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arXiv:1706.02603 · Physical Review Letters

Quantum Slow Relaxation and Metastability due to Dynamical Constraints

Zhihao Lan, Merlijn van Horssen, Stephen Powell, Juan P. Garrahan

Published Jul 27, 2018• 121 citations
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Abstract

One of the general mechanisms that give rise to the slow cooperative relaxation characteristic of classical glasses is the presence of kinetic constraints in the dynamics. Here we show that dynamical constraints can similarly lead to slow thermalization and metastability in translationally invariant quantum many-body systems. We illustrate this general idea by considering two simple models: (i) a one-dimensional quantum analogue to classical constrained lattice gases where excitation hopping is constrained by the state of neighboring sites, mimicking excluded-volume interactions of dense fluids; and (ii) fully packed quantum dimers on the square lattice. Both models have a Rokhsar-Kivelson (RK) point at which kinetic and potential energy constants are equal. To one side of the RK point, where kinetic energy dominates, thermalization is fast. To the other, where potential energy dominates, thermalization is slow, memory of initial conditions persists for long times, and separation of timescales leads to pronounced metastability before eventual thermalization. Furthermore, in analogy with what occurs in the relaxation of classical glasses, the slow-thermalization regime displays dynamical heterogeneity as manifested by spatially segregated growth of entanglement.

DOI
10.1103/physrevlett.121.040603

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One of the general mechanisms that give rise to the slow cooperative relaxation characteristic of classical glasses is the presence of kinetic constraints in the dynamics. Here we show that dynamical constraints can similarly lead to slow thermalization and metastability in translationally invariant quantum many-body systems. We illustrate this general idea by considering two simple models: (i) a one-dimensional quantum analogue to classical constrained lattice gases where excitation hopping is constrained by the state of neighboring sites, mimicking excluded-volume interactions of dense fluids; and (ii) fully packed quantum dimers on the square lattice. Both models have a Rokhsar-Kivelson (RK) point at which kinetic and potential energy constants are equal. To one side of the RK point, where kinetic energy dominates, thermalization is fast. To the other, where potential energy dominates, thermalization is slow, memory of initial conditions persists for long times, and separation of timescales leads to pronounced metastability before eventual thermalization. Furthermore, in analogy with what occurs in the relaxation of classical glasses, the slow-thermalization regime displays dynamical heterogeneity as manifested by spatially segregated growth of entanglement.
With the aim to understand the role of the constraints in the thermalization of quantum systems, we study the dynamics of a family of kinetically constrained models arising through duality from the XXZ spin chain. We find that integrable and nonintegrable deformations around the stochastic point give rise to ground state phase transitions between localised and delocalised phases, which in turn determine the nature of the relaxation dynamics at finite energy densities. While in the delocalised phase thermalization is fast and homogeneous, in the localised phase relaxation is slow, temporal autocorrelations exhibit plateaus indicative of metastability, and the growth of entanglement is heterogeneous in space. Furthermore, by considering relaxation from initial product states, we demostrate that this slow thermalization can be rationalised directly from the presence of constraints in the dynamics.
We study in detail the properties of the quantum East model, an interacting quantum spin chain inspired by simple kinetically constrained models of classical glasses.Through a combination of analytics, exact diagonalization, and tensor-network methods, we show the existence of a transition, from a fast to a slow thermalization regime, which manifests itself throughout the spectrum.On the slow side, by exploiting the localization of the ground state and the form of the Hamiltonian, we explicitly construct a large (exponential in size) number of nonthermal states that become exact finite-energy-density eigenstates in the large size limit, as expected for a true phase transition.A "superspin" generalization allows us to find a further large class of area-law states proved to display very slow relaxation.These states retain memory of their initial conditions for extremely long times.Our numerical analysis reveals that the localization properties are not limited to the ground state and that many eigenstates have large overlap with product states and can be approximated well by matrix product states at arbitrary energy densities.The mechanism that induces localization to the ground state, and hence the nonthermal behavior of the system, can be extended to a wide range of models including a number of simple spin chains.We discuss implications of our results for slow thermalization and nonergodicity more generally in disorder-free systems with constraints, and we give numerical evidence that these results may be extended to two-dimensional systems.
We study in detail the properties of the quantum East model, an interacting quantum spin chain inspired by simple kinetically-constrained models of classical glasses. Through a combination of analytics, exact diagonalization and tensor-network methods we show the existence of a transition, from a fast to a slow thermalization regime, which manifests itself throughout the spectrum. On the slow side, by exploiting the localization of the ground state and the form of the Hamiltonian, we explicitly construct a large (exponential in size) number of non-thermal states which become exact finite-energy-density eigenstates in the large-size limit, as expected for a true phase transition. A ``super-spin'' generalization allows us to find a further large class of area-law states proved to display very slow relaxation. These states retain memory of their initial conditions for extremely long times. Our numerical analysis reveals that the localization properties are not limited to the ground state and that} many eigenstates have large overlap with product states and can be approximated well by matrix product states at arbitrary energy densities. The mechanism that induces localization to the ground state, and hence the non-thermal behavior of the system, can be extended to a wide range of models including a number of simple spin chains. We discuss implications of our results for slow thermalization and non-ergodicity more generally in disorder-free systems with constraints and we give numerical evidence that these results may be extended to two dimensional systems.
We identify the mechanism of slow heterogeneous relaxation in quantum kinetically constrained models (KCMs) in which the potential energy strength is controlled by a coupling parameter. The regime of slow relaxation includes the large-coupling limit. By expanding around that limit, we reveal a of states that remain frozen on time scales determined by powers of the coupling. The classification of such states, together with the evolution of their Krylov complexity, reveals that these time scales are related to the distance between the sites where facilitated dynamics is allowed by the kinetic constraint. While correlations within frozen states relax slowly and exhibit metastable plateaus that persist on time scales set by powers of the coupling parameter, the correlations in the rest of the states decay rapidly. We compute the plateau heights of correlations across all frozen states up to second-order corrections in the inverse coupling. Our results explain slow relaxation in quantum KCMs and elucidate dynamical heterogeneity by relating the relaxation times to the spatial separations between the active regions.
Kinetically constrained spin systems play an important role in understanding key properties of the dynamics of slowly relaxing materials, such as glasses. Recent experimental studies have revealed that manifest kinetic constraints govern the evolution of strongly interacting gases of highly excited atoms in a noisy environment. Motivated by this development we explore which types of kinetically constrained dynamics can generally emerge in quantum spin systems subject to strong noise and show how, in this framework, constraints are accompanied by conservation laws. We discuss an experimentally realizable case of a lattice gas, where the interplay between those and the geometry of the lattice leads to collective behavior and time-scale separation even at infinite temperature. This is in contrast to models of glass-forming substances which typically rely on low temperatures and the consequent suppression of thermal activation.
In the study of the thermalization of closed quantum systems, the role of kinetic constraints on the temporal dynamics and the eventual thermalization is attracting significant interest. Kinetic constraints typically lead to long-lived metastable states depending on initial conditions. We consider a model of interacting hardcore bosons with an additional kinetic constraint that was originally devised to capture glassy dynamics at high densities. As a main result, we demonstrate that the system is highly prone to localization in the presence of uncorrelated disorder. Adding disorder quickly triggers long-lived dynamics as evidenced in the time evolution of density autocorrelations. Moreover, the kinetic constraint favors localization also in the eigenstates, where a finite-size transition to a many-body localized phase occurs for much lower disorder strengths than for the same model without a kinetic constraint. Our work sheds light on the intricate interplay of kinetic constraints and localization and may provide additional control over many-body localized phases in the time domain.