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arXiv:1612.06534 · Optica

Nonequilibrium phase transition in a spin-1 Dicke model

Zhang Zhiqiang, Chern Hui Lee, Ravi Kumar, K. J. Arnold, Stuart J. Masson, A. S. Parkins, M. D. Barrett

Published Mar 31, 2017• 178 citations
arXivHTMLPDF

Abstract

We realize a spin-1 Dicke model using magnetic sub-levels of the lowest F=1 hyperfine level of $^{87}$Rb atoms confined to a high finesse cavity. We study this system under conditions of imbalanced driving, which is predicted to have a rich phase diagram of nonequilibrium phases and phase transitions. We observe both super-radiant and oscillatory phases from the cavity output spectra as predicted by theory. Exploring the system over a wide range of parameters, we obtain the boundaries between the normal, super-radiant and the oscillatory phases, and compare with a theoretical model.

DOI
10.1364/optica.4.000424

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We realize a spin-1 Dicke model using magnetic sub-levels of the lowest F=1 hyperfine level of 87^{87}87Rb atoms confined to a high finesse cavity. We study this system under conditions of imbalanced driving, which is predicted to have a rich phase diagram of nonequilibrium phases and phase transitions. We observe both super-radiant and oscillatory phases from the cavity output spectra as predicted by theory. Exploring the system over a wide range of parameters, we obtain the boundaries between the normal, super-radiant and the oscillatory phases, and compare with a theoretical model.
Abstract The Dicke model describes the coupling between a quantized cavity field and a large ensemble of two‐level atoms. When the number of atoms tends to infinity, this model can undergo a transition to a superradiant phase, belonging to the mean‐field Ising universality class. The superradiant transition was first predicted for atoms in thermal equilibrium and was recently realized with a quantum simulator made of atoms in an optical cavity, subject to both dissipation and driving. This progress report offers an introduction to some theoretical concepts relevant to the Dicke model, reviewing the critical properties of the superradiant phase transition and the distinction between equilibrium and nonequilibrium conditions. In addition, it explains the fundamental difference between the superradiant phase transition and the more common lasing transition. This report mostly focuses on the steady states of atoms in single‐mode optical cavities, but it also mentions some aspects of real‐time dynamics, as well as other quantum simulators, including superconducting qubits, trapped ions, and using spin–orbit coupling for cold atoms. These realizations differ in regard to whether they describe equilibrium or nonequilibrium systems.
The Dicke model is a staple of theoretical cavity quantum electrodynamics (cavity QED), describing the interaction between an ensemble of atoms and a single radiation mode of an optical cavity. It is studied both quantum mechanically and semiclassically for two-level atoms, and demonstrates a rich variety of dynamics such as phase transitions, phase multistability, and chaos. In this work we explore an open, spin-1 Dicke model with independent co and counterrotating coupling terms as well as a quadratic Zeeman shift enabling control over the atomic energy-level structure. We investigate the stability of operator and moment equations under two approximations and show the system undergoes phase transitions. To compliment these results, we relax the aforementioned approximations and investigate the system semiclassically. We show evidence of phase transitions to steady-state and oscillatory superradiance in this semiclassical model, as well as the emergence of chaotic dynamics. The varied and complex behaviors admitted by the model highlights the need to more rigorously map its dynamics.
Present-day experiments have started to couple traditional simulations of ultracold atom experiments with quantum light-fields in cavities. This has provided a wealth of op- portunities to enlarge the number of interaction potentials: cavity mediated long-range interactions compete with kinetic energies, longitudinal fields, short-ranged collisional or magnetic spin-spin interactions. The intracavity many-body lattice models often have to be maintained far from equilibrium through the presence of external driving lasers that help to boost and engineer the various interaction potentials. The steady influx of energy is compensated by a steady stream of energy out of the atom-cavity system for example by photon losses or atomic spontaneous emission. Several experiments have demonstrated that such environments can give rise to new competing quantum phases. \nBut this long-standing ambition to push for models with tailorable interaction potentials can bring with it also considerable challenges in their theoretical description, since sponta- neous symmetry breaking transitions in many body lattice systems coupled to dynamical light-fields with single-photon character occur in the presence of drive and dissipation for the photonic force carriers. This clearly calls for model systems where the above men- tioned interplay of interactions, drive, dissipation and cooperative many-body behaviour can be theoretically studied to provide simple, experimentally verifiable predictions. \nThe Dicke model is, through its simplicity (an exactly solved ferromagnet with infinite range atom-atom interactions mediated by a single cavity mode), an exceptionally well- suited candidate. As the generic model for atom-light interactions, it has been experimen- tally realized in a variety of modern quantum optical systems, highlighting its relevance for present-day research. The Dicke model is also highly versatile itself. It has been extended into the dissipative realm, was promoted to account for multiple optical light modes and was used to describe multiple, coupled single-mode cavity structures. It was adapted to treat spin-selective coupling to a cavity to describe superradiance phase tran- sitions in multi-level atomic systems. Moreover, it was realised in electronic circuits where the dipole coupling of real atoms to single mode fields