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arXiv:1701.01552 · Bulletin of the American Physical Society

Topological Spin Liquid with Symmetry-Protected Edge States

Yan-Cheng Wang, Chen Fang, Meng Cheng, Chen Fang, Zi Yang Meng

Published Jan 6, 2017• 12 citations
arXivHTMLPDF

Abstract

Topological spin liquids are robust quantum states of matter with long-range entanglement and possess many exotic properties such as the fractional statistics of the elementary excitations. Yet these states, short of local parameters like all topological states, are elusive for conventional experimental probes. In this work, we combine theoretical analysis and quantum Monte Carlo numerics on a frustrated spin model which hosts a $\mathbb Z_2$ topological spin liquid ground state, and demonstrate that the presence of symmetry-protected gapless edge modes is a characteristic feature of the state, originating from the nontrivial symmetry fractionalization of the elementary excitations. Experimental observation of these modes on the edge would directly indicate the existence of the topological spin liquids in the bulk, analogous to the fact that the observation of Dirac edge states confirmed the existence of topological insulators.

DOI
10.48550/arxiv.1701.01552

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The formation of quantum spin liquids in frustrated magnets represents an exciting possibility due to the rather exotic features they harbor, including fractionalized excitations and emergent gauge fields. \nUnfortunately, they are notoriously difficult to study as there are often no good analytical methods available and quantum Monte Carlo simulations are hindered by the negative sign problem. \nThe Kitaev honeycomb model is a notable exception of a frustrated quantum model which is exactly solvable and which hosts a number of distinct quantum spin liquid ground states. \nAs such, it allows for a rare opportunity to study the physics of spin liquids with full analytical control. \n \nIn this thesis, we study the fractionalization of spin-1/2 moments into Majorana fermions and an emergent Z2 gauge field in a generalization of the Kitaev honeycomb model to a number of three-dimensional lattices. \nWhile the excitations of the gauge field are always gapped, the fermionic quasiparticles may exhibit a gapless dispersion, forming fully two-dimensional Fermi surfaces, symmetry protected nodal lines, or topological Weyl nodes. \nWe show that one can deduce rather general constraints on the possible gapless excitations by making use of an object called the projective symmetry group. \nIn doing so we provide a scheme for classifying the various gapless Kitaev spin liquids. \nA thorough analysis is carried out for a number of these spin liquids, primarily investigating the stability of the gapless modes and the novel features resulting from their sometimes non-trivial topology, as well as their effects on certain equal-time correlation functions.

