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arXiv:1705.01026 · Physical Review A

Supersolidity of lattice bosons immersed in strongly correlated Rydberg dressed atoms

Yongqiang Li, Andreas Geißler, Walter Hofstetter, Weibin Li

Published Feb 12, 2018• 31 citations
arXivHTMLPDF

Abstract

Recent experiments have illustrated that long-range two-body interactions can be induced by laser coupling atoms to highly excited Rydberg states. Stimulated by this achievement, we study the supersolidity of lattice bosons in an experimentally relevant situation. In our setup, we consider two-component atoms on a square lattice, where one species is weakly dressed to an electronically high-lying (Rydberg) state, generating a tunable, soft-core shape long-range interaction. Interactions between atoms of the second species and between the two species are characterized by local inter- and intraspecies interactions. Using a dynamical mean-field calculation, we find that interspecies on-site interactions can stabilize a pronounced region of supersolid phases. This is characterized by two distinctive types of supersolids, where the bare species forms supersolid phases that are immersed in strongly correlated quantum phases, i.e., a crystalline solid or supersolid of the dressed atoms. We show that the interspecies interaction leads to a rotonlike instability in the bare species and therefore is crucially important to the supersolid formation. We provide a detailed calculation of the interaction potential to show how our results can be explored under current experimental conditions.

