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arXiv:1705.03700 · Physical Review A

Electromagnetically induced transparency of ultra-long-range Rydberg molecules

Ivan Mirgorodskiy, Florian Christaller, Christoph Braun, Asaf Paris-Mandoki, Christoph Tresp, Sebastian Hofferberth

Published Jul 25, 2017• 23 citations
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Abstract

We study the impact of Rydberg molecule formation on the storage and retrieval of Rydberg polaritons in an ultracold atomic medium. We observe coherent revivals appearing in the storage and retrieval efficiency of stored photons that originate from simultaneous excitation of Rydberg atoms and Rydberg molecules in the system with subsequent interference between the possible storage paths. We show that over a large range of principal quantum numbers the observed results can be described by a two-state model including only the atomic Rydberg state and the Rydberg dimer molecule state. At higher principal quantum numbers the influence of polyatomic molecules becomes relevant and the dynamics of the system undergoes a transition from coherent evolution of a few-state system to an effective dephasing into a continuum of molecular states.

DOI
10.1103/physreva.96.011402

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We study the impact of Rydberg molecule formation on the storage and retrieval of Rydberg polaritons in an ultracold atomic medium. We observe coherent revivals appearing in the storage and retrieval efficiency of stored photons that originate from simultaneous excitation of Rydberg atoms and Rydberg molecules in the system with subsequent interference between the possible storage paths. We show that over a large range of principal quantum numbers the observed results can be described by a two-state model including only the atomic Rydberg state and the Rydberg dimer molecule state. At higher principal quantum numbers the influence of polyatomic molecules becomes relevant and the dynamics of the system undergoes a transition from coherent evolution of a few-state system to an effective dephasing into a continuum of molecular states.
The combination of electromagnetically induced transparency with the nonlinear interaction between Rydberg atoms provides an effective interaction between photons. In this Letter, we investigate the storage of optical pulses as collective Rydberg atomic excitations in a cold atomic ensemble. By measuring the dynamics of the stored Rydberg polaritons, we experimentally demonstrate that storing a probe pulse as Rydberg polaritons strongly enhances the Rydberg mediated interaction compared to the slow propagation case. We show that the process is characterized by two time scales. At short storage times, we observe a strong enhancement of the interaction due to the reduction of the Rydberg polariton group velocity down to 0. For longer storage times, we observe a further, weaker enhancement dominated by Rydberg induced dephasing of the multiparticle components of the state. In this regime, we observe a nonlinear dependence of the Rydberg polariton coherence time with the input photon number. Our results have direct consequences in Rydberg quantum optics and may enable the test of new theories of strongly interacting Rydberg systems.
The combination of electromagnetically induced transparency with the nonlinear interaction between Rydberg atoms provides an effective interaction between photons. In this Letter, we investigate the storage of optical pulses as collective Rydberg atomic excitations in a cold atomic ensemble. By measuring the dynamics of the stored Rydberg polaritons, we experimentally demonstrate that storing a probe pulse as Rydberg polaritons strongly enhances the Rydberg mediated interaction compared to the slow propagation case. We show that the process is characterized by two time scales. At short storage times, we observe a strong enhancement of the interaction due to the reduction of the Rydberg polariton group velocity down to 0. For longer storage times, we observe a further, weaker enhancement dominated by Rydberg induced dephasing of the multiparticle components of the state. In this regime, we observe a nonlinear dependence of the Rydberg polariton coherence time with the input photon number. Our results have direct consequences in Rydberg quantum optics and may enable the test of new theories of strongly interacting Rydberg systems.
High optical nonlinearities can be achieved at the single photon level by coupling the photon states to strongly interacting Rydberg excitations under the conditions of electromagnetically induced transparency. The nonlinear response in Rydberg quantum optics comes as a direct result of the long range dipole-dipole interactions via Rydberg blockade and interaction induced dephasing. In this thesis, Rydberg quantum optics experiments are performed with two spatially separated mediums with a nonlinear response at the single photon level. Two ultracold rubidium atomic clouds are tightly confined by a pair of in-vacuo aspheric lenses such that only a few Rydberg excitations can exist in each one of the clouds simultaneously. The long range character of the dipole-dipole interactions leads to the generation of quantum states of light. The effective photon-photon interactions are directly observed as an anti-correlation in the simultaneous photon retrieval as a result of the non resonant van der Waals interactions. The collective Rydberg excitations, stored in the non-overlapping mediums, experience an additional spatial non-uniform phase. In addition, we experimentally characterize the cooperative optical response of a cold atomic medium at a single photon level. This aims to exploit the enhancement of the spontaneous emissions decay rate (superradiance) as a dependence of the number of atoms involved in the ensemble. The observed atomic response in two different regimes gives a further understanding of the system dynamics and unlocks a promising potential route towards the implementation in scalable, multichannel quantum optical devices.
A comprehensive analysis of photon storage in a Rydberg state of ultracold 87{}^{87}87Rb gas based on electromagnetically induced transparency is performed both experimentally and theoretically. The theoretical model shows that the retrieval efficiency is related to the decay of fringe visibility in Ramsey spectroscopy.
Interacting Rydberg excitations in cold atomic ensembles can exhibit large quantum nonlinearities that enable engineering of strong interactions between individual photons. Consequently, Rydberg ensembles are a promising platform for quantum information applications and the study of more fundamental physics of few- and many-body phenomena with interacting photons. This thesis presents a series of experiments that study and exploit different regimes of Rydberg-mediated interactions. We report the realization of an efficient on-demand single-photon source. The strong long-range Rydberg interactions allow the excitation of only a single collective Rydberg state within the entire atomic medium. The collective excitation can be subsequently retrieved as a single-photon. We use this scheme to generate highly pure and highly indistinguishable photons, which are suitable for scalable quantum information applications. These photons can be compatible with other atomic systems due to their narrow bandwidth, which makes building practical hybrid quantum systems feasible. Here, we demonstrate high visibility two-photon quantum interference between our Rydberg-produced photons, and photons emitted by a remote single-trapped ion. We also study Rydberg atoms under electromagnetically induced transparency conditions, where coherent superpostions of photons and Rydberg excitations propagate through the atomic medium as lossless dark-state polaritons. In the experiment, we use the external control fields to tune the interactions to a many-body regime where we can observe resonant scattering of dark-state polaritons to lossy channels. We show that the enhanced scattering process arises as a pure three-body effect.
Abstract The combination of Rydberg atoms and electromagnetically induced transparency (EIT) has been extensively studied in the strong-interaction regime. Here we proposed utilizing an EIT medium with a high optical depth (OD) and a Rydberg state of low principal quantum number to create a many-body system of Rydberg polaritons in the weak-interaction regime. The phase shift and attenuation induced by the dipole–dipole interaction (DDI) were still significant, and can be viewed as the consequences of elastic and inelastic collisions among Rydberg polaritons. We further observed that the width of the transverse momentum distribution of Rydberg polaritons at the exit of the system became notably smaller as compared with that at the entrance. The observation demonstrates the cooling effect in this system. The μs-long interaction time due to the high-OD EIT medium plus the μm2-size collision cross section due to the DDI suggests a feasible platform of polariton Bose–Einstein condensation.