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Topological spin liquids are robust quantum states of matter with long-range entanglement and possess many exotic properties such as the fractional statistics of the elementary excitations. Yet these states, short of local parameters like all topological states, are elusive for conventional experimental probes. In this work, we combine theoretical analysis and quantum Monte Carlo numerics on a frustrated spin model which hosts a Z2\mathbb Z_2Z2​ topological spin liquid ground state, and demonstrate that the presence of symmetry-protected gapless edge modes is a characteristic feature of the state, originating from the nontrivial symmetry fractionalization of the elementary excitations. Experimental observation of these modes on the edge would directly indicate the existence of the topological spin liquids in the bulk, analogous to the fact that the observation of Dirac edge states confirmed the existence of topological insulators.
Topological phases of matter are purely quantum mechanical and have no classical analogue. Most phases in nature can be classified and studied classically through the concept of symmetry breaking and its theoretical description, Landau-Ginzburg field theory. In contrast to the general wisdom of Landau-Ginzburg field theory, the topological phases share the same symmetry as a trivial insulator and still are different phases. Having gapped spectrum in bulk, they support a metallic edge excition robust against symmetry-respecting perturbation or an emergent fractional excitation in bulk. Following after fractional quantum Hall fluids, many topologically orderd phases, such as spin liquids and topological insulators, have been found and studied. Spin liquids are disordered phases of frustrated antiferromagnets and do not freeze and order even at the lowest temperature. 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As they are intrinsically quantum many-body states, the quantum field theory is an invaluable tool to explore the venue of the phases and will be used thorougly in this work. First, we present a topological field theoretic description of the topological insulators and translational symmetric Z2 spin liquid. We demostrate that abelian BF theory is an effective field theory for the two and three dimensional topological insulators. We show that the phenomenologies of BF theory are consistent with those of the topological insulators such as gapless edge and surface excitations and response functions to external gauge field. The same form of the BF theory is also applicable to study the certain classes of Z2 spin liquids with the gapless edge states. We closely examine the possible gapless edge theory of the BF theory and the translational symmetric spin liquids, and we show that the effective BF theories capture the bulk properties as well as the gapless edge spectrum of the spin liquid. Also we discuss the zero-temperature phase diagram of a thin film three dimensional topological insulators with two competing mass terms: time-reversal symmetric exciton condensation and time-reversal symmetry breaking Zeeman effect. There are two phases, quantum spin Hall phase and quantum anomalous Hall phase, and both phases support fractional excitations. We derive an effective topological field theory for the fractional excitations and examine the origin of the fractional excitations. Next we consider the relatives of the topological insulators. First we discuss the proximate symmetry broken phases of topological Mott insulator, a U(1) spin liquid with fermionic spinons in the topological insulator state. The topologically non-trivial band structure of the spinon generates the axion term for the gauge field, and we show that the axion term changes the nature of the confined phase of the spin liquid. Contrast to the conventional confined phase which has only a bond order, the confined phase of the spin liquid is in general a coexisting phase of the two different orders : a current order and a bond order. We then consider another relative of the topological insulator: a bosonic symmetry protected topological phase in two dimensional space, with both PSU(N) and time reversal symmetry. We develop an effective field theory for the phase, which is a SU(N) principal chiral model with a theta-term, and reveal the physics of the topological phase in detail.Finally we consider a topological semimetal, namely a Weyl semimetal. We first demonstrate that the Weyl semimetal can be realized in the magnetically doped topological band insulators. We explicitly derive the low energy theory of Weyl points from the general continuum Hamiltonian and tight-binding model of the topological insulators. Then we study superconducting instabilities of doped Weyl semimetals. We consider a minimal model for a Weyl semimetal and study the superconducting instabilities induced by a short-ranged attractive interaction. With the interaction, we find two competing states: a fully gapped finite-momentum pairing state and a nodal even-parity pairing state. We show that, in a mean field approximateion, the finite-momentum pairing state wins energetically against the usual even-parity paired state. We also show that exotic modes are localized at the full and half quantum vortices of the finite-momentum pairing state.