is replaced by a capacitive cou- pling of artificial atoms to a resonator mode. This illustrates that the Dicke model and its extended variants are ’future-proof’ and continue to be of relevance for fundamental light-matter interactions and for driven-dissipative phase transitions. \nIn this thesis, we investigate magnetic phase transitions in driven-dissipative atomic en- sembles interacting with quantum light. We present three research projects on variants of cooperative radiation of an ensemble of laser driven two-level atoms in a single mode optical cavity, as described by the Dicke model. \nThroughout the chapters 2,3 and 4 that contain the main body of research of this thesis, we investigate phase transitions between non-equilibrium stationary states in engineered quantum-optical systems each of which extends the conventional Dicke model physics. As a starting point, we map the quantum equations of motion onto a set of semiclassical nonlinear stochastic equations and analyse their stationary states and instabilities with master equations for atomic spin and photon mean-field amplitudes. These are used to obtain experimentally relevant parameters such as critical atom-light couplings for phase transitions, phase diagrams and properties of stationary non-equilibrium states in addition to cavity output spectra that identify the imprint of magnetic correlations in the light-field. \nIn chapter 2, we help resolve a discrepancy between earlier experimental investigations of the critical atom-light coupling strength for the superradiance transition in the Dicke model: higher external pumping strengths than theoretically predicted were needed to observe a coherent, superradiant state of the light field in an optical cavity. By including incoherent spontaneous emission of atomic excitations, we extend the dissipative Dicke model to a two loss channel variant containing both photon leakage and atomic decay that reproduces the experimentally observed critical atom-light coupling. \nRecent experiments have started to interface quantum many body lattice models with coherent cavity fields, thereby allowing to realize new quantum phases through competing atom-cavity and atom-atom interactions. In chapter 3, we consider a simplified model for such a set-up where a single quantized mode of the light-field interacts with an ensemble of Rydberg-dressed atoms inside a high finesse optical cavity. This model provides a base case for further studies of quantum magnets in optical cavities. At the heart of this model is a competition of short- (dipolar atom-atom) and long-range (atom-light) interactions at the Hamiltonian level in the presence of both spontaneous emission and photon leak- age through the cavity mirrors. We show that different magnetic phases can coexist with coherent atomic radiation and provide clear experimental signatures to identify the mag- netic structure and intra-cavity dynamics. We suggest an experimental level-scheme for a quantum optical implementation of our model. \nIn chapter 4 we consider a generic, collective decay for many-body excitations in the paradigmatic Dicke model. This extension drastically enriches the dynamics as it induces a bicritical point and a bistable regime dominated by true non-equilibrium fluctuations that induce a dissipative first-order phase transition that can only be resolved by including finite fluctuation corrections with the help of stochastic Langevin equations. We investigate the hysteretic response to time-dependent ramps of the atom-light coupling. Discontinuous first-order phase transitions where metastable states coexist in a hysteresis domain have been investigated in recent dissipative quantum-optical experiments. We review noise- activation far from thermal equilibrium in chapter 5.
Control and manipulation of quantum engineered systems allows for the utilization of time-dependent parametric modulations for accessing novel out-of-equilibrium phenomena. In the absence of such driving, the dissipative Dicke model exhibits a fascinating out-of-equilibrium many-body phase transition as a function of a coupling between a driven photonic cavity and numerous two-level atoms. We study the effect of a parametric modulation of this coupling and discover a rich phase diagram as a function of the modulation strength. We find that in addition to the established normal and super-radiant phases, a new phase with pulsed superradiance, which we term dynamical normal phase, appears when the system is parametrically driven. Employing different methods, we characterize the different phases and the transitions between them. Specific heed is paid to the role of dissipation in determining the phase boundaries. Our analysis paves the road for the experimental study of dynamically stabilized phases of interacting light and matter.
The Dicke model was proposed by Dicke in 1954 to describe a single mode of photon coupled to an assembly of N atoms with the same strength. It was found that there is a quantum phase transition from a normal phase at weak coupling to a super-radiant phase at strong coupling at the thermodynamic limit N =∞. Here, we solve the model at N ≥ 1 and also discuss its possible experimental implementations inside a cavity. By studying the Dicke model by 1/N expansion, we identify an emergent quantum phase diffusion mode inside the super-radiant phase and also work out many remarkable experimental consequences of this mode such as its low frequency, photon number squeezing properties and photon statistics. The energy of the phase diffusion modecan be continuously tuned into many frequency ranges from Micro-wave to Terahertz (THz) to Infra-red. The photons from the super-radiant phase are in a number squeezed state with much enhanced signal/noise ratio which may have wide applications in quantum information processing. The photon statistics is strong sub-Poissonian. The effects of dissipations due to leaking photons out of the cavity are also discussed. The connections with the recent experiments of the strong coupling of a BEC of N ~ 105 87Rb atoms to the photons inside an ultrahigh-finess optical cavity are carefully analyzed. Several experimental schemes to detect the phase diffusion mode are proposed.