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arXiv:1705.06030 · Atoms

Entanglement, Complementarity, and Vacuum Fields in Spontaneous Parametric Down-Conversion

Ralf Menzel, Axel Heuer, Peter W. Milonni

Published Feb 19, 2019• 7 citations
arXivHTMLPDF

Abstract

Using two crystals for spontaneous parametric down-conversion in a parallel setup, we observe two-photon interference with high visibility. The high visibility is consistent with complementarity and the absence of which-path information. The observations are explained as the effects of entanglement or equivalently in terms of interfering probability amplitudes and also by the calculation of a second-order field correlation function in the Heisenberg picture. The latter approach brings out explicitly the role of the vacuum fields in the down-conversion at the crystals and in the photon coincidence counting. For comparison, we show that the Hong–Ou–Mandel dip can be explained by the same approach in which the role of the vacuum signal and idler fields, as opposed to entanglement involving vacuum states, is emphasized. We discuss the fundamental limitations of a theory in which these vacuum fields are treated as classical, stochastic fields.

DOI
10.3390/atoms7010027

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Using two crystals for spontaneous parametric down-conversion in a parallel setup, we observe two-photon interference with high visibility. The high visibility is consistent with complementarity and the absence of which-path information. The observations are explained as the effects of entanglement or equivalently in terms of interfering probability amplitudes and also by the calculation of a second-order field correlation function in the Heisenberg picture. The latter approach brings out explicitly the role of the vacuum fields in the down-conversion at the crystals and in the photon coincidence counting. For comparison, we show that the Hong–Ou–Mandel dip can be explained by the same approach in which the role of the vacuum signal and idler fields, as opposed to entanglement involving vacuum states, is emphasized. We discuss the fundamental limitations of a theory in which these vacuum fields are treated as classical, stochastic fields.
Coherence can be induced or stimulated in parametric down-conversion using two or three crystals when, for example, the idler modes of the crystals are aligned. Previous experiments with induced coherence [Phys. Rev. Lett. 114, 053601 (2015)] focused on which-path information and the role of vacuum fields in realizing complementarity via reduced visibility in single-photon interference. Here we describe experiments comparing induced and stimulated coherence. Different single-photon interference experiments were performed by blocking one of the pump beams in a three-crystal setup. Each counted photon is emitted from one of two crystals and which-way information may or not be available, depending on the setup. Distinctly different results are obtained in the induced and stimulated cases, especially when a variable transmission filter is inserted between the crystals. A simplified theoretical model accounts for all the experimental results and is also used to address the question of whether the phases of the signal and idler fields in parametric down-conversion are correlated.
It is well established that spontaneous parametric down-conversion with induced coherence across two coupled interferometers results in high-visibility single-photon interference. We describe experiments in which additional photon channels are introduced such that "which-path" information is made possible and the fringe visibility in single-photon interference is reduced in accordance with basic notions of complementarity. However, these additional pathways result in nearly perfect visibility when photons are counted in coincidence. A simplified theoretical model accounts for these observations and attributes them directly to the vacuum fields at the different crystals.
Quantum spectroscopy and imaging with undetected idler photons have been demonstrated by measuring one-photon interference between the corresponding entangled signal fields from two spontaneous parametric down conversion (SPDC) crystals. In this Report, we present a new quantum optical measurement scheme utilizing three SPDC crystals in a cascading arrangement; here, neither the detection of the idler photons which interact with materials of interest nor their conjugate signal photons which do not interact with the sample is required. The coherence of signal beams in a single photon W-type path-entangled state is induced and modulated by indistinguishabilities of the idler beams and crucially the quantum vacuum fields. As a result, the optical properties of materials or objects interacting with the idler beam from the first SPDC crystal can be measured by detecting second-order interference between the signal beams generated by the other two SPDC crystals further down the set-up. This gedankenexperiment illustrates the fundamental importance of vacuum fields in generating an optical tripartite entangled state and thus its crucial role in quantum optical measurements.
We probe the principle of complementarity by performing a double-slit experiment based on entangled photons created by spontaneous parametric down-conversion from a pump mode in a TEM01-mode. Our setup brings out the need for a careful selection of the signal-idler photon pairs for our study of visibility and distinguishability. Indeed, when the signal photons interfering at the double-slit belong to this double-hump mode we obtain almost perfect visibility of the interference fringes and no "which-slit" information is available. However, when we break the symmetry between the two maxima of the mode by detecting the entangled idler photon, the paths through the slits become distinguishable and the visibility vanishes. It is the mode function of the photons selected by the detection system which decides if interference, or "which-slit" information is accessible in the experiment.
The coincidence rate in two detectors that register signal and idler photons in parametric down-conversion is calculated using a quantum description of the radiation field that extends the semiclassical theory to the resonance regime. The signal is given by a sum over paths in the joint field plus matter space, each involving a pair of sites (molecules) and six radiation field modes. It may not be factorized into amplitudes representing one-site, three-mode paths. All effects of multiple vacuum modes are accounted for by theses paths without adding a Langevin noise source. The molecular information is given by a time-ordered superoperator Green's function rather than the susceptibility ${\ensuremath{\chi}}^{(2)}$ used in the semiclassical theory.
Parametric down-conversion is a second-order nonlinear optical process annihilating a pump photon and creating a pair of photons in the signal and idler modes. Then, by using two parametric down-converters and introducing a path indistinguishability for the two generated idler modes, a quantum coherence between two conjugate signal beams can be induced. Such a double spontaneous or stimulated parametric down-conversion scheme has been used to demonstrate quantum spectroscopy and imaging with undetected idler photons via measuring one-photon interference between their correlated signal beams. Recently, we considered another quantum optical measurement scheme utilizing W-type tripartite entangled signal photons that can be generated by employing three spontaneous parametric down-conversion crystals and by inducing coherences or path-indistinguishabilities between their correlated idler beams and between quantum vacuum fields. Here, we consider an extended triple stimulated parametric down-conversion scheme for quantum optical measurement of sample properties with undetected idler and photons. Noting the real effect of vacuum field indistinguishability on the fringe visibility as well as the role of zero-point field energy in the interferometry, we show that this scheme is an ideal and efficient way to create a coherent state of W-type entangled signal photons. We anticipate that this scheme would be of critical use in further developing quantum optical measurements in spectroscopy and microscopy with undetected photons.