103/physreva.96.053861

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The Dicke-Ising model describes cavity quantum electrodynamics setups in which dipoles couple not only with the photonic cavity field but also with each other through dipole-dipole interaction. In this work we diagonalize such a model in terms of bosonic polaritonic operators for arbitrarily large values of the light-matter coupling and for values of the dipole-dipole interaction until the onset of the ferromagnetic Ising phase transition. In order to accomplish this task we exploit higher-order terms of the Holstein-Primakoff transformation, developing a general method which allows us to solve the normal phase of the Ising model in terms of bosonic excitations for large values of the dipole-dipole interaction. Our results shed light on the interplay between the dipole-dipole and light-matter coupling strengths and their effect on the virtual excitations which populate the ground state when the interactions become comparable with the bare transition frequency.
In this paper, we reveal a second-order phase transition for the Dicke model with the dipole–dipole interaction between the atoms. By means of Holstein–Primakoff transformation, the energy spectra for both the normal and superradiant phases are explicitly obtained and therefore the scaling behaviour near the critical transition point can be given clearly. It is also shown that the dipole–dipole interactions between the atoms deeply affect the critical transition point, the ground-state and excitation energies and the scaled atomic inversion in the ground state.
We gain quantitative insights on effects of light-matter interactions on correlated quantum matter by quantum Monte Carlo simulations. We introduce a wormhole algorithm for the paradigmatic Dicke-Ising model which combines the light-matter interaction of the Dicke model with Ising interactions. The quantum phase diagrams for ferro- and antiferromagnetic interactions on the chain and the square lattice are determined. The occurring superradiant phase transitions are in the same universality class as the Dicke model, leading to a well-known peculiar finite-size scaling that we elucidate in terms of scaling above the upper critical dimension. For the ferromagnetic case, the transition between the normal and the superradiant phase is of second order with Dicke criticality (first order) for large (small) longitudinal fields separated by a multicritical point. For antiferromagnetic interactions, we establish the light-matter analog of a lattice supersolid with off-diagonal superradiant and diagonal magnetic order and determine the nature of all transition lines. Our achievements allow to quantitatively enter the domain of mesoscopic light-matter systems, which is an increasingly prominent topic at the interface of quantum optics and condensed matter physics.
In the thermodynamic limit, the Dicke-Ising chain maps exactly onto an effective self-consistent matter Hamiltonian with the photon field acting solely as a self-consistent effective field. As a consequence, no quantum correlations between photons and spins are needed to understand the quantum phase diagram. This enables us to determine the quantum phase diagram in the thermodynamic limit using numerical linked-cluster expansions combined with density matrix renormalization group calculations (NLCE+DMRG) to solve the resulting self-consistent matter Hamiltonian. This includes magnetically ordered phases with significantly improved accuracy compared to previous estimates. For ferromagnetic Ising couplings, we refine the location of the multicritical point governing the change in the order of the superradiant phase transition, reaching a relative accuracy of 10−410^{-4}10−4. For antiferromagnetic Ising couplings, we confirm the existence of the narrow antiferromagnetic superradiant phase in the thermodynamic limit. The effective matter Hamiltonian framework identifies the antiferromagnetic superradiant phase as the many-body ground state of an antiferromagnetic transverse-field Ising model with longitudinal field. This phase emerges through continuous Dicke-type polariton condensation from the antiferromagnetic normal phase, followed by a first-order transition to the paramagnetic superradiant phase. Thus, NLCE+DMRG provides a precise determination of the Dicke-Ising phase diagram in one dimension by solving the self-consistent effective matter Hamiltonian.
A potential phase transition between a normal ground state and a photon-condensed ground state in many-dipole light-matter systems is a topic of considerable controversy, exacerbated by conflicting no-go and counter no-go theorems and often ill-defined models. We contribute to the clarification of this long-lasting debate by analyzing two specific arrangements of atoms, including a three-dimensional cubic lattice and a cavity-embedded square lattice layer—which provides a physical model for single-mode cavity QED with coupled dipoles in the thermodynamic limit. These models are shown to significantly differ from the standard Dicke model and, in the thermodynamic limit, give rise to renormalized Hopfield models. We show that a ferroelectric phase transition can, in principle, still occur and the description of the abnormal phase beyond the critical point requires the inclusion of nonlinear terms in the Holstein-Primakoff mapping. We also demonstrate how our model agrees with recent experiments.
We investigate a generalized Dicke model by introducing two interacting spin ensembles coupled with a single-mode bosonic field. Apart from the normal to superradiant phase transition induced by the strong spin-boson coupling, interactions between the two spin ensembles enrich the phase diagram by introducing ferromagnetic, antiferromagnetic and paramagnetic phases. The mean-field approach reveals a phase diagram comprising three phases: paramagnetic-normal phase, ferromagnetic-superradiant phase, and antiferromagnetic-normal phase. Ferromagnetic spin-spin interaction can significantly reduce the required spin-boson coupling strength to observe the superradiant phase, where the macroscopic excitation of the bosonic field occurs. Conversely, antiferromagnetic spin-spin interaction can strongly suppress the superradiant phase. To examine higher-order quantum effects beyond the mean-field contribution, we utilize the Holstein-Primakoff transformation, which converts the generalized Dicke model into three coupled harmonic oscillators in the thermodynamic limit. Near the critical point, we observe the close of the energy gap between the ground and the first excited states, the divergence of entanglement entropy and quantum fluctuation in certain quadrature. These observations further confirm the quantum phase transition and offer additional insights into critical behaviors.
The dissipative phase transitions in the open transverse and longitudinal Dicke-Ising model (DIM), which incorporates nearest-neighbor Ising-type spin interactions into the Dicke framework, are investigated within a mean-field approach and further validated by detailed stability analysis. While the dissipative phase diagram of the transverse DIM is only slightly shifted upward compared with its ground-state counterpart, dissipation in the longitudinal DIM stabilizes bistable nonequilibrium steady states and induces first-order phase transitions that are absent in the ground-state phase diagram. This bistable phase is characterized by the coexistence of superradiant and antiferromagnetic orders, and it converts a ground-state triple point into a tetracritical point, at which the boundaries of the first- and second-order transitions intersect. Our results reveal that the interplay among spin interactions, light-matter coupling, and dissipation supports a diverse set of nonequilibrium phase transitions and provides broad tunability of the phase diagram. These findings offer a theoretical foundation for exploring nonequilibrium physics in realistic open solid-state quantum systems.