We demonstrate the coherent coupling and the resulting transfer of phase information between microwave and optical fields in a single nitrogen vacancy center in diamond. The relative phase of two microwave fields is encoded in a coherent superposition spin state. This phase information is then retrieved with a pair of optical fields. A related process is also used for the transfer of phase information from optical to microwave fields. These studies show the essential role of dark states, including optical pumping into the dark states, in the coherent microwave-optical coupling and open the door to the full quantum state transfer between microwave and optical fields in a solid-state spin ensemble.We demonstrate the coherent coupling and the resulting transfer of phase information between microwave and optical fields in a single nitrogen vacancy center in diamond. The relative phase of two microwave fields is encoded in a coherent superposition spin state. This phase information is then retrieved with a pair of optical fields. A related process is also used for the transfer of phase information from optical to microwave fields. These studies show the essential role of dark states, including optical pumping into the dark states, in the coherent microwave-optical coupling and open the door to the full quantum state transfer between microwave and optical fields in a solid-state spin ensemble.

Physical Review LettersAug 8, 201735 citations

Quantum microwave-optical interface with nitrogen-vacancy centers in diamond

Bo Li, Fuli Li, Yuan Zhou +2 more

We propose an efficient scheme for a coherent quantum interface between microwave and optical photons using nitrogen-vacancy (NV) centers in diamond. In this setup, an NV center ensemble is simultaneously coupled to an optical and a microwave cavity. We show that, by using the collective spin excitation modes as an intermediary, quantum states can be transferred between the microwave cavity and the optical cavity through either a double-swap scheme or a dark-state protocol. This hybrid quantum interface may provide interesting applications in single microwave photon detections or quantum information processing.We propose an efficient scheme for a coherent quantum interface between microwave and optical photons using nitrogen-vacancy (NV) centers in diamond. In this setup, an NV center ensemble is simultaneously coupled to an optical and a microwave cavity. We show that, by using the collective spin excitation modes as an intermediary, quantum states can be transferred between the microwave cavity and the optical cavity through either a double-swap scheme or a dark-state protocol. This hybrid quantum interface may provide interesting applications in single microwave photon detections or quantum information processing.

arXiv:1709.04852Physical Review ASep 29, 201751 citations

Combined optical and microwave approach for performing quantum spin operations on the nitrogen-vacancy center in diamond

Forrest T. Charnock, Thomas A. Kennedy

Electron spin echoes were performed on nitrogen-vacancy $(\mathrm{N}\ensuremath{-}V)$ centers in diamond using optical polarization and detection and 35 GHz microwave control. The experiments demonstrate an approach to quantum information in the solid state. A phase memory time of $3.6 \ensuremath{\mu}\mathrm{s}$ was measured, and coupling of the electronic spin to the ${}^{14}\mathrm{N}$ nuclear spin was observed. Because of the favorable properties of the $\mathrm{N}\ensuremath{-}V$ center, interesting extensions of these single-qubit operations can be proposed.Electron spin echoes were performed on nitrogen-vacancy $(\mathrm{N}\ensuremath{-}V)$ centers in diamond using optical polarization and detection and 35 GHz microwave control. The experiments demonstrate an approach to quantum information in the solid state. A phase memory time of $3.6 \ensuremath{\mu}\mathrm{s}$ was measured, and coupling of the electronic spin to the ${}^{14}\mathrm{N}$ nuclear spin was observed. Because of the favorable properties of the $\mathrm{N}\ensuremath{-}V$ center, interesting extensions of these single-qubit operations can be proposed.

Physical review. B, Condensed matterJun 29, 200161 citations

Dressed-State Resonant Coupling between Bright and Dark Spins in Diamond

Chinmay Belthangady, Nir Bar‐Gill, Linh Pham +4 more

Under ambient conditions, spin impurities in solid-state systems are found in thermally mixed states and are optically "dark"; i.e., the spin states cannot be optically controlled. Nitrogen-vacancy (NV) centers in diamond are an exception in that the electronic spin states are "bright"; i.e., they can be polarized by optical pumping, coherently manipulated with spin-resonance techniques, and read out optically, all at room temperature. Here we demonstrate a scheme to resonantly couple bright NV electronic spins to dark substitutional-nitrogen (P1) electronic spins by dressing their spin states with oscillating magnetic fields. This resonant coupling mechanism can be used to transfer spin polarization from NV spins to nearby dark spins and could be used to cool a mesoscopic bath of dark spins to near-zero temperature, thus providing a resource for quantum information and sensing, and aiding studies of quantum effects in many-body spin systems.Under ambient conditions, spin impurities in solid-state systems are found in thermally mixed states and are optically "dark"; i.e., the spin states cannot be optically controlled. Nitrogen-vacancy (NV) centers in diamond are an exception in that the electronic spin states are "bright"; i.e., they can be polarized by optical pumping, coherently manipulated with spin-resonance techniques, and read out optically, all at room temperature. Here we demonstrate a scheme to resonantly couple bright NV electronic spins to dark substitutional-nitrogen (P1) electronic spins by dressing their spin states with oscillating magnetic fields. This resonant coupling mechanism can be used to transfer spin polarization from NV spins to nearby dark spins and could be used to cool a mesoscopic bath of dark spins to near-zero temperature, thus providing a resource for quantum information and sensing, and aiding studies of quantum effects in many-body spin systems.

