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arXiv:1612.05249 · Physical Review Letters

Exploring Localization in Nuclear Spin Chains

Ken Xuan Wei, Chandrasekhar Ramanathan, Paola Cappellaro

Published Feb 12, 2018• 271 citations
arXivHTMLPDF

Abstract

Characterizing out-of-equilibrium many-body dynamics is a complex but crucial task for quantum applications and understanding fundamental phenomena. A central question is the role of localization in quenching thermalization in many-body systems and whether such localization survives in the presence of interactions. Probing this question in real systems necessitates the development of an experimentally measurable metric that can distinguish between different types of localization. While it is known that the localized phase of interacting systems [many-body localization (MBL)] exhibits a long-time logarithmic growth in entanglement entropy that distinguishes it from the noninteracting case of Anderson localization (AL), entanglement entropy is difficult to measure experimentally. Here, we present a novel correlation metric, capable of distinguishing MBL from AL in high-temperature spin systems. We demonstrate the use of this metric to detect localization in a natural solid-state spin system using nuclear magnetic resonance (NMR). We engineer the natural Hamiltonian to controllably introduce disorder and interactions, and observe the emergence of localization. In particular, while our correlation metric saturates for AL, it slowly keeps increasing for MBL, demonstrating analogous features to entanglement entropy, as we show in simulations. Our results show that our NMR techniques, akin to measuring out-of-time correlations, are well suited for studying localization in spin systems.

