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arXiv:1706.08095 · Physical review. B./Physical review. B

Robust electric dipole transition at microwave frequencies for nuclear spin qubits in silicon

G. Tosi, Fahd A. Mohiyaddin, Stefanie Tenberg, Arne Laucht, Andrea Morello

Published Aug 30, 2018• 20 citations
arXivHTMLPDF

Abstract

The nuclear spin state of a phosphorus donor ($^{31}\mathrm{P}$) in isotopically enriched silicon-28 is an excellent host to store quantum information in the solid state. The spin's insensitivity to electric fields yields a solid-state qubit with record coherence times but also renders coupling to other quantum systems very challenging. Here, we describe how to generate a strong electric dipole ($>100$ D) at microwave frequencies for the nuclear spin. This is achieved by applying a magnetic drive to the spin of the donor-bound electron while simultaneously controlling its charge state with electric fields. Under certain conditions, the microwave magnetic drive also renders the nuclear spin resonance frequency and electric dipole strongly insensitive to electrical noise, yielding long ($>1$ ms) dephasing times and robust gate operations. The nuclear spin could then be strongly coupled to microwave resonators, with a vacuum Rabi splitting of the order of 1 MHz, or to other nuclear spins, nearly half a micrometer apart, via strong electric dipole-dipole interaction. This work brings the $^{31}\mathrm{P}$ nuclear qubit into the realm of hybrid quantum systems and opens up new avenues in quantum information processing.

