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arXiv:1703.08339 · Physical Review A

Anderson localization of a Rydberg electron along a classical orbit

Krzysztof Giergiel, Krzysztof Sacha

Published Jun 1, 2017• 34 citations
arXivHTMLPDF

Abstract

Anderson localization is related to exponential localization of a particle in the configuration space in the presence of a disorder potential. Anderson localization can be also observed in the momentum space and corresponds to quantum suppression of classical diffusion in systems that are classically chaotic. Another kind of Anderson localization has been recently proposed, i.e., localization in the time domain due to the presence of disorder in time. That is, the probability density for the detection of a system at a fixed position in the configuration space is localized exponentially around a certain moment of time if a system is driven by a force that fluctuates in time. We show that an electron in a Rydberg atom, perturbed by a fluctuating microwave field, Anderson localizes along a classical periodic orbit. In other words the probability density for the detection of an electron at a fixed position on an orbit is exponentially localized around a certain time moment. This phenomenon can be experimentally observed.

DOI
10.1103/physreva.95.063402

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Anderson localization is related to exponential localization of a particle in the configuration space in the presence of a disorder potential. Anderson localization can be also observed in the momentum space and corresponds to quantum suppression of classical diffusion in systems that are classically chaotic. Another kind of Anderson localization has been recently proposed, i.e., localization in the time domain due to the presence of disorder in time. That is, the probability density for the detection of a system at a fixed position in the configuration space is localized exponentially around a certain moment of time if a system is driven by a force that fluctuates in time. We show that an electron in a Rydberg atom, perturbed by a fluctuating microwave field, Anderson localizes along a classical periodic orbit. In other words the probability density for the detection of an electron at a fixed position on an orbit is exponentially localized around a certain time moment. This phenomenon can be experimentally observed.
Particles in space periodic potentials constitute standard models for investigation of crystalline phenomena in solid state physics. Time periodicity of periodically driven systems is a close analogue of space periodicity of solid state crystals. There is an intriguing question if solid state phenomena can be observed in the time domain. Here we show that wave-packets localized on resonant classical trajectories of periodically driven systems are ideal elements to realize Anderson localization or Mott insulator phase in the time domain. Uniform superpositions of the wave-packets form stationary states of a periodically driven particle. However, an additional perturbation that fluctuates in time results in disorder in time and Anderson localization effects emerge. Switching to many-particle systems we observe that depending on how strong particle interactions are, stationary states can be Bose-Einstein condensates or single Fock states where definite numbers of particles occupy the periodically evolving wave-packets. Our study shows that non-trivial crystal-like phenomena can be observed in the time domain.
New experimental results are presented for short-pulse microwave ionization of highly excited hydrogen atoms. A comparison of these results with quantum numerical computations and analytical predictions provides for the first time experimentally grounded evidence of the localization phenomenon that leads to the suppression of the quantum version of the chaotic diffusion in action space occurring in the classical limit. The onset of chaotic motion in externally driven classical systems is a key problem in nonlinear dynamics that is now well understood in its essential aspects. In many physically interesting cases, as the perturbation strength increases beyond some critical value, the system starts absorbing energy in a diffusive way. The question whether “diffusive” excitation processes can take place also in externally driven quantum systems is then a very interesting one for the physics of atoms and molecules in external electromagnetic fields. This is a deep question involving the nature and the validity of the quasiclassical approximation when the underlying classical dynamics is chaotic. The question of “quantum diffusion” was first addressed in a simple model system, the kicked rotator. It was chosen because the features of classical chaos in it were relatively clean and well understood. Besides that, the numerical simulation of its quantum dynamics could be easily accomplished. The major indication of this model was that quantum mechanics suppresses the classical chaotic diffusion in action via a destructive interference effect similar to that responsible for the Anderson localization well known in condensed matter physics.
In 1958, P.W. Anderson predicted the exponential localization1 of electronic wave functions in disordered crystals and the resulting absence of diffusion. It has been realized later that Anderson localization (AL) is ubiquitous in wave physics2 as it originates from the interference between multiple scattering paths, and this has prompted an intense activity. Experimentally, localization has been reported in light waves 3 microwaves4, sound waves5, and electron gases6 but to our knowledge there is no direct observation of exponential spatial localization of matter-waves (electrons or others). We present here the observation of Anderson localization7 of a Bose-Einstein condensate (BEC) released into a one-dimensional waveguide in the presence of a controlled disorder created by laser speckle. We also show that, in our one-dimensional speckle potentials whose noise spectrum has a high spatial frequency cut-off, exponential localization occurs only when the de Broglie wavelengths of the atoms in the expanding BEC are larger than an effective mobility edge corresponding to that cut-off. In the opposite case, we find that the density profiles decay algebraically8.
Microwave ionization of Rydberg atoms is well described as the onset of classical chaos when the microwave frequency omega is less than the Kepler frequency 1/n(3). However, when omega>1/n(3), i.e., at high scaled frequency Omega=omegan(3)>1, classical ionization is predicted to be suppressed by quantum interference, an analogue to Anderson localization in a solid. Using 17.55 GHz microwave fields we have observed the ionization of Sr Rydberg atoms in the regime 1</=Omega</=5 . Our measurements demonstrate the quantum suppression of classical diffusive ionization and show the ionization field to be n independent in this regime.
In 1958, P.W. Anderson predicted the exponential localization of electronic wave functions in disordered solids, and the resulting absence of diffusion. It has been realized later that Anderson localization is ubiquitous in wave physics as it originates from the interference between multiple scattering paths, and this has prompted an intense activity to observe it with light waves, microwaves, sound waves, and electron gases, but there was no direct observation of exponential spatial localization of matterwaves (electrons or others).