DOI
10.1103/physrevlett.120.070501

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Characterizing out-of-equilibrium many-body dynamics is a complex but crucial task for quantum applications and understanding fundamental phenomena. A central question is the role of localization in quenching thermalization in many-body systems and whether such localization survives in the presence of interactions. Probing this question in real systems necessitates the development of an experimentally measurable metric that can distinguish between different types of localization. While it is known that the localized phase of interacting systems [many-body localization (MBL)] exhibits a long-time logarithmic growth in entanglement entropy that distinguishes it from the noninteracting case of Anderson localization (AL), entanglement entropy is difficult to measure experimentally. Here, we present a novel correlation metric, capable of distinguishing MBL from AL in high-temperature spin systems. We demonstrate the use of this metric to detect localization in a natural solid-state spin system using nuclear magnetic resonance (NMR). We engineer the natural Hamiltonian to controllably introduce disorder and interactions, and observe the emergence of localization. In particular, while our correlation metric saturates for AL, it slowly keeps increasing for MBL, demonstrating analogous features to entanglement entropy, as we show in simulations. Our results show that our NMR techniques, akin to measuring out-of-time correlations, are well suited for studying localization in spin systems.
We analyze a disordered central spin model, where a central spin interacts equally with each spin in a periodic one-dimensional (1D) random-field Heisenberg chain. If the Heisenberg chain is initially in the many-body localized (MBL) phase, we find that the coupling to the central spin suffices to delocalize the chain for a substantial range of coupling strengths. We calculate the phase diagram of the model and identify the phase boundary between the MBL and ergodic phase. Within the localized phase, the central spin significantly enhances the rate of the logarithmic entanglement growth and its saturation value. We attribute the increase in entanglement entropy to a nonextensive enhancement of magnetization fluctuations induced by the central spin. Finally, we demonstrate that correlation functions of the central spin can be utilized to distinguish between MBL and ergodic phases of the 1D chain. Hence, we propose the use of a central spin as a possible experimental probe to identify the MBL phase.
The law of statistical physics dictates that generic closed quantum many-body systems initialized in nonequilibrium will thermalize under their own dynamics. However, the emergence of many-body localization (MBL) owing to the interplay between interaction and disorder, which is in stark contrast to Anderson localization, which only addresses noninteracting particles in the presence of disorder, greatly challenges this concept, because it prevents the systems from evolving to the ergodic thermalized state. One critical evidence of MBL is the long-time logarithmic growth of entanglement entropy, and a direct observation of it is still elusive due to the experimental challenges in multiqubit single-shot measurement and quantum state tomography. Here we present an experiment fully emulating the MBL dynamics with a 10-qubit superconducting quantum processor, which represents a spin-1/2 XY model featuring programmable disorder and long-range spin-spin interactions. We provide essential signatures of MBL, such as the imbalance due to the initial nonequilibrium, the violation of eigenstate thermalization hypothesis, and, more importantly, the direct evidence of the long-time logarithmic growth of entanglement entropy. Our results lay solid foundations for precisely simulating the intriguing physics of quantum many-body systems on the platform of large-scale multiqubit superconducting quantum processors.
An interacting quantum system that is subject to disorder may cease to thermalize owing to localization of its constituents, thereby marking the breakdown of thermodynamics. The key to understanding this phenomenon lies in the system's entanglement, which is experimentally challenging to measure. We realize such a many-body-localized system in a disordered Bose-Hubbard chain and characterize its entanglement properties through particle fluctuations and correlations. We observe that the particles become localized, suppressing transport and preventing the thermalization of subsystems. Notably, we measure the development of nonlocal correlations, whose evolution is consistent with a logarithmic growth of entanglement entropy, the hallmark of many-body localization. Our work experimentally establishes many-body localization as a qualitatively distinct phenomenon from localization in noninteracting, disordered systems.
The characterizing feature of a many-body localized phase is the existence of an extensive set of quasi-local conserved quantities with an exponentially localized support. This structure endows the system with the signature logarithmic in time entanglement growth between spatial partitions. This feature differentiates the phase from Anderson localization, in a non-interacting model. Experimentally measuring the entanglement between large partitions of an interacting many-body system requires highly non-local measurements which are currently beyond the reach of experimental technology. In this work we demonstrate that the defining structure of many-body localization can be detected by the dynamics of a simple quantity from quantum information known as the total correlations which is connected to the local entropies. Central to our finding is the necessity to propagate specific initial states, drawn from the Hamiltonian unbiased basis (HUB). The dynamics of the local entropies and total correlations requires only local measurements in space and therefore is potentially experimentally accessible in a range of platforms.
The non-equilibrium dynamics of disordered many-body quantum systems after a global quantum quench unveils important insights about the competition between interactions and disorder, yielding in particular an insightful perspective on many body localization (MBL). Still, the experimentally relevant effect of bond randomness in long-range interacting spin chains on the quantum quench dynamics have so far not been investigated. In this letter, we examine the entanglement entropy growth after a global quench in a quantum spin chain with randomly placed spins and long-range tunable interactions decaying with distance with power ααα. Using a dynamical version of the strong disorder renormalization group (SDRG) we find for α>αcα>α_cα>αc​ that the entanglement entropy grows logarithmically with time and becomes smaller with larger ααα as S(t)=Spln⁡(t)/(2α)S(t) = S_p \ln(t)/(2α)S(t)=Sp​ln(t)/(2α). Here, Sp=2ln⁡2−1S_p= 2 \ln2 -1Sp​=2ln2−1. We use numerical exact diagonalization (ED) simulations to verify our results for system sizes up to $ N\sim 16$ spins, yielding good agreement for sufficiently large α>αc≈1.8α> α_c \approx 1.8α>αc​≈1.8. For α<αcα<α_cα<αc​, we find that the entanglement entropy grows as a power-law with time, S(t)∼tγ(α)S(t)\sim t^{γ(α)}S(t)∼tγ(α) with 0<γ(α)<10<γ(α)<10<γ(α)<1 a decaying function of the interaction exponent ααα.
Classical statistical mechanics relies on the ergodic hypothesis, which states that a system explores the entire allowed phase space during its time evolution. Pure quantum states are at odds with this concept as they remain in a single quantum state even if the system's parameters are suddenly altered. However, in a generic many-body system, coherent dynamics drive local thermalization of its subsystems. In this case, any local observable appears thermal and can be described by a statistical ensemble even though the full state remains pure. The key to understanding the phenomenon of quantum thermalization lies in the entanglement properties of the system: The presence of entanglement creates local entropy that validates the use of statistical physics.\nIn this thesis, we experimentally study the emergence of statistical mechanics in a quantum state and observe the fundamental role of quantum entanglement in facilitating this emergence. We perform microscopy on an evolving quantum system, and we see thermalization occur on a local scale while we measure that the full quantum state remains pure.\nThe only known robust exception from the paradigm of quantum thermalization is provided by disordered systems. In this case, the particle transport ceases through the system, preventing the formation of a sufficient amount of entanglement required for thermalization. However, if the many-body system is interacting, the state develops non-local quantum correlations that are inaccessible to any local observable. These correlations spread exponentially slowly in time throughout the entire system and are considered a hallmark feature of many-body-localized states.\nIn order to study the interplay between thermalization and localization in our system, we develop novel methods for high fidelity state preparation and readout. We achieved an exquisite isolation of our system from the environment, which allows us to monitor coherent many-body dynamics over multiple decades of time evolution.\nWe experimentally realize such a many-body localized system and observe the formation of non-local quantum correlations, while the particle transport is frozen in the system. Our work experimentally establishes many-body localization as a qualitatively distinct phenomenon from localization in non-interacting, disordered systems.