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arXiv:1705.10344 · Physical Review Applied

Probing Decoherence in Plasmonic Waveguides in the Quantum Regime

S. G. Dlamini, J. T. Francis, X. Zhang, Ş. K. Özdemir, Síle Nic Chormaic, Francesco Petruccione, Mark Tame

Published Feb 6, 2018• 12 citations
arXivHTMLPDF

Abstract

$Q\phantom{\rule{0}{0ex}}u\phantom{\rule{0}{0ex}}a\phantom{\rule{0}{0ex}}n\phantom{\rule{0}{0ex}}t\phantom{\rule{0}{0ex}}u\phantom{\rule{0}{0ex}}m$ $p\phantom{\rule{0}{0ex}}l\phantom{\rule{0}{0ex}}a\phantom{\rule{0}{0ex}}s\phantom{\rule{0}{0ex}}m\phantom{\rule{0}{0ex}}o\phantom{\rule{0}{0ex}}n\phantom{\rule{0}{0ex}}i\phantom{\rule{0}{0ex}}c\phantom{\rule{0}{0ex}}s$ is an emerging field with a wide range of applications in quantum information science. Despite significant progress so far, it is not known how decoherence affects quantum plasmonic systems. This experimental study shows that damping of either amplitude or phase can lead to decoherence in these systems, and provides important information for designing plasmonic waveguide systems for loss-tolerant and phase-sensitive applications, such as quantum sensing and imaging. The techniques developed here may be useful for studying decoherence in other plasmonic structures, too, including nanoantennas, unit cells in metamaterials, and nanotraps for cold atoms.

DOI
10.1103/physrevapplied.9.024003

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Q\phantom{\rule{0}{0ex}}u\phantom{\rule{0}{0ex}}a\phantom{\rule{0}{0ex}}n\phantom{\rule{0}{0ex}}t\phantom{\rule{0}{0ex}}u\phantom{\rule{0}{0ex}}m p\phantom{\rule{0}{0ex}}l\phantom{\rule{0}{0ex}}a\phantom{\rule{0}{0ex}}s\phantom{\rule{0}{0ex}}m\phantom{\rule{0}{0ex}}o\phantom{\rule{0}{0ex}}n\phantom{\rule{0}{0ex}}i\phantom{\rule{0}{0ex}}c\phantom{\rule{0}{0ex}}s is an emerging field with a wide range of applications in quantum information science. Despite significant progress so far, it is not known how decoherence affects quantum plasmonic systems. This experimental study shows that damping of either amplitude or phase can lead to decoherence in these systems, and provides important information for designing plasmonic waveguide systems for loss-tolerant and phase-sensitive applications, such as quantum sensing and imaging. The techniques developed here may be useful for studying decoherence in other plasmonic structures, too, including nanoantennas, unit cells in metamaterials, and nanotraps for cold atoms.
Decoherence is one of the limiting factors in quantum technology. To use plasmonic components here, knowing whether the quantum properties of individual surface plasmons can be protected over long distances is crucial, yet has not been fully addressed experimentally. The authors investigate the quantum decoherence of single surface plasmons in the high-confinement regime, where the excitation's significant matter component is expected to cause prompt decoherence. Surprisingly, the coherence properties of plasmons are well preserved even in this regime, highlighting that, despite intrinsic losses, plasmonic devices can have a remarkable range of utility for quantum applications.
This thesis investigates properties of quantum states of light while travelling as surface plasmon polaritons in plasmonic waveguides and structures. The bosonic nature of SPPs has been shown in previous work by performing a Hong-Ou-Mandel interference experiment with a plasmonic scattering-based beam splitter. Here, we show the same interference with a higher statistical power thanks to an improved set-up. A visibility of 59 ± 1 % is obtained in the two-photon interference, clearly breaking the classical limit of 50 %. The importance of the phase-relations between the different modes in the beam splitter is experimentally probed. The output state of the interference is then further analyzed by a quantum state tomography set-up. This makes it possible to quantify the entanglement generated in the interference. As the interference happens in the plasmonic beam splitter, this shows, to our knowledge for the first time, entanglement generated in a plasmonic structure. Together with the recent results in terms of entanglement and coherence preservation of SPPs, this clearly shows the potential of quantum plasmonic devices. To move into the realm of applications, we also investigate theoretically the enhancements in sensitivity quantum states of light can deliver for plasmonic sensing. It is shown that despite the losses, quantum metrology techniques can be useful in an interferometer with plasmonic waveguides. Considering the strengths and successes of plasmonic sensing techniques in a wide range of fields, we envision that entangled and squeezed states of light will become a new route to push the limits in sensitivity.
Plasmonics offers sub-diffraction confinement of light, which affords enhanced coupling to emitter systems (e.g.quantum dots).This feature makes possible a range of on-chip quantum photonic components -most notably single-photon sources and switches.This potential use of plasmonics, along with the nonlinearity provided by emitter systems, opens up quantum plasmonics as a viable route to realising quantum information processing.In this setting, the excitation of single surface plasmon polaritons (SPPs) on waveguides via single photons and the confirmation of single-photon states upon output is an important goal.In the work reported here, plasmonic waveguides were experimentally probed with single photons.A measurement of the secondorder quantum coherence function yielded a value of g (2) (0) = 0.160 ± 0.002.A value less than 0.5 is indicative of single-excitation states.Furthermore, to confirm successful SPP excitation, the transverse-magnetic mode restriction and exponential decay of SPPs were verified.Having firmly established the ability to probe plasmonic waveguides in the classical and quantum regimes, quantum random number generation was implemented using a plasmonic beam splitter.The random bit sequences produced passed the NIST Statisitical Test Suite once post-processed to correct for a slightly asymmetric beamsplitter.
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The extraordinary sensitivity of plasmonic sensors is well-known in the optics and photonics community. These sensors exploit simultaneously the enhancement and the localization of electromagnetic fields close to the interface between a metal and a dielectric. This enables, for example, the design of integrated biochemical sensors at scales far below the diffraction limit. Despite their practical realization and successful commercialization, the sensitivity and associated precision of plasmonic sensors are starting to reach their fundamental classical limit given by quantum fluctuations of light-known as the shot-noise limit. To improve the sensing performance of these sensors beyond the classical limit, quantum resources are increasingly being employed. This area of research has become known as "quantum plasmonic sensing", and it has experienced substantial activity in recent years for applications in chemical and biological sensing. This review aims to cover both plasmonic and quantum techniques for sensing, and it shows how they have been merged to enhance the performance of plasmonic sensors beyond traditional methods. We discuss the general framework developed for quantum plasmonic sensing in recent years, covering the basic theory behind the advancements made, and describe the important works that made these advancements. We also describe several key works in detail, highlighting their motivation, the working principles behind them, and their future impact. The intention of the review is to set a foundation for a burgeoning field of research that is currently being explored out of intellectual curiosity and for a wide range of practical applications in biochemistry, medicine, and pharmaceutical research.