Physical Review LettersApr 12, 201392 citations

Dressed-State Polarization Transfer between Bright & Dark Spins in Diamond

Chinmay Belthangady, Nir Bar‐Gill, Linh Pham +4 more

Under ambient conditions, spin impurities in solid-state systems are found in thermally-mixed states and are optically "dark", i.e., the spin states cannot be optically controlled. Nitrogen-vacancy (NV) centers in diamond are an exception in that the electronic spin states are "bright", i.e., they can be polarized by optical pumping, coherently manipulated with spin-resonance techniques, and read out optically, all at room temperature. Here we demonstrate a dressed-state, double-resonance scheme to transfer polarization from bright NV electronic spins to dark substitutional-Nitrogen (P1) electronic spins in diamond. This polarization-transfer mechanism could be used to cool a mesoscopic bath of dark spins to near-zero temperature, thus providing a resource for quantum information and sensing, and aiding studies of quantum effects in many-body spin systems.Under ambient conditions, spin impurities in solid-state systems are found in thermally-mixed states and are optically "dark", i.e., the spin states cannot be optically controlled. Nitrogen-vacancy (NV) centers in diamond are an exception in that the electronic spin states are "bright", i.e., they can be polarized by optical pumping, coherently manipulated with spin-resonance techniques, and read out optically, all at room temperature. Here we demonstrate a dressed-state, double-resonance scheme to transfer polarization from bright NV electronic spins to dark substitutional-Nitrogen (P1) electronic spins in diamond. This polarization-transfer mechanism could be used to cool a mesoscopic bath of dark spins to near-zero temperature, thus providing a resource for quantum information and sensing, and aiding studies of quantum effects in many-body spin systems.

arXiv:1211.2749Nov 12, 20120 citations

Single-Qubit Operations with the Nitrogen-Vacancy Center in Diamond

Thomas A. Kennedy, Forrest T. Charnock, John S. Colton +3 more

A concept combining optics and microwave pulses with the negative charge-state of the nitrogen-vacancy (NV—) center in diamond is demonstrated through experiments that are equivalent to single-qubit gates, and decoherence for this qubit is examined. The spin levels of the ground state provide the two-level system. Optical excitation provides polarization of these states. The polarized state is operated coherently by 35 GHz microwave pulses. The final state is read out through the photoluminescence intensity. Decoherence arises from different sources for different samples. For high-pressure, high-temperature synthetic diamonds, the high concentration of substitutional N limits the phase-memory to a few μs. In a single-crystal CVD diamond, the phase memory time is at least 32 μs at 100 K. 14N is tightly coupled to the electronic spin and produces modulation of the electron–spin echo decay under certain conditions. A two-qubit gate is proposed using this nuclear spin. This demonstration provides a great deal of insight into quantum devices in the solid state with some possibility for real application.A concept combining optics and microwave pulses with the negative charge-state of the nitrogen-vacancy (NV—) center in diamond is demonstrated through experiments that are equivalent to single-qubit gates, and decoherence for this qubit is examined. The spin levels of the ground state provide the two-level system. Optical excitation provides polarization of these states. The polarized state is operated coherently by 35 GHz microwave pulses. The final state is read out through the photoluminescence intensity. Decoherence arises from different sources for different samples. For high-pressure, high-temperature synthetic diamonds, the high concentration of substitutional N limits the phase-memory to a few μs. In a single-crystal CVD diamond, the phase memory time is at least 32 μs at 100 K. 14N is tightly coupled to the electronic spin and produces modulation of the electron–spin echo decay under certain conditions. A two-qubit gate is proposed using this nuclear spin. This demonstration provides a great deal of insight into quantum devices in the solid state with some possibility for real application.

physica status solidi (b)Oct 1, 200243 citations

{}^{14}\mathrm{N}

nuclear spin was observed. Because of the favorable properties of the $\mathrm{N}\ensuremath{-}V$ center, interesting extensions of these single-qubit operations can be proposed.