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arXiv:1704.08594 · Journal of Physics B Atomic Molecular and Optical Physics

Tuning the collective decay of two entangled emitters by means of a nearby surface

R Palacino, Roberto Passante, L Rizzuto, P Barcellona, S Y Buhmann

Published May 31, 2017• 21 citations
arXivHTMLPDF

Abstract

Abstract We consider the radiative properties of a system of two identical correlated atoms interacting with the electromagnetic field in its vacuum state in the presence of a generic dielectric environment. We suppose that the two emitters are prepared in a symmetric or antisymmetric superposition of one ground state and one excited state and we evaluate the transition rate to the collective ground state, showing distinctive cooperative radiative features. Using a macroscopic quantum electrodynamics approach to describe the electromagnetic field, we first obtain an analytical expression for the decay rate of the two entangled two-level atoms in terms of the Green’s tensor of the generic external environment. We then investigate the emission process when both atoms are in free space and, subsequently, when a perfectly reflecting mirror is present, showing how the boundary affects the physical features of the superradiant and subradiant emission by the two coupled emitters. The possibility to control and tailor radiative processes is also discussed.

DOI
10.1088/1361-6455/aa75f4

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Abstract We consider the radiative properties of a system of two identical correlated atoms interacting with the electromagnetic field in its vacuum state in the presence of a generic dielectric environment. We suppose that the two emitters are prepared in a symmetric or antisymmetric superposition of one ground state and one excited state and we evaluate the transition rate to the collective ground state, showing distinctive cooperative radiative features. Using a macroscopic quantum electrodynamics approach to describe the electromagnetic field, we first obtain an analytical expression for the decay rate of the two entangled two-level atoms in terms of the Green’s tensor of the generic external environment. We then investigate the emission process when both atoms are in free space and, subsequently, when a perfectly reflecting mirror is present, showing how the boundary affects the physical features of the superradiant and subradiant emission by the two coupled emitters. The possibility to control and tailor radiative processes is also discussed.
We consider the cooperative spontaneous emission of a system of two identical atoms interacting with the electromagnetic field in the vacuum state and in the presence of an oscillating mirror. We assume that the two atoms, one in the ground state and the other in the excited state, are prepared in a correlated (symmetric or antisymmetric) Bell-type state. We also suppose that the perfectly reflecting plate oscillates adiabatically, with the field modes satisfying the boundary conditions at the mirror surface at any given instant, so that the time dependence of the interaction Hamiltonian is entirely enclosed in the instantaneous atom-wall distance. Using time-dependent perturbation theory, we investigate the spectrum of the radiation emitted by the two-atom system, showing how the oscillation of the boundary modifies the features of the emitted spectrum, which exhibits two lateral peaks not present in the case of a static boundary. We also evaluate the transition rate to the collective ground state of the two-atom system in both cases of the superradiant (symmetric) and subradiant (antisymmetric) state. We show that it is modulated in time and that the presence of the oscillating mirror can enhance or inhibit the decay rate compared to the case of atoms in vacuum space or near a static boundary. Our results thus suggest that a dynamical (i.e., time-modulated) environment can offer further possibilities to control and manipulate radiative processes of atoms or molecules nearby, such as the cooperative decay, and strongly indicate a similar possibility for other radiative processes, for example, the resonance interaction and the energy transfer between atoms or molecules.
We analyze radiative processes of a quantum system composed by two identical two-level atoms interacting with a massless scalar field prepared in the vacuum state in the presence of perfect reflecting flat mirrors. We consider that the atoms are prepared in a stationary maximally entangled state. We investigate the spontaneous transitions rates from the entangled states to the collective ground state induced by vacuum fluctuations. In the empty-space case, the spontaneous decay rates can be enhanced or inhibited depending on the specific entangled state and changes with the distance between the atoms. Next, we consider the presence of perfect mirrors and impose Dirichlet boundary conditions on such surfaces. In the presence of a single mirror the transition rate for the symmetric state undergoes a slight reduction, whereas for the antisymmetric state our results indicate a slightly enhancement. Finally, we investigate the effect of multiple reflections by two perfect mirrors on the transition rates.
The radiative properties of quantum emitters are profoundly influenced by their electromagnetic environment. When coupled to a waveguide terminated at one end by a mirror, distant emitters interact strongly via virtual photon exchange, leading to collective superradiant and subradiant states with enhanced or suppressed decay rates. We demonstrate that applying optimal frequency shifts to each emitter enables the formation of perfect single-excitation dark states (i.e. states with zero decay rate) and near-perfect multi-excitation dark states in small ensembles. These collective states can be deterministically prepared with high fidelity using classical driving fields or few-photon pulses propagating along the waveguide. These results, readily implementable in superconducting qubit platforms, open new avenues for quantum information storage, networking and control of light.
Spontaneous emission of atoms in free space is modified by the presence of other atoms in close vicinity inducing collective super- and subradiance. For two nearby atoms with a single decay channel the entangled antisymmetric superposition state of the two single excited states will not decay spontaneously. No such excited two-atom dark state exists, if the excited state has two independent optical decay channels of different frequencies or polarizations. However, we show that for an excited atomic state with N-1 independent spontaneous decay channels one can find a highly entangled N-particle dark state, which completely decouples from the vacuum radiation field. It does not decay spontaneously, nor will it absorb resonant laser light. Mathematically, we see that this state is the only such state orthogonal to the subspace spanned by the atomic ground states. Moreover, by means of generic numerical examples we demonstrate that the subradiant behavior largely survives at finite atomic distances including dipole-dipole interactions.
Recent works have shown that collective single photon spontaneous emission from an ensemble of N resonant two-level atoms is a rich field of study. Superradiance describes emission from a completely symmetric state of N atoms, with a single excited atom prepared with a given phase, for instance imprinted by an external laser. Instead, subradiance is associated with the emission from the remaining N−1 asymmetric states, with a collective decay rate less than the single-atom value. Here, we discuss the properties of the orthonormal basis of symmetric and asymmetric states and the entanglement properties of superradiant and subradiant states.
We consider the time-dependent resonance interaction energy between two identical atoms, one in the ground state and the other in an excited state, and interacting with the vacuum electromagnetic field, during a nonequilibrium situation such as the dynamical atomic self-dressing process. We suppose the two atoms prepared in a correlated, symmetric or antisymmetric, state. Since the atoms start from a nonequilibrium conditions, their interaction energy is time dependent. We obtain, at second order in the atom-field coupling, an analytic expression for the time-dependent resonance interaction energy between the atoms. We show that this interaction vanishes when the two atoms are outside the light cone of each other, in agreement with relativistic causality, while it instantaneously settles to its stationary value after time t=R/ct=R/ct=R/c (RRR being the interatomic distance), as obtained in a time-independent approach. We also investigate the time-dependent electric energy density in the space around the two correlated atoms, in both cases of antisymmetric (subradiant) and symmetric (super-radiant) states, during the dressing process of our two-atom system. We show that the field energy density vanishes in points outside the light cone of both atoms, thus preserving relativistic causality. On the other hand, inside the light cone of both atoms, the energy density instantaneously settles to its stationary value. Specifically, for points at equal distance from the two atoms, we find that it vanishes if the two atoms are prepared in the antisymmetric (subradiant) state, while it is enhanced, with respect to the case of atoms in a factorized state, in the symmetric (super-radiant) state. The physical meaning of these results is discussed in detail in terms of interference effects of the field emitted by the two atoms.