Spin liquids represent exotic types of quantum matter that evade conventional symmetry-breaking order even at zero temperature. Exhaustive classifications of spin liquids have been carried out in several systems, particularly in the presence of full SU(2) spin-rotation symmetry. Real magnetic compounds, however, generically break SU(2) spin symmetry as a result of spin-orbit coupling---which in many materials provides an ``order one'' effect. We generalize previous works by using the projective symmetry group method to classify Z2{\mathbb{Z}}_{2}Z2​ spin liquids on the square lattice when SU(2) spin symmetry is maximally lifted. We find that, counterintuitively, the lifting of spin symmetry actually results in vastly more spin-liquid phases compared to SU(2)-invariant systems. A generic feature of the SU(2)-broken case is that the spinons naturally undergo p+ipp+ipp+ip pairing; consequently, many of these Z2{\mathbb{Z}}_{2}Z2​ spin liquids feature a topologically nontrivial spinon band structure supporting gapless Majorana edge states. We study in detail several spin-liquid phases with varying numbers of gapless edge states and discuss their topological protection. The edge states are often protected by a combination of time reversal and lattice symmetries and hence resemble recently proposed topological crystalline superconductors.
Protected chiral edge modes are a well-known signature of topologically ordered phases, such as the fractional quantum Hall states (FQHS). Using the framework of projected entangled pair states (PEPS) on the square lattice, the authors construct a family of chiral spin-12\frac{1}{2}21​ quantum spin liquids with Z2{\mathbb{Z}}_{2}Z2​ gauge symmetry and analyze in full detail the properties of the edge modes. Surprisingly, the results show that the latter can be well described by a chiral conformal field theory of free bosons (SU(2)1{}_{1}1​), as is the case for the $\ensuremath{\nu}$=12\frac{1}{2}21​ (bosonic) gapped Laughlin state, despite the fact that the numerical data here suggest a critical bulk. The authors thus propose that our family of PEPS physically describes a boundary between a chiral topological phase and a trivial phase and might be closely connected to an (unknown) analogous FQHS.
Using density-matrix renormalization-group calculations for infinite cylinders, we elucidate the properties of the spin-liquid phase of the spin-$\frac{1}{2}\phantom{\rule{4pt}{0ex}}{J}_{1}\text{\ensuremath{-}}{J}_{2}$ Heisenberg model on the triangular lattice. We find four distinct ground states characteristic of a nonchiral, Z2{Z}_{2}Z2​ topologically ordered state with vison and spinon excitations. We shed light on the interplay of topological ordering and global symmetries in the model by detecting fractionalization of time-reversal and space-group dihedral symmetries in the anyonic sectors, which leads to the coexistence of symmetry protected and intrinsic topological order. The anyonic sectors, and information on the particle statistics, can be characterized by degeneracy patterns and symmetries of the entanglement spectrum. We demonstrate the ground states on finite-width cylinders are short-range correlated and gapped; however, some features in the entanglement spectrum suggest that the system develops gapless spinonlike edge excitations in the large-width limit.
Despite rapid progress in understanding gapped topological states, much less is known about gapless topological phases of matter, especially in strongly correlated electrons. In this work, we discuss a large class of robust gapless quantum spin liquids in frustrated magnets made of half-integer spins, which are described by gapless fermionic spinons coupled to dynamical Z2{\mathbb{Z}}_{2}Z2​ gauge fields. Requiring U(1)\text{U}(1)U(1) spin conservation, time-reversal, and certain space-group symmetries, we show that certain spinon symmetry fractionalization class necessarily leads to a gapless spectrum. These gapless excitations are stable against any perturbations, as long as the required symmetries are preserved. Applying these gapless criteria to spin-12\frac{1}{2}21​ systems on square, triangular, and kagome lattices, we show that all gapped symmetric Z2{\mathbb{Z}}_{2}Z2​ spin liquids in Abrikosov-fermion representation can also be realized in Schwinger-boson representation. This leads to 64 gapped Z2{\mathbb{Z}}_{2}Z2​ spin liquids on square lattice, and 8 gapped states on both kagome and triangular lattices.
The formation of quantum spin liquids in frustrated magnets represents an exciting possibility due to the rather exotic features they harbor, including fractionalized excitations and emergent gauge fields. \nUnfortunately, they are notoriously difficult to study as there are often no good analytical methods available and quantum Monte Carlo simulations are hindered by the negative sign problem. \nThe Kitaev honeycomb model is a notable exception of a frustrated quantum model which is exactly solvable and which hosts a number of distinct quantum spin liquid ground states. \nAs such, it allows for a rare opportunity to study the physics of spin liquids with full analytical control. \n \nIn this thesis, we study the fractionalization of spin-1/2 moments into Majorana fermions and an emergent Z2 gauge field in a generalization of the Kitaev honeycomb model to a number of three-dimensional lattices. \nWhile the excitations of the gauge field are always gapped, the fermionic quasiparticles may exhibit a gapless dispersion, forming fully two-dimensional Fermi surfaces, symmetry protected nodal lines, or topological Weyl nodes. \nWe show that one can deduce rather general constraints on the possible gapless excitations by making use of an object called the projective symmetry group. \nIn doing so we provide a scheme for classifying the various gapless Kitaev spin liquids. \nA thorough analysis is carried out for a number of these spin liquids, primarily investigating the stability of the gapless modes and the novel features resulting from their sometimes non-trivial topology, as well as their effects on certain equal-time correlation functions.