DOI
10.1103/physreva.97.023619

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•Jan 1, 2017•2 citations
Recent experiments have illustrated that long-range two-body interactions can be induced by laser coupling atoms to highly excited Rydberg states. Stimulated by this achievement, we study the supersolidity of lattice bosons in an experimentally relevant situation. In our setup, we consider two-component atoms on a square lattice, where one species is weakly dressed to an electronically high-lying (Rydberg) state, generating a tunable, soft-core shape long-range interaction. Interactions between atoms of the second species and between the two species are characterized by local inter- and intraspecies interactions. Using a dynamical mean-field calculation, we find that interspecies on-site interactions can stabilize a pronounced region of supersolid phases. This is characterized by two distinctive types of supersolids, where the bare species forms supersolid phases that are immersed in strongly correlated quantum phases, i.e., a crystalline solid or supersolid of the dressed atoms. We show that the interspecies interaction leads to a rotonlike instability in the bare species and therefore is crucially important to the supersolid formation. We provide a detailed calculation of the interaction potential to show how our results can be explored under current experimental conditions.
We study the dynamics of bosonic atoms on a two-dimensional square lattice, where atomic interactions are long ranged with either a box or soft-core shape. The latter can be realized through laser dressing ground-state atoms to electronically excited Rydberg states. When the range of interactions is equal or larger than the lattice constant, the system is governed by an extended Bose-Hubbard model. We propose a quench process by varying the atomic hopping linearly across phase boundaries of the Mott insulator-supersolid and supersolid-superfluid phases. Starting from a Mott insulating state, the dynamical evolution of the superfluid order parameter exhibits a universal behavior at the early stage, largely independent of interactions. The dynamical evolution is significantly altered by strong, long-range interactions at later times. Particularly, we demonstrate that density wave excitation is important when the quench rate is small. Moreover, we show that the quench dynamics can be analyzed through time-of-flight images, i.e., measuring the momentum distribution and noise correlations.
Recent experiments with ultracold Rydberg-excited atoms have shown that long-range interactions can give rise to spatially ordered structures. Observation of crystalline phases in a system with Rydberg atoms loaded into an optical lattice seems also within reach. Here we investigate a bosonic model on a triangular lattice suitable for description of such experiments. Numerical simulations based on bosonic dynamical mean-field theory reveal a rich phase diagram with different supersolid phases. Comparison with the results obtained for a square lattice geometry shows qualitatively similar results in a wide range of parameters; however, on a triangular lattice we do not observe the checkerboard supersolid. Moreover, unlike on a square lattice, we did not find a phase transition from uniform superfluid to supersolid induced by increase of the hopping amplitude on a triangular lattice. Based on our results, we propose an intuitive interpretation of the nature of different supersolid phases. We also propose parameters for the experimental realization.
We study the dynamics of an atomic Bose-Einstein condensate in an optical lattice in which the electronic ground state of each atom is weakly coupled to a highly excited Rydberg state by a far off-resonant laser. This dressing induces a switchable effective soft-core interaction between ground-state atoms which, in the lattice, gives rise to on-site as well as long-range interaction terms. Upon switching on the dressing laser the coherence properties of the atomic superfluid undergo a nontrivial collapse and revival dynamics which can be observed in the interference pattern that is created after a release of the atoms from the optical lattice. This interference signal strongly depends on the strength and the duration of the dressing laser pulse and can be used to probe and characterize the effective interaction between Rydberg-dressed atoms.
We investigate a cold-atom mixture of spinless bosons and fermions in two-dimensional optical lattices. In the presence of a nested Fermi surface, the bosons may develop a fascinating supersolid behavior characterized by a finite superfluid density as well as a spatial density wave order. Focusing on the triangular lattice geometry and combining a general Landau-Ginzburg-Wilson approach with microscopically derived mean-field theory, we find an exotic supersolid phase at a fermionic band filling of nf=3∕4{n}_{f}=3∕4nf​=3∕4 with a kagome-type crystalline order. We also address the case of anisotropic hopping amplitudes and show that striped supersolid phases emerge on the square and triangular lattices. For weak interactions, the supersolid competes with phase separation. For strong intraspecies and interspecies interactions, with the total number of fermions and bosons corresponding to one particle per site, the bosons form an alternating Mott insulator ground state. Finally, for a mixture of 87Rb40K^{87}\mathrm{Rb}^{40}\mathrm{K}87Rb40K and 23Na6Li^{23}\mathrm{Na}^{6}\mathrm{Li}23Na6Li, we show that supersolidity can be observed in the range of accessible temperatures in the square lattice geometry.
Neutral atoms become strongly interacting when their electrons are excited to loosely bound Rydberg states. We investigate the strongly correlated quantum phases of matter that emerge in two-dimensional atom arrays where three Rydberg levels are used to encode an effective spin-1 degree of freedom. Dipolar exchange between such spin-1 Rydberg atoms naturally yields two distinct models: (i) a two-species hardcore boson model, and (ii) upon tuning near a Förster resonance, a dipolar spin-1 XY model. Through extensive, large-scale infinite density matrix renormalization group calculations, we provide a broad roadmap predicting the quantum phases that emerge from these models on a variety of lattice geometries: square, triangular, kagome, and ruby. We identify a wealth of correlated states, including lattice supersolids and simplex phases, all of which can be naturally realized in near-term experiments.
Interacting ultracold atomic quantum gases provide an ideal test bed to study strongly correlated quantum matter. The interactions between atoms in such an ultracold quantum gas are typically short-ranged and well described by an effective contact potential. Introducing longer-range interactions promises the realization of novel quantum phases which are absent in systems with only short-range interactions. Trapped atoms, resonantly laser-coupled to highly excited, strongly interacting Rydberg states have been proposed as a versatile platform to realize such long-range interacting quantum matter. In a first experiment presented in this thesis, we combined the single-atom-sensitive local preparation and detection enabled by a quantum gas microscope to prepare and microscopically characterize an ensemble of rubidium-87 atoms trapped in an optical lattice in the regime of strong Rydberg blockade. There, we observe collectively enhanced optical coupling in an effective two-level system, the so-called “superatom”, and infer the presence of entanglement. Detuned optical coupling to Rydberg states, termed “Rydberg dressing”, has been proposed as an alternative approach to induce long-range interactions. Rather than directly exciting an atom to a Rydberg state, the properties of the latter are admixed to a ground state, which consequently acquires long-range interactions. In the context of this thesis, we have designed a laser system in the ultraviolet spectral range to admix Rydberg P-state character to the ground state of atoms in an optical lattice. In an emerging Ising quantum magnet, the presence of Rydberg-dressed interactions was demonstrated by an interferometric technique combined with spatially resolved spin correlation measurements. The theoretically predicted tunability of the isotropy and range of the interaction were confirmed experimentally. While these initial measurements exhibited unexpected dissipation, in a subsequent experiment in a one-dimensional spin chain this dissipation was overcome. We substantiated the improved coherence times by tracking the time evolution of the magnetization upon suddenly switching on interactions and observing coherent collapse and revival dynamics, one of the hallmarks of coherent quantum evolution. Our results establish Rydberg-dressed interactions in ultracold gases and pave the way to realize and study novel exotic quantum phases.