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arXiv:1705.06850 · Physical Review A

Concept of quantum timing jitter and non-Markovian limits in single-photon detection

Li‐Ping Yang, Hong X. Tang, Zubin Jacob

Published Jan 22, 2018• 11 citations
arXivHTMLPDF

Abstract

Single atoms form a model system for understanding the limits of single-photon detection. Here, we develop a non-Markovian theory of single-photon absorption by a two-level atom to place limits on the absorption (transduction) time. We show the existence of a finite rise time in the probability of excitation of the atom during the absorption event which is infinitely fast in previous Markov theories. This rise time is governed by the bandwidth of the atom-field interaction spectrum and leads to a fundamental jitter in time stamping the absorption event. Our theoretical framework captures both the weak and strong atom-field coupling regimes and sheds light on the spectral matching between the interaction bandwidth and single-photon Fock state pulse spectrum. Our work opens questions whether such jitter in the absorption event can be observed in a multimode realistic single-photon detector. Finally, we also shed light on the fundamental differences between linear and nonlinear detector outputs for single-photon Fock-state vs coherent-state pulses.

DOI
10.1103/physreva.97.013833

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Single atoms form a model system for understanding the limits of single-photon detection. Here, we develop a non-Markovian theory of single-photon absorption by a two-level atom to place limits on the absorption (transduction) time. We show the existence of a finite rise time in the probability of excitation of the atom during the absorption event which is infinitely fast in previous Markov theories. This rise time is governed by the bandwidth of the atom-field interaction spectrum and leads to a fundamental jitter in time stamping the absorption event. Our theoretical framework captures both the weak and strong atom-field coupling regimes and sheds light on the spectral matching between the interaction bandwidth and single-photon Fock state pulse spectrum. Our work opens questions whether such jitter in the absorption event can be observed in a multimode realistic single-photon detector. Finally, we also shed light on the fundamental differences between linear and nonlinear detector outputs for single-photon Fock-state vs coherent-state pulses.
We present a formula to evaluate the spontaneous emission spectra of an atom in contact with a radiation field with non-Markovian effects. This formula is written in terms of a two-time correlation of system observables and the environmental correlation function, and depends on the distance between the emitting atom and the detector. As an example, we use it to analyze the fluorescence spectra of a two level atom placed as an impurity in a photonic crystal. The radiation field within those materials has a gap or discontinuity where electromagnetic modes cannot propagate in the stationary limit. In that situation, the atomic emission occurs in the form of evanescent waves which are detected with less efficiency the farther we place the detector. The methodology presented in this paper may be useful to study the non-Markovian dynamics of any quantum open system in linear interaction with a harmonic oscillator reservoir and within the weak-coupling approximation.
The interaction between photons and a single two-level atom constitutes a fundamental paradigm in quantum physics. The nonlinearity provided by the atom leads to a strong dependence of the light-matter interface on the number of photons interacting with the two-level system within its emission lifetime. This nonlinearity unveils strongly correlated quasiparticles known as photon bound states, giving rise to key physical processes such as stimulated emission and soliton propagation. Although signatures consistent with the existence of photon bound states have been measured in strongly interacting Rydberg gases, their hallmark excitation-number-dependent dispersion and propagation velocity have not yet been observed. Here we report the direct observation of a photon-number-dependent time delay in the scattering off a single artificial atom-a semiconductor quantum dot coupled to an optical cavity. By scattering a weak coherent pulse off the cavity-quantum electrodynamics system and measuring the time-dependent output power and correlation functions, we show that single photons and two- and three-photon bound states incur different time delays, becoming shorter for higher photon numbers. This reduced time delay is a fingerprint of stimulated emission, where the arrival of two photons within the lifetime of an emitter causes one photon to stimulate the emission of another.
Single-photon detectors have achieved impressive performance and have led to a number of new scientific discoveries and technological applications. Existing models of photodetectors are semiclassical in that the field-matter interaction is treated perturbatively and time-separated from physical processes in the absorbing matter. An open question is whether a fully quantum detector, whereby the optical field, the optical absorption, and the amplification are considered as one quantum system, could have improved performance. Here we develop a theoretical model of such photodetectors and employ simulations to reveal the critical role played by quantum coherence and amplification backaction in dictating the performance. We show that coherence and backaction lead to trade-offs between detector metrics and also determine optimal system designs through control of the quantum-classical interface. Importantly, we establish the design parameters that result in a ideal photodetector with 100% efficiency, no dark counts, and minimal jitter, thus paving the route for next-generation detectors.
The temporal dynamics of large quantum systems perturbed weakly by a single excitation can give rise to unique phenomena at the quantum phase boundaries. Here, we develop a time-dependent model to study the temporal dynamics of a single photon interacting with a defect within a large system of interacting spins. Our model can lead to a single-photon detector if the system of spins is engineered to simulate a first-order quantum phase transition (QPT). We show that the absorption of a single photon pulse by an engineered defect (i.e., a nitrogen-vacancy center) can nucleate a single shot quantum measurement. This concept of a single-shot detection event (click) is different from parameter estimation which requires repeated measurements. The crucial step of amplifying the weak quantum signal occurs by coupling the defect to a system of interacting spins biased close to a QPT point. The macroscopic spin-order change during the QPT generates an amplified signal, which can be read out by a classical device. Our work paves the way for studying the temporal dynamics of large quantum systems interacting with a single photon.
We examine the dynamics of bipartite quantum entanglement between a two-level atom and the electromagnetic field. We begin with the Jaynes-Cummings model with a single field mode and examine in detail the exact time evolution of entanglement, including cases where the atomic state is initially mixed and the atomic transition is detuned from resonance. We then explore the effects of other nearby modes by calculating the exact time evolution of entanglement in more complex systems with two, three, and five field modes. For these cases we can obtain exact solutions which include the strong-coupling regime. Finally, we consider the entanglement of a two-level atom with the infinite collection of modes present in the intracavity field of a Fabre-Perot cavity. In contrast to the usual treatment of atom-field interactions with a continuum of modes using the Born-Markov approximation, our treatment in all cases describes the full non-Markovian dynamics of the atomic subsystem under general couplings. Only when an analytic expression for the infinite mode case is desired do we need to make a weak coupling assumption which at late times approximates Markovian dynamics.