DOI
10.1103/physrevb.98.075313

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The nuclear spin state of a phosphorus donor (31P^{31}\mathrm{P}31P) in isotopically enriched silicon-28 is an excellent host to store quantum information in the solid state. The spin's insensitivity to electric fields yields a solid-state qubit with record coherence times but also renders coupling to other quantum systems very challenging. Here, we describe how to generate a strong electric dipole (>100>100>100 D) at microwave frequencies for the nuclear spin. This is achieved by applying a magnetic drive to the spin of the donor-bound electron while simultaneously controlling its charge state with electric fields. Under certain conditions, the microwave magnetic drive also renders the nuclear spin resonance frequency and electric dipole strongly insensitive to electrical noise, yielding long (>1>1>1 ms) dephasing times and robust gate operations. The nuclear spin could then be strongly coupled to microwave resonators, with a vacuum Rabi splitting of the order of 1 MHz, or to other nuclear spins, nearly half a micrometer apart, via strong electric dipole-dipole interaction. This work brings the 31P^{31}\mathrm{P}31P nuclear qubit into the realm of hybrid quantum systems and opens up new avenues in quantum information processing.
The spins of atoms and atom-like systems are among the most coherent objects in which to store quantum information. However, the need to address them using oscillating magnetic fields hinders their integration with quantum electronic devices. Here, we circumvent this hurdle by operating a single-atom "flip-flop" qubit in silicon, where quantum information is encoded in the electron-nuclear states of a phosphorus donor. The qubit is controlled using local electric fields at microwave frequencies, produced within a metal-oxide-semiconductor device. The electrical drive is mediated by the modulation of the electron-nuclear hyperfine coupling, a method that can be extended to many other atomic and molecular systems and to the hyperpolarization of nuclear spin ensembles. These results pave the way to the construction of solid-state quantum processors where dense arrays of atoms can be controlled using only local electric fields.
Practical quantum computers require a large network of highly coherent qubits, interconnected in a design robust against errors. Donor spins in silicon provide state-of-the-art coherence and quantum gate fidelities, in a platform adapted from industrial semiconductor processing. Here we present a scalable design for a silicon quantum processor that does not require precise donor placement and leaves ample space for the routing of interconnects and readout devices. We introduce the flip-flop qubit, a combination of the electron-nuclear spin states of a phosphorus donor that can be controlled by microwave electric fields. Two-qubit gates exploit a second-order electric dipole-dipole interaction, allowing selective coupling beyond the nearest-neighbor, at separations of hundreds of nanometers, while microwave resonators can extend the entanglement to macroscopic distances. We predict gate fidelities within fault-tolerance thresholds using realistic noise models. This design provides a realizable blueprint for scalable spin-based quantum computers in silicon.Quantum computers will require a large network of coherent qubits, connected in a noise-resilient way. Tosi et al. present a design for a quantum processor based on electron-nuclear spins in silicon, with electrical control and coupling schemes that simplify qubit fabrication and operation.
The nuclear spin of a phosphorus atom in silicon is considered as a promising quantum information carrier for quantum computing due to its long coherence time. Coherent control of the nuclear spin is typically realized using nuclear magnetic resonance (NMR). In this work, we theoretically propose that with the aid of hyperfine interactions and magnetic field gradients, fast electric-dipole-induced nuclear electric resonance (EDNER) can be achieved. The stronger EDNER (compared with NMR) arises from the combined effects of hyperfine interaction between the nuclear and electron spins and coupling between the electron spin and charge degrees of freedom mediated by magnetic field gradients in this scheme. By operating at specific working points, the nuclear-spin splitting becomes less sensitive to electrical noise, enabling long coherence times and high-fidelity quantum operations. All elctrical, addressable control of nuclear spins paves the way for scalable silicon-based quantum computing.
A high degree of controllability and long coherence time make the nuclear spin of a phosphorus donor in isotopically purified silicon a promising candidate for a quantum bit. However, long-distance two-qubit coupling and fast, robust gates remain outstanding challenges for these systems. Here, following recent proposals for long-distance coupling via dipole-dipole interactions, we present a simple method to implement fast, high-fidelity arbitrary single- and two-qubit gates in the absence of charge noise. Moreover, we provide a method to make the single-qubit gates robust to moderate levels of charge noise to well within an error bound of ${10}^{\ensuremath{-}3}$.
Nuclear spins show exceptionally long coherence times but the underlying good isolation from their environment is a challenge when it comes to controlling nuclear spin qubits. A particular difficulty, not only for nuclear spin qubits, is the realization of two-qubit gates between distant qubits. Recently, strong coupling between an electron spin and microwave resonator photons as well as a microwave resonator mediated coupling between two electron spins both in the resonant and the dispersive regime have been reported and, thus, a microwave resonator mediated electron spin two-qubit gate seems to be in reach. Inspired by these findings, we theoretically investigate the interaction of a microwave resonator with a hybrid quantum dot-donor (QDD) system consisting of a gate-defined Si QD and a laterally displaced 31P^{31}\mathrm{P}31P phosphorous donor atom implanted in the Si host material. We find that driving the QDD system allows to compensate the frequency mismatch between the donor nuclear spin splitting in the MHz regime and typical superconducting resonator frequencies in the GHz regime, and also enables an effective nuclear spin-photon coupling. While we expect this coupling to be weak, we predict that coupling the nuclear spins of two distant QDD systems dispersively to the microwave resonator allows the implementation of a resonator-mediated nuclear spin two-qubit iSWAP\sqrt{i\mathrm{SWAP}}iSWAP​ gate with a gate fidelity approaching 9090%90.
Abstract Single electron spins bound to multi-phosphorus nuclear spin registers in silicon have demonstrated fast (0.8 ns) two-qubit SWAP\sqrt{\mathrm{SWAP}}SWAP​ SWAP gates and long spin relaxation times (~30 s). In these spin registers, when the donors are ionized, the nuclear spins remain weakly coupled to their environment, allowing exceptionally long coherence times. When the electron is present, the hyperfine interaction allows coupling of the spin and charge degrees of freedom for fast qubit operation and control. Here we demonstrate the use of the hyperfine interaction to enact electric dipole spin resonance to realize high-fidelity ( F=100−6+0F=10{0}_{-6}^{+0}F=100−6+0​ F = 10 0 − 6 + 0 %) initialization of all the nuclear spins within a four-qubit nuclear spin register. By controllably initializing the nuclear spins to ∣⇓⇓⇓⟩\left\vert \Downarrow \Downarrow \Downarrow \right\rangle∣⇓⇓⇓⟩ ⇓ ⇓ ⇓ , we achieve single-electron qubit gate fidelities of F = 99.78 ± 0.07% (Clifford gate fidelities of 99.58 ± 0.14%), above the fault-tolerant threshold for the surface code with a coherence time of $${T}_{2}^{\,* }=12\,\upmu {{{\rm{s}}}}$$ T 2 * = 